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Massively parallel coherent laser ranging using a soliton microcomb 期刊论文
NATURE, 2020, 581 (7807) : 164-+
作者:  Casanova, Emmanuelle;  Knowles, Timothy D. J.;  Bayliss, Alex;  Dunne, Julie;  Baranski, Marek Z.;  Denaire, Anthony;  Lefranc, Philippe;  di Lernia, Savino;  Roffet-Salque, Melanie;  Smyth, Jessica;  Barclay, Alistair;  Gillard, Toby;  Classen, Erich;  Coles, Bryony;  Ilett, Michael;  Jeunesse, Christian;  Krueger, Marta;  Marciniak, Arkadiusz;  Minnitt, Steve;  Rotunno, Rocco;  van de Velde, Pieter;  van Wijk, Ivo;  Cotton, Jonathan;  Daykin, Andy;  Evershed, Richard P.
收藏  |  浏览/下载:44/0  |  提交时间:2020/07/03

Coherent ranging, also known as frequency-modulated continuous-wave (FMCW) laser-based light detection and ranging (lidar)(1) is used for long-range three-dimensional distance and velocimetry in autonomous driving(2,3). FMCW lidar maps distance to frequency(4,5) using frequency-chirped waveforms and simultaneously measures the Doppler shift of the reflected laser light, similar to sonar or radar(6,7) and coherent detection prevents interference from sunlight and other lidar systems. However, coherent ranging has a lower acquisition speed and requires precisely chirped(8) and highly coherent(5) laser sources, hindering widespread use of the lidar system and impeding parallelization, compared to modern time-of-flight ranging systems that use arrays of individual lasers. Here we demonstrate a massively parallel coherent lidar scheme using an ultra-low-loss photonic chip-based soliton microcomb(9). By fast chirping of the pump laser in the soliton existence range(10) of a microcomb with amplitudes of up to several gigahertz and a sweep rate of up to ten megahertz, a rapid frequency change occurs in the underlying carrier waveform of the soliton pulse stream, but the pulse-to-pulse repetition rate of the soliton pulse stream is retained. As a result, the chirp from a single narrow-linewidth pump laser is transferred to all spectral comb teeth of the soliton at once, thus enabling parallelism in the FMCW lidar. Using this approach we generate 30 distinct channels, demonstrating both parallel distance and velocity measurements at an equivalent rate of three megapixels per second, with the potential to improve sampling rates beyond 150 megapixels per second and to increase the image refresh rate of the FMCW lidar by up to two orders of magnitude without deterioration of eye safety. This approach, when combined with photonic phase arrays(11) based on nanophotonic gratings(12), provides a technological basis for compact, massively parallel and ultrahigh-frame-rate coherent lidar systems.


  
In situ NMR metrology reveals reaction mechanisms in redox flow batteries 期刊论文
NATURE, 2020, 579 (7798) : 224-+
作者:  Ma, Jianfei;  You, Xin;  Sun, Shan;  Wang, Xiaoxiao;  Qin, Song;  Sui, Sen-Fang
收藏  |  浏览/下载:11/0  |  提交时间:2020/07/03

Large-scale energy storage is becoming increasingly critical to balancing renewable energy production and consumption(1). Organic redox flow batteries, made from inexpensive and sustainable redox-active materials, are promising storage technologies that are cheaper and less environmentally hazardous than vanadium-based batteries, but they have shorter lifetimes and lower energy density(2,3). Thus, fundamental insight at the molecular level is required to improve performance(4,5). Here we report two in situ nuclear magnetic resonance (NMR) methods of studying redox flow batteries, which are applied to two redox-active electrolytes: 2,6-dihydroxyanthraquinone (DHAQ) and 4,4 '  -((9,10-anthraquinone-2,6-diyl)dioxy) dibutyrate (DBEAQ). In the first method, we monitor the changes in the H-1 NMR shift of the liquid electrolyte as it flows out of the electrochemical cell. In the second method, we observe the changes that occur simultaneously in the positive and negative electrodes in the full electrochemical cell. Using the bulk magnetization changes (observed via the H-1 NMR shift of the water resonance) and the line broadening of the H-1 shifts of the quinone resonances as a function of the state of charge, we measure the potential differences of the two single-electron couples, identify and quantify the rate of electron transfer between the reduced and oxidized species, and determine the extent of electron delocalization of the unpaired spins over the radical anions. These NMR techniques enable electrolyte decomposition and battery self-discharge to be explored in real time, and show that DHAQ is decomposed electrochemically via a reaction that can be minimized by limiting the voltage used on charging. We foresee applications of these NMR methods in understanding a wide range of redox processes in flow and other electrochemical systems.


  
Hiding from the climate: Characterizing microrefugia for boreal forest understory species 期刊论文
GLOBAL CHANGE BIOLOGY, 2019
作者:  Greiser, Caroline;  Ehrlen, Johan;  Meineri, Eric;  Hylander, Kristoffer
收藏  |  浏览/下载:10/0  |  提交时间:2020/02/17
cold-adapted species  marginal populations  microclimate  range contraction  range edge  range shift  rear edge  thermal niche  
Soil alters seedling establishment responses to climate 期刊论文
ECOLOGY LETTERS, 2019
作者:  Ford, Kevin R.;  HilleRisLambers, Janneke
收藏  |  浏览/下载:11/0  |  提交时间:2019/11/27
Abies lasiocarpa  Cascade Range  climate change  edaphic  Mount Rainier  Pacific Northwest  plant  range shift  soil  treeline  
Northward range expansion in spring-staging barnacle geese is a response to climate change and population growth, mediated by individual experience 期刊论文
GLOBAL CHANGE BIOLOGY, 2019, 25 (11) : 3680-3693
作者:  Tombre, Ingunn M.;  Oudman, Thomas;  Shimmings, Paul;  Griffin, Larry;  Prop, Jouke
收藏  |  浏览/下载:12/0  |  提交时间:2019/11/27
age effects  dynamic strategies  explorative behaviour  food quality  population increase  range shift  spring migration  
Rapid shifts in distribution and high-latitude persistence of oceanographic habitat revealed using citizen science data from a climate change hotspot 期刊论文
GLOBAL CHANGE BIOLOGY, 2018, 24 (11) : 5440-5453
作者:  Champion, Curtis;  Hobday, Alistair J.;  Tracey, Sean R.;  Pecl, Gretta T.
收藏  |  浏览/下载:11/0  |  提交时间:2019/04/09
citizen science  climate change  global change  habitat suitability model  mixed-effects modelling  range shift  Seriola lalandi  species distribution model  species redistribution  
Dramatic loss of seagrass habitat under projected climate change in the Mediterranean Sea 期刊论文
GLOBAL CHANGE BIOLOGY, 2018, 24 (10) : 4919-4928
作者:  Chefaoui, Rosa M.;  Duarte, Carlos M.;  Serrao, Ester A.
收藏  |  浏览/下载:6/0  |  提交时间:2019/04/09
climate change  Cymodocea nodosa  ecological niche modeling  genetic diversity  Mediterranean Sea  Posidonia oceanica  range shift  seagrass decline  
Annual temperature variation as a time machine to understand the effects of long-term climate change on a poleward range shift 期刊论文
GLOBAL CHANGE BIOLOGY, 2018, 24 (8) : 3804-3819
作者:  Crickenberger, Sam;  Wethey, David S.
收藏  |  浏览/下载:8/0  |  提交时间:2019/04/09
climate change  climate variability  competency window  dispersal  interior range fragmentation  range shift  Semibalanus balanoides  
"Stick with your own kind, or hang with the locals?' Implications of shoaling strategy for tropical reef fish on a range-expansion frontline 期刊论文
GLOBAL CHANGE BIOLOGY, 2018, 24 (4) : 1663-1672
作者:  Smith, Shannen M.;  Fox, Rebecca J.;  Booth, David J.;  Donelson, Jennifer M.
收藏  |  浏览/下载:6/0  |  提交时间:2019/04/09
behaviour  biological invasion  competition  coral reef fish  range-shift  social system  vagrant fish  
Southwestern white pine (Pinus strobiformis) species distribution models project a large range shift and contraction due to regional climatic changes 期刊论文
FOREST ECOLOGY AND MANAGEMENT, 2018, 411: 176-186
作者:  Shirk, Andrew J.;  Cushman, Samuel A.;  Waring, Kristen M.;  Wehenkel, Christian A.;  Leal-Saenz, Alejandro;  Toney, Chris;  Lopez-Sanchez, Carlos A.
收藏  |  浏览/下载:10/0  |  提交时间:2019/04/09
Climate change  Multi-scale  Pinus strobiformis  Range shift  Southwestern white pine  Species distribution model