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A preliminary study on wind tunnel simulations of the explosive growth and dissipation of fine particulate matter in ambient air 期刊论文
ATMOSPHERIC RESEARCH, 2020, 235
作者:  Xu, Jingxin;  Zhu, Fahua;  Wang, Sheng;  Zhao, Xiuyong;  Zhang, Ming;  Ge, Xinlei;  Wang, Junfeng;  Tian, Wenxin;  Wang, Liwen;  Yang, Liu;  Ding, Li;  Lu, Xiaobo;  Chen, Xinxin;  Zheng, Youfei;  Guo, Zhaobing
收藏  |  浏览/下载:12/0  |  提交时间:2020/07/02
Wind tunnel  Fine particulate matter  Explosive growth  Dissipation  Relative humidity  Liquid water content  
In situ NMR metrology reveals reaction mechanisms in redox flow batteries 期刊论文
NATURE, 2020, 579 (7798) : 224-+
作者:  Ma, Jianfei;  You, Xin;  Sun, Shan;  Wang, Xiaoxiao;  Qin, Song;  Sui, Sen-Fang
收藏  |  浏览/下载:13/0  |  提交时间:2020/07/03

Large-scale energy storage is becoming increasingly critical to balancing renewable energy production and consumption(1). Organic redox flow batteries, made from inexpensive and sustainable redox-active materials, are promising storage technologies that are cheaper and less environmentally hazardous than vanadium-based batteries, but they have shorter lifetimes and lower energy density(2,3). Thus, fundamental insight at the molecular level is required to improve performance(4,5). Here we report two in situ nuclear magnetic resonance (NMR) methods of studying redox flow batteries, which are applied to two redox-active electrolytes: 2,6-dihydroxyanthraquinone (DHAQ) and 4,4 '  -((9,10-anthraquinone-2,6-diyl)dioxy) dibutyrate (DBEAQ). In the first method, we monitor the changes in the H-1 NMR shift of the liquid electrolyte as it flows out of the electrochemical cell. In the second method, we observe the changes that occur simultaneously in the positive and negative electrodes in the full electrochemical cell. Using the bulk magnetization changes (observed via the H-1 NMR shift of the water resonance) and the line broadening of the H-1 shifts of the quinone resonances as a function of the state of charge, we measure the potential differences of the two single-electron couples, identify and quantify the rate of electron transfer between the reduced and oxidized species, and determine the extent of electron delocalization of the unpaired spins over the radical anions. These NMR techniques enable electrolyte decomposition and battery self-discharge to be explored in real time, and show that DHAQ is decomposed electrochemically via a reaction that can be minimized by limiting the voltage used on charging. We foresee applications of these NMR methods in understanding a wide range of redox processes in flow and other electrochemical systems.


  
A droplet-based electricity generator with high instantaneous power density 期刊论文
NATURE, 2020, 578 (7795) : 392-+
作者:  Dabney, Will;  Kurth-Nelson, Zeb;  Uchida, Naoshige;  Starkweather, Clara Kwon;  Hassabis, Demis;  Munos, Remi;  Botvinick, Matthew
收藏  |  浏览/下载:175/0  |  提交时间:2020/07/03

Extensive efforts have been made to harvest energy from water in the form of raindrops(1-6), river and ocean waves(7,8), tides(9) and others(10-17). However, achieving a high density of electrical power generation is challenging. Traditional hydraulic power generation mainly uses electromagnetic generators that are heavy, bulky, and become inefficient with low water supply. An alternative, the water-droplet/solid-based triboelectric nanogenerator, has so far generated peak power densities of less than one watt per square metre, owing to the limitations imposed by interfacial effects-as seen in characterizations of the charge generation and transfer that occur at solid-liquid(1-4) or liquid-liquid(5,18) interfaces. Here we develop a device to harvest energy from impinging water droplets by using an architecture that comprises a polytetrafluoroethylene film on an indium tin oxide substrate plus an aluminium electrode. We show that spreading of an impinged water droplet on the device bridges the originally disconnected components into a closed-loop electrical system, transforming the conventional interfacial effect into a bulk effect, and so enhancing the instantaneous power density by several orders of magnitude over equivalent devices that are limited by interfacial effects.


A device involving a polytetrafluoroethylene film, an indium tin oxide substrate and an aluminium electrode allows improved electricity generation from water droplets, which bridge the previously disconnected circuit components.


  
The Vertical Structure of Liquid Water Content in Shallow Clouds as Retrieved From Dual-Wavelength Radar Observations 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2019, 124 (24) : 14184-14197
作者:  Zhu, Zeen;  Lamer, Katia;  Kollias, Pavlos;  Clothiaux, Eugene E.
收藏  |  浏览/下载:8/0  |  提交时间:2020/02/17
boundary layer cloud observation  dual-wavelength ratio technique  liquid water content retrieval  liquid water content vertical distribution  cloud adiabaticity  dynamic and microphysical process  
Aircraft Icing: In-Cloud Measurements and Sensitivity to Physical Parameterizations 期刊论文
GEOPHYSICAL RESEARCH LETTERS, 2019
作者:  Merino, A.;  Garcia-Ortega, E.;  Fernandez-Gonzalez, S.;  Diaz-Fernandez, J.;  Quitian-Hernandez, L.;  Martin, M. L.;  Lopez, L.;  Marcos, J. L.;  Valero, F.;  Sanchez, J. L.
收藏  |  浏览/下载:10/0  |  提交时间:2019/11/27
Aircraft icing  Cloud microphysics  Liquid water content  WRF  
Toward understanding the process-level impacts of aerosols on microphysical properties of shallow cumulus cloud using aircraft observations 期刊论文
ATMOSPHERIC RESEARCH, 2019, 221: 27-33
作者:  Yang, Yang;  Zhao, Chuanfeng;  Dong, Xiaobo;  Fan, Genchang;  Zhou, Yuquan;  Wang, Yang;  Zhao, Lijun;  Lv, Feng;  Yan, Fei
收藏  |  浏览/下载:7/0  |  提交时间:2019/11/26
Shallow cumulus  Aerosol  Vertical velocity  Cloud droplet effective radius  Liquid water content  Aircraft observation  
Retrieval of Snow Water Equivalent, Liquid Water Content, and Snow Height of Dry and Wet Snow by Combining GPS Signal Attenuation and Time Delay 期刊论文
WATER RESOURCES RESEARCH, 2019, 55 (5) : 4465-4487
作者:  Koch, Franziska;  Henkel, Patrick;  Appel, Florian;  Schmid, Lino;  Bach, Heike;  Lamm, Markus;  Prasch, Monika;  Schweizer, Juerg;  Mauser, Wolfram
收藏  |  浏览/下载:9/0  |  提交时间:2019/11/26
snow water equivalent  liquid water content  snow cover  SnowSense  GNSS signals  Global Positioning System  
High-Speed Quantification of Pore-Scale Multiphase Flow of Water and Supercritical CO2 in 2-D Heterogeneous Porous Micromodels: Flow Regimes and Interface Dynamics 期刊论文
WATER RESOURCES RESEARCH, 2019, 55 (5) : 3758-3779
作者:  Li, Yaofa;  Blois, Gianluca;  Kazemifar, Farzan;  Christensen, Kenneth T.
收藏  |  浏览/下载:8/0  |  提交时间:2019/11/26
pore-scale flow  water and liquid CO2  micro-PIV  geologic CO2 sequestration  
Aerosol Indirect Effects in Marine Stratocumulus: The Importance of Explicitly Predicting Cloud Droplet Activation 期刊论文
GEOPHYSICAL RESEARCH LETTERS, 2019, 46 (6) : 3473-3481
作者:  Bulatovic, I.;  Ekman, A. M. L.;  Savre, J.;  Riipinen, I.;  Leck, C.
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/26
aerosol indirect effect  cloud droplet number concentration  liquid water path  large-eddy simulation  
Satellite-Based Detection of Daytime Supercooled Liquid-Topped Mixed-Phase Clouds Over the Southern Ocean Using the Advanced Himawari Imager 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2019, 124 (5) : 2677-2701
作者:  Noh, Yoo-Jeong;  Miller, Steven D.;  Heidinger, Andrew K.;  Mace, Gerald G.;  Protat, Alain;  Alexander, Simon P.
收藏  |  浏览/下载:9/0  |  提交时间:2019/11/26
cloud phase  satellite algorithm  supercooled liquid water