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DOI10.1029/2018WR024635
High-Speed Quantification of Pore-Scale Multiphase Flow of Water and Supercritical CO2 in 2-D Heterogeneous Porous Micromodels: Flow Regimes and Interface Dynamics
Li, Yaofa1,2; Blois, Gianluca1; Kazemifar, Farzan3; Christensen, Kenneth T.1,2,4
2019-05-01
发表期刊WATER RESOURCES RESEARCH
ISSN0043-1397
EISSN1944-7973
出版年2019
卷号55期号:5页码:3758-3779
文章类型Article
语种英语
国家USA; Japan
英文摘要

The pore-scale flow of CO2 and water in 2-D heterogeneous porous micromodels over a Ca range of nearly three orders of magnitude was explored experimentally. The porous geometry is a close reprint of real sandstone, and the experiments were performed under reservoir-relevant conditions (i.e., 8 MPa and 21 degrees C), thus ensuring relevance to practical CO2 operations. High-speed fluorescent microscopy and image processing were employed to achieve temporally and spatially resolved data, providing a unique view of the dynamics underlying this multiphase flow scenario. Under conditions relevant to CO2 sequestration, final CO2 saturation was found to decrease and increase logarithmically with Ca within the capillary and viscous-fingering regimes, respectively, with a minimum occurring during regime crossover. Specific interfacial length generally scales linearly with CO2 saturation, with higher slopes noted at high Ca due to stronger viscous and inertial forces, as supported by direct pore-scale observations. Statistical analysis of the interfacial movements revealed that pore-scale events are controlled by their intrinsic dynamics at low Ca, but overrun by the bulk flow at high Ca. During postfront flow, while permeability is typically correlated with total CO2 saturation in the porous domain (regardless of its mobility), the saturation of active CO2 pathways in the current study correlated very well with permeability. This alternate approach to characterize relative permeability could serve to mitigate hysteresis in relative permeability curves. Taken together, these results provide unique insights that address inconsistent observations in the literature and previously unanswered questions about the underlying flow dynamics of this important multiphase flow scenario.


英文关键词pore-scale flow water and liquid CO2 micro-PIV geologic CO2 sequestration
领域资源环境
收录类别SCI-E
WOS记录号WOS:000474848500009
WOS关键词IMMISCIBLE 2-PHASE FLOW ; CAPILLARY-PRESSURE ; FLUID DISPLACEMENT ; CARBON-DIOXIDE ; VELOCITY-FIELD ; MEDIA ; SEQUESTRATION ; SIMULATIONS ; SATURATION ; CROSSOVER
WOS类目Environmental Sciences ; Limnology ; Water Resources
WOS研究方向Environmental Sciences & Ecology ; Marine & Freshwater Biology ; Water Resources
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/183117
专题资源环境科学
作者单位1.Univ Notre Dame, Dept Aerosp & Mech Engn, Notre Dame, IN 46556 USA;
2.Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Fukuoka, Fukuoka, Japan;
3.Calif State Univ Sacramento, Dept Mech Engn, Sacramento, CA 95819 USA;
4.Univ Notre Dame, Dept Civil & Environm Engn & Earth Sci, Notre Dame, IN 46556 USA
推荐引用方式
GB/T 7714
Li, Yaofa,Blois, Gianluca,Kazemifar, Farzan,et al. High-Speed Quantification of Pore-Scale Multiphase Flow of Water and Supercritical CO2 in 2-D Heterogeneous Porous Micromodels: Flow Regimes and Interface Dynamics[J]. WATER RESOURCES RESEARCH,2019,55(5):3758-3779.
APA Li, Yaofa,Blois, Gianluca,Kazemifar, Farzan,&Christensen, Kenneth T..(2019).High-Speed Quantification of Pore-Scale Multiphase Flow of Water and Supercritical CO2 in 2-D Heterogeneous Porous Micromodels: Flow Regimes and Interface Dynamics.WATER RESOURCES RESEARCH,55(5),3758-3779.
MLA Li, Yaofa,et al."High-Speed Quantification of Pore-Scale Multiphase Flow of Water and Supercritical CO2 in 2-D Heterogeneous Porous Micromodels: Flow Regimes and Interface Dynamics".WATER RESOURCES RESEARCH 55.5(2019):3758-3779.
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