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Global radiation in a rare biosphere soil diatom 期刊论文
NATURE COMMUNICATIONS, 2020, 11 (1)
作者:  Pinseel, Eveline;  Janssens, Steven B.;  Verleyen, Elie;  Vanormelingen, Pieter;  Kohler, Tyler J.;  Biersma, Elisabeth M.;  Sabbe, Koen;  Van de Vijver, Bart;  Vyverman, Wim
收藏  |  浏览/下载:7/0  |  提交时间:2020/05/20
Field-resolved infrared spectroscopy of biological systems 期刊论文
NATURE, 2020, 577 (7788) : 52-+
作者:  Pupeza, Ioachim;  Huber, Marinus;  Trubetskov, Michael;  Schweinberger, Wolfgang;  Hussain, Syed A.;  Hofer, Christina;  Fritsch, Kilian;  Poetzlberger, Markus;  Vamos, Lenard;  Fill, Ernst;  Amotchkina, Tatiana;  Kepesidis, Kosmas V.;  Apolonski, Alexander;  Karpowicz, Nicholas;  Pervak, Vladimir;  Pronin, Oleg;  Fleischmann, Frank;  Azzeer, Abdallah;  Zigman, Mihaela;  Krausz, Ferenc
收藏  |  浏览/下载:14/0  |  提交时间:2020/07/03

The proper functioning of living systems and physiological phenotypes depends on molecular composition. Yet simultaneous quantitative detection of a wide variety of molecules remains a challenge(1-8). Here we show how broadband optical coherence opens up opportunities for fingerprinting complex molecular ensembles in their natural environment. Vibrationally excited molecules emit a coherent electric field following few-cycle infrared laser excitation(9-12), and this field is specific to the sample'  s molecular composition. Employing electro-optic sampling(10,12-15), we directly measure this global molecular fingerprint down to field strengths 10(7) times weaker than that of the excitation. This enables transillumination of intact living systems with thicknesses of the order of 0.1 millimetres, permitting broadband infrared spectroscopic probing of human cells and plant leaves. In a proof-of-concept analysis of human blood serum, temporal isolation of the infrared electric-field fingerprint from its excitation along with its sampling with attosecond timing precision results in detection sensitivity of submicrograms per millilitre of blood serum and a detectable dynamic range of molecular concentration exceeding 10(5). This technique promises improved molecular sensitivity and molecular coverage for probing complex, real-world biological and medical settings.


  
Extreme weather events recorded by daily to hourly resolution biogeochemical proxies of marine giant clam shells 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2020, 117 (13) : 7038-7043
作者:  Yan, Hong;  Liu, Chengcheng;  An, Zhisheng;  Yang, Wei;  Yang, Yuanjian;  Huang, Ping;  Qiu, Shican;  Zhou, Pengchao;  Zhao, Nanyu;  Fei, Haobai;  Ma, Xiaolin;  Shi, Ge;  Dodson, John;  Hao, Jialong;  Yu, Kefu;  Wei, Gangjian;  Yang, Yanan;  Jin, Zhangdong;  Zhou, Weijian
收藏  |  浏览/下载:14/0  |  提交时间:2020/05/13
Tridacna shell  daily growth bands  ultra-high resolution  biogeochemical proxies  weather-timescale extreme events  
Global airborne sampling reveals a previously unobserved dimethyl sulfide oxidation mechanism in the marine atmosphere 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2020, 117 (9) : 4505-4510
作者:  Veres, Patrick R.;  Neuman, J. Andrew;  Bertram, Timothy H.;  Assaf, Emmanuel;  Wolfe, Glenn M.;  Williamson, Christina J.;  Weinzierl, Bernadett;  Tilmes, Simone;  Thompson, Chelsea R.;  Thames, Alexander B.;  Schroder, Jason C.;  Saiz-Lopez, Alfonso;  Rollins, Andrew W.;  Roberts, James M.;  Price, Derek;  Peischl, Jeff;  Nault, Benjamin A.;  Moller, Kristian H.;  Miller, David O.;  Meinardi, Simone;  Li, Qinyi;  Lamarque, Jean-Francois;  Kupc, Agnieszka;  Kjaergaard, Henrik G.;  Kinnison, Douglas;  Jimenez, Jose L.;  Jernigan, Christopher M.;  Hornbrook, Rebecca S.;  Hills, Alan;  Dollner, Maximilian;  Day, Douglas A.;  Cuevas, Carlos A.;  Campuzano-Jost, Pedro;  Burkholder, James;  Bui, T. Paul;  Brune, William H.;  Brown, Steven S.;  Brock, Charles A.;  Bourgeois, Ilann;  Blake, Donald R.;  Apel, Eric C.;  Ryerson, Thomas B.
收藏  |  浏览/下载:23/0  |  提交时间:2020/05/13
dimethyl sulfide  marine sulfur  autoxidation  marine aerosols  aerosol sulfate  
Shale gas development has limited effects on stream biology and geochemistry in a gradient-based, multiparameter study in Pennsylvania 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2020, 117 (7) : 3670-3677
作者:  Mumford, Adam C.;  Maloney, Kelly O.;  Akob, Denise M.;  Nettemann, Sarah;  Proctor, Arianne;  Ditty, Jason;  Ulsamer, Luke;  Lookenbill, Josh;  Cozzarelli, Isabelle M.
收藏  |  浏览/下载:7/0  |  提交时间:2020/05/13
Marcellus Shale  hydraulic fracturing  water quality  microbiology  macroinvertebrates  
Soil structure is an important omission in Earth System Models 期刊论文
NATURE COMMUNICATIONS, 2020, 11 (1)
作者:  Fatichi, Simone;  Or, Dani;  Walko, Robert;  Vereecken, Harry;  Young, Michael H.;  Ghezzehei, Teamrat A.;  Hengl, Tomislav;  Kollet, Stefan;  Agam, Nurit;  Avissar, Roni
收藏  |  浏览/下载:5/0  |  提交时间:2020/05/13
Windborne long-distance migration of malaria mosquitoes in the Sahel 期刊论文
NATURE, 2019, 574 (7778) : 404-+
作者:  Huestis, Diana L.;  Dao, Adama;  Diallo, Moussa;  Sanogo, Zana L.;  Samake, Djibril;  Yaro, Alpha S.;  Ousman, Yossi;  Linton, Yvonne-Marie;  Krishna, Asha;  Veru, Laura;  Krajacich, Benjamin J.;  Faiman, Roy;  Florio, Jenna;  Chapman, Jason W.;  Reynolds, Don R.;  Weetman, David;  Mitchell, Reed;  Donnelly, Martin J.;  Talamas, Elijah;  Chamorro, Lourdes;  Strobach, Ehud;  Lehmann, Tovi
收藏  |  浏览/下载:5/0  |  提交时间:2019/11/27
Multiplatform evaluation of global trends in wind speed and wave height 期刊论文
SCIENCE, 2019, 364 (6440) : 548-+
作者:  Young, Ian R.;  Ribal, Agustinus
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/27
Stratification of reactivity determines nitrate removal in groundwater 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2019, 116 (7) : 2494-2499
作者:  Kolbe, Tamara;  de Dreuzy, Jean-Raynald;  Abbott, Benjamin W.;  Aquilina, Luc;  Babey, Tristan;  Green, Christopher T.;  Fleckenstein, Jan H.;  Labasque, Thierry;  Laverman, Anniet M.;  Marcais, Jean;  Peiffer, Stefan;  Thomas, Zahra;  Pinay, Gilles
收藏  |  浏览/下载:8/0  |  提交时间:2019/11/27
groundwater  denitrification  reactivity pattern  transit times  reaction times  
Temporal variability largely explains top-down/bottom-up difference in methane emission estimates from a natural gas production region 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2018, 115 (46) : 11712-11717
作者:  Vaughn, Timothy L.;  Bell, Clay S.;  Pickering, Cody K.;  Schwietzke, Stefan;  Heath, Garvin A.;  Petron, Gabrielle;  Zimmerle, Daniel J.;  Schnell, Russell C.;  Nummedal, Dag
收藏  |  浏览/下载:10/0  |  提交时间:2019/11/27
natural gas  methane emissions  top-down  bottom-up  spatiotemporal inventory model