Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-19-2497-2019 |
The SPARC water vapour assessment II: profile-to-profile and climatological comparisons of stratospheric delta D(H2O) observations from satellite | |
Hogberg, Charlotta1; Lossow, Stefan2; Khosrawi, Farahnaz2; Bauer, Ralf3; Walker, Kaley A.3; Eriksson, Patrick4; Murtagh, Donal P.4; Stiller, Gabriele P.2; Steinwagner, Joerg5; Zhang, Qiong1 | |
2019-02-27 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2019 |
卷号 | 19期号:4页码:2497-2526 |
文章类型 | Article |
语种 | 英语 |
国家 | Sweden; Germany; Canada |
英文摘要 | Within the framework of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapour assessment (WAVAS-II), we evaluated five data sets of delta D(H2O) obtained from observations by Odin/SMR (Sub-Millimetre Radiometer), Envisat/MIPAS (Environmental Satellite/Michelson Interferometer for Passive Atmospheric Sounding), and SCISAT/ACE-FTS (Science Satellite/Atmospheric Chemistry Experiment - Fourier Transform Spectrometer) using profile-to-profile and climatological comparisons. These comparisons aimed to provide a comprehensive overview of typical uncertainties in the observational database that could be considered in the future in observational and modelling studies. Our primary focus is on stratospheric altitudes, but results for the upper troposphere and lower mesosphere are also shown. There are clear quantitative differences in the measurements of the isotopic ratio, mainly with regard to comparisons between the SMR data set and both the MIPAS and ACE-FTS data sets. In the lower stratosphere, the SMR data set shows a higher depletion in delta D than the MIPAS and ACE-FTS data sets. The differences maximise close to 50 hPa and exceed 200 parts per thousand. With increasing altitude, the biases decrease. Above 4 hPa, the SMR data set shows a lower delta D depletion than the MIPAS data sets, occasionally exceeding 100 parts per thousand. Overall, the delta D biases of the SMR data set are driven by HDO biases in the lower stratosphere and by H2O biases in the upper stratosphere and lower mesosphere. In between, in the middle stratosphere, the biases in delta D are the result of deviations in both HDO and H2O. These biases are attributed to issues with the calibration, in particular in terms of the sideband filtering, and uncertainties in spectroscopic parameters. The MIPAS and ACE-FTS data sets agree rather well between about 100 and 10 hPa. The MIPAS data sets show less depletion below approximately 15 hPa (up to about 30 parts per thousand), due to differences in both HDO and H2O. Higher up this behaviour is reversed, and towards the upper stratosphere the biases increase. This is driven by increasing biases in H2O, and on occasion the differences in delta D exceed 80 parts per thousand. Below 100 hPa, the differences between the MIPAS and ACE-FTS data sets are even larger. In the climatological comparisons, the MIPAS data sets continue to show less depletion in delta D than the ACE-FTS data sets below 15 hPa during all seasons, with some variations in magnitude. The differences between the MIPAS and ACE-FTS data have multiple causes, such as differences in the temporal and spatial sampling (except for the profile-to-profile comparisons), cloud influence, vertical resolution, and the microwindows and spectroscopic database chosen. Differences between data sets from the same instrument are typically small in the stratosphere. Overall, if the data sets are considered together, the differences in delta D among them in key areas of scientific interest (e.g. tropical and polar lower stratosphere, lower mesosphere, and upper troposphere) are too large to draw robust conclusions on atmospheric processes affecting the water vapour budget and distribution, e.g. the relative importance of different mechanisms transporting water vapour into the stratosphere. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000459867200003 |
WOS关键词 | ISOTOPIC COMPOSITION ; METHANE OXIDATION ; HDO MEASUREMENTS ; ODIN SATELLITE ; OZONE ; DEHYDRATION ; VALIDATION ; EVOLUTION ; DATABASE ; MIPAS |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/30450 |
专题 | 地球科学 |
作者单位 | 1.Stockholm Univ, Dept Phys Geog, Svante Arrhenius Vag 8, S-10691 Stockholm, Sweden; 2.Karlsruhe Inst Technol, Inst Meteorol & Climate Res, Hermann von Helmholtz Pl 1, D-76344 Leopoldshafen, Germany; 3.Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada; 4.Chalmers Univ Technol, Dept Earth & Space Sci, Horsalsvagen 11, S-41296 Gothenburg, Sweden; 5.Max Planck Inst Extraterr Phys, Giessenbachstr 1, D-85748 Garching, Germany |
推荐引用方式 GB/T 7714 | Hogberg, Charlotta,Lossow, Stefan,Khosrawi, Farahnaz,et al. The SPARC water vapour assessment II: profile-to-profile and climatological comparisons of stratospheric delta D(H2O) observations from satellite[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(4):2497-2526. |
APA | Hogberg, Charlotta.,Lossow, Stefan.,Khosrawi, Farahnaz.,Bauer, Ralf.,Walker, Kaley A..,...&Zhang, Qiong.(2019).The SPARC water vapour assessment II: profile-to-profile and climatological comparisons of stratospheric delta D(H2O) observations from satellite.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(4),2497-2526. |
MLA | Hogberg, Charlotta,et al."The SPARC water vapour assessment II: profile-to-profile and climatological comparisons of stratospheric delta D(H2O) observations from satellite".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.4(2019):2497-2526. |
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