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DOI10.5194/acp-17-4229-2017
Evaluation of the absorption angstrom ngstrom exponents for traffic and wood burning in the Aethalometer-based source apportionment using radiocarbon measurements of ambient aerosol
Zotter, Peter1,8; Herich, Hanna2,9; Gysel, Martin1; El-Haddad, Imad1; Zhang, Yanlin1,3,4,5,10; Mocnik, Grisa6,7; Huglin, Christoph2; Baltensperger, Urs1; Szidat, Sonke3,4; Prevot, Andres. H.1
2017-03-29
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2017
卷号17期号:6
文章类型Article
语种英语
国家Switzerland; Slovenia; Peoples R China
英文摘要

Equivalent black carbon (EBC) measured by a multi-wavelength Aethalometer can be apportioned to traffic and wood burning. The method is based on the differences in the dependence of aerosol absorption on the wavelength of light used to investigate the sample, parameterized by the source-specific absorption angstrom ngstrom exponent (alpha). While the spectral dependence (defined as alpha values) of the traffic-related EBC light absorption is low, wood smoke particles feature enhanced light absorption in the blue and near ultraviolet. Source apportionment results using this methodology are hence strongly dependent on the alpha values assumed for both types of emissions: traffic alpha TR, and wood burning alpha WB. Most studies use a single alpha TR and alpha WB pair in the Aethalometer model, derived from previous work. However, an accurate determination of the source specific alpha values is currently lacking and in some recent publications the applicability of the Aethalometer model was questioned.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000397939000003
WOS关键词FINE-PARTICLE EMISSIONS ; OXYGENATED ORGANIC AEROSOLS ; ATTENUATION CROSS-SECTION ; BLACK CARBON AEROSOL ; LIGHT-ABSORPTION ; CHEMICAL-CHARACTERIZATION ; FIREPLACE COMBUSTION ; BROWN CARBON ; PARTICULATE MATTER ; OPTICAL-PROPERTIES
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/24935
专题地球科学
作者单位1.PSI, Lab Atmospher Chem, CH-5232 Villigen, Switzerland;
2.Swiss Fed Labs Mat Sci & Technol Empa, Lab Air Pollut & Environm Technol, Uberlandstr 129, CH-8600 Dubendorf, Switzerland;
3.Univ Bern, Dept Chem & Biochem, Bern, Switzerland;
4.Univ Bern, Oeschger Ctr Climate Change Res, Bern, Switzerland;
5.PSI, Lab Radiochem & Environm Chem, CH-5232 Villigen, Switzerland;
6.Aerosol Doo, Res & Dev Dept, Ljubljana, Slovenia;
7.Jozef Stefan Inst, Dept Condensed Matter Phys, Ljubljana, Slovenia;
8.Lucerne Univ Appl Sci & Arts, Sch Engn & Architecture, Bioenergy Res, Technikumstr 21, CH-6048 Horw, Switzerland;
9.Kanton St Gallen, Amt Umwelt & Energie, CH-9001 St Gallen, Switzerland;
10.Nanjing Univ Informat Sci & Technol, Yale NUIST Ctr Atmospher Environm, Nanjing 210044, Jiangsu, Peoples R China
推荐引用方式
GB/T 7714
Zotter, Peter,Herich, Hanna,Gysel, Martin,et al. Evaluation of the absorption angstrom ngstrom exponents for traffic and wood burning in the Aethalometer-based source apportionment using radiocarbon measurements of ambient aerosol[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(6).
APA Zotter, Peter.,Herich, Hanna.,Gysel, Martin.,El-Haddad, Imad.,Zhang, Yanlin.,...&Prevot, Andres. H..(2017).Evaluation of the absorption angstrom ngstrom exponents for traffic and wood burning in the Aethalometer-based source apportionment using radiocarbon measurements of ambient aerosol.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(6).
MLA Zotter, Peter,et al."Evaluation of the absorption angstrom ngstrom exponents for traffic and wood burning in the Aethalometer-based source apportionment using radiocarbon measurements of ambient aerosol".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.6(2017).
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