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DOI | 10.1029/2019JD031701 |
Optical Modeling of Black Carbon With Different Coating Materials: The Effect of Coating Configurations | |
Luo, Jie1; Zhang, Qixing1; Luo, Jianfei2; Liu, Jia1; Huo, Yinuo1; Zhang, Yongming1 | |
2019-12-16 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
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ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2019 |
卷号 | 124期号:23页码:13230-13253 |
文章类型 | Article |
语种 | 英语 |
国家 | Peoples R China |
英文摘要 | In this work, an assembly of coating structures is generated for coated black carbon (BC) based on two different coating methods with limited tunable parameters. By defining typical parameters, the proposed coating structures show great agreement with the detailed morphologies of coated BC particles in the atmosphere. Our models can accurately reproduce the measured linear backscattering depolarization ratio (LDR). We noticed that BC with spherical coatings (Configuration E) has difficulty estimating large LDRs, while the ability to reproduce a large LDR is improved by making the coating structure slightly nonspherical (Configuration C). Our models also show a better performance in reproducing the laboratory-measured absorption enhancement (E-abs), mass absorption/scattering cross sections, and absorption Angstrom exponent than the simplified models. In addition, sizable uncertainties in the optical properties of coated BC with different coating configurations are found. The uncertainties in the LDR, E-abs, mass absorption cross section, and absorption Angstrom exponent caused by the coating configurations can reach approximately 220%, 35%, 90%, and 20%, respectively. Therefore, complex coating structures should be carefully considered. In this work, various coating structures are represented by limited tunable parameters, which is beneficial to the parameterization of the optical properties of BC with a complex coating structure. Our models can also provide tools for exploring the agreement between calculations and measurements. |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000505626200049 |
WOS关键词 | DISCRETE-DIPOLE APPROXIMATION ; LIGHT-ABSORPTION ENHANCEMENT ; MIXING STATE ; BROWN CARBON ; RADIATIVE PROPERTIES ; SOOT PARTICLES ; AMBIENT BLACK ; SCATTERING PROPERTIES ; ABSORBING CARBON ; RAMAN LIDAR |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/225931 |
专题 | 环境与发展全球科技态势 |
作者单位 | 1.Univ Sci & Technol China, State Key Lab Fire Sci, Hefei, Peoples R China; 2.NARI Grp Corp, State Grid Elect Power Res Inst, Nanjing, Peoples R China |
推荐引用方式 GB/T 7714 | Luo, Jie,Zhang, Qixing,Luo, Jianfei,et al. Optical Modeling of Black Carbon With Different Coating Materials: The Effect of Coating Configurations[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2019,124(23):13230-13253. |
APA | Luo, Jie,Zhang, Qixing,Luo, Jianfei,Liu, Jia,Huo, Yinuo,&Zhang, Yongming.(2019).Optical Modeling of Black Carbon With Different Coating Materials: The Effect of Coating Configurations.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,124(23),13230-13253. |
MLA | Luo, Jie,et al."Optical Modeling of Black Carbon With Different Coating Materials: The Effect of Coating Configurations".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 124.23(2019):13230-13253. |
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