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DOI | 10.1038/s41467-019-12431-y |
Coherent multidimensional spectroscopy of dilute gas-phase nanosystems | |
Bruder, Lukas1; Bangert, Ulrich1; Binz, Marcel1; Uhl, Daniel1; Vexiau, Romain2; Bouloufa-Maafa, Nadia2; Dulieu, Olivier2; Stienkemeier, Frank1,3 | |
2019-09-27 | |
发表期刊 | NATURE COMMUNICATIONS |
ISSN | 2041-1723 |
出版年 | 2018 |
卷号 | 9 |
文章类型 | Article |
语种 | 英语 |
国家 | Germany; France |
英文摘要 | Two-dimensional electronic spectroscopy (2DES) is one of the most powerful spectroscopic techniques with unique sensitivity to couplings, coherence properties and real-time dynamics of a quantum system. While successfully applied to a variety of condensed phase samples, high precision experiments on isolated systems in the gas phase have been so far precluded by insufficient sensitivity. However, such experiments are essential for a precise understanding of fundamental mechanisms and to avoid misinterpretations. Here, we solve this issue by extending 2DES to isolated nanosystems in the gas phase prepared by helium nanodroplet isolation in a molecular beam-type experiment. This approach uniquely provides high flexibility in synthesizing tailored, quantum state-selected model systems of single and many-body character. In a model study of weakly-bound Rb-2 and Rb-3 molecules we demonstrate the method's unique capacity to elucidate interactions and dynamics in tailored quantum systems, thereby also bridging the gap to experiments in ultracold quantum science. |
领域 | 资源环境 |
收录类别 | SCI-E |
WOS记录号 | WOS:000450273500010 |
WOS关键词 | 2-DIMENSIONAL ELECTRONIC SPECTROSCOPY ; ULTRACOLD RB-2 MOLECULES ; LIQUID-HELIUM ; DYNAMICS ; ATOMS ; SPECTRA ; STATES |
WOS类目 | Multidisciplinary Sciences |
WOS研究方向 | Science & Technology - Other Topics |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/204565 |
专题 | 资源环境科学 |
作者单位 | 1.Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany; 2.Univ Paris Saclay, ENS Cachan, Univ Paris Sud, Lab Aime Cotton,CNRS, F-91405 Orsay, France; 3.Univ Freiburg, Freiburg Inst Adv Studies FRIAS, Albertstr 19, D-79194 Freiburg, Germany |
推荐引用方式 GB/T 7714 | Bruder, Lukas,Bangert, Ulrich,Binz, Marcel,et al. Coherent multidimensional spectroscopy of dilute gas-phase nanosystems[J]. NATURE COMMUNICATIONS,2019,9. |
APA | Bruder, Lukas.,Bangert, Ulrich.,Binz, Marcel.,Uhl, Daniel.,Vexiau, Romain.,...&Stienkemeier, Frank.(2019).Coherent multidimensional spectroscopy of dilute gas-phase nanosystems.NATURE COMMUNICATIONS,9. |
MLA | Bruder, Lukas,et al."Coherent multidimensional spectroscopy of dilute gas-phase nanosystems".NATURE COMMUNICATIONS 9(2019). |
条目包含的文件 | 条目无相关文件。 |
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