GSTDTAP

浏览/检索结果: 共16条,第1-10条 帮助

已选(0)清除 条数/页:   排序方式:
Detection of metastable electronic states by Penning trap mass spectrometry 期刊论文
NATURE, 2020, 581 (7806) : 42-+
作者:  Rauch, Jennifer N.;  Luna, Gabriel;  Guzman, Elmer;  Audouard, Morgane;  Challis, Collin;  Sibih, Youssef E.;  Leshuk, Carolina;  Hernandez, Israel;  Wegmann, Susanne;  Hyman, Bradley T.;  Gradinaru, Viviana;  Kampmann, Martin;  Kosik, Kenneth S.
收藏  |  浏览/下载:9/0  |  提交时间:2020/07/03

State-of-the-art optical clocks(1) achieve precisions of 10(-18) or better using ensembles of atoms in optical lattices(2,3) or individual ions in radio-frequency traps(4,5). Promising candidates for use in atomic clocks are highly charged ions(6) (HCIs) and nuclear transitions(7), which are largely insensitive to external perturbations and reach wavelengths beyond the optical range(8) that are accessible to frequency combs(9). However, insufficiently accurate atomic structure calculations hinder the identification of suitable transitions in HCIs. Here we report the observation of a long-lived metastable electronic state in an HCI by measuring the mass difference between the ground and excited states in rhenium, providing a non-destructive, direct determination of an electronic excitation energy. The result is in agreement with advanced calculations. We use the high-precision Penning trap mass spectrometer PENTATRAP to measure the cyclotron frequency ratio of the ground state to the metastable state of the ion with a precision of 10(-11)-an improvement by a factor of ten compared with previous measurements(10,11). With a lifetime of about 130 days, the potential soft-X-ray frequency reference at 4.96 x 10(16) hertz (corresponding to a transition energy of 202 electronvolts) has a linewidth of only 5 x 10(-8) hertz and one of the highest electronic quality factors (10(24)) measured experimentally so far. The low uncertainty of our method will enable searches for further soft-X-ray clock transitions(8,12) in HCIs, which are required for precision studies of fundamental physics(6).


Penning trap mass spectrometry is used to measure the electronic transition energy from a long-lived metastable state to the ground state in highly charged rhenium ions with a precision of 10(-11).


  
Laser spectroscopy of pionic helium atoms 期刊论文
NATURE, 2020, 581 (7806) : 37-+
作者:  Shang, Jian;  Ye, Gang;  Shi, Ke;  Wan, Yushun;  Luo, Chuming;  Aihara, Hideki;  Geng, Qibin;  Auerbach, Ashley;  Li, Fang
收藏  |  浏览/下载:20/0  |  提交时间:2020/07/03

Charged pions(1) are the lightest and longest-lived mesons. Mesonic atoms are formed when an orbital electron in an atom is replaced by a negatively charged meson. Laser spectroscopy of these atoms should permit the mass and other properties of the meson to be determined with high precision and could place upper limits on exotic forces involving mesons (as has been done in other experiments on antiprotons(2-9)). Determining the mass of the pi(-) meson in particular could help to place direct experimental constraints on the mass of the muon antineutrino(10-13). However, laser excitations of mesonic atoms have not been previously achieved because of the small number of atoms that can be synthesized and their typically short (less than one picosecond) lifetimes against absorption of the mesons into the nuclei(1). Metastable pionic helium (pi He-4(+)) is a hypothetical(14-16) three-body atom composed of a helium-4 nucleus, an electron and a pi(-) occupying a Rydberg state of large principal (n approximate to 16) and orbital angular momentum (l approximate to n - 1) quantum numbers. The pi He-4(+) atom is predicted to have an anomalously long nanosecond-scale lifetime, which could allow laser spectroscopy to be carried out(17). Its atomic structure is unique owing to the absence of hyperfine interactions(18,19) between the spin-0 pi(-) and the He-4 nucleus. Here we synthesize pi He-4(+) in a superfluid-helium target and excite the transition (n, l) = (17, 16) -> (17, 15) of the pi(-)-occupied pi He-4(+) orbital at a near-infrared resonance frequency of 183,760 gigahertz. The laser initiates electromagnetic cascade processes that end with the nucleus absorbing the pi(-) and undergoing fission(20,21). The detection of emerging neutron, proton and deuteron fragments signals the laser-induced resonance in the atom, thereby confirming the presence of pi He-4(+). This work enables the use of the experimental techniques of quantum optics to study a meson.


Long-lived pionic helium atoms (composed of a helium-4 nucleus, an electron and a negatively charged pion) are synthesized in a superfluid-helium target, as confirmed by laser spectroscopy involving the pion-occupied orbitals.


  
The mutational landscape of normal human endometrial epithelium 期刊论文
NATURE, 2020, 580 (7805) : 640-+
作者:  Rogelj, Joeri;  Forster, Piers M.;  Kriegler, Elmar;  Smith, Christopher J.;  Seferian, Roland
收藏  |  浏览/下载:12/0  |  提交时间:2020/07/03

All normal somatic cells are thought to acquire mutations, but understanding of the rates, patterns, causes and consequences of somatic mutations in normal cells is limited. The uterine endometrium adopts multiple physiological states over a lifetime and is lined by a gland-forming epithelium(1,2). Here, using whole-genome sequencing, we show that normal human endometrial glands are clonal cell populations with total mutation burdens that increase at about 29 base substitutions per year and that are many-fold lower than those of endometrial cancers. Normal endometrial glands frequently carry '  driver'  mutations in cancer genes, the burden of which increases with age and decreases with parity. Cell clones with drivers often originate during the first decades of life and subsequently progressively colonize the epithelial lining of the endometrium. Our results show that mutational landscapes differ markedly between normal tissues-perhaps shaped by differences in their structure and physiology-and indicate that the procession of neoplastic change that leads to endometrial cancer is initiated early in life.


Whole-genome sequencing of normal human endometrial glands shows that most are clonal cell populations and frequently carry cancer driver mutations that occur early in life, and that parity has a protective effect.


  
Direct-bandgap emission from hexagonal Ge and SiGe alloys 期刊论文
NATURE, 2020, 580 (7802) : 205-+
作者:  Meiners, Thorsten;  Frolov, Timofey;  Rudd, Robert E.;  Dehm, Gerhard;  Liebscher, Christian H.
收藏  |  浏览/下载:28/0  |  提交时间:2020/07/03

Silicon crystallized in the usual cubic (diamond) lattice structure has dominated the electronics industry for more than half a century. However, cubic silicon (Si), germanium (Ge) and SiGe alloys are all indirect-bandgap semiconductors that cannot emit light efficiently. The goal(1) of achieving efficient light emission from group-IV materials in silicon technology has been elusive for decades(2-6). Here we demonstrate efficient light emission from direct-bandgap hexagonal Ge and SiGe alloys. We measure a sub-nanosecond, temperature-insensitive radiative recombination lifetime and observe an emission yield similar to that of direct-bandgap group-III-V semiconductors. Moreover, we demonstrate that, by controlling the composition of the hexagonal SiGe alloy, the emission wavelength can be continuously tuned over a broad range, while preserving the direct bandgap. Our experimental findings are in excellent quantitative agreement with ab initio theory. Hexagonal SiGe embodies an ideal material system in which to combine electronic and optoelectronic functionalities on a single chip, opening the way towards integrated device concepts and information-processing technologies.


A hexagonal (rather than cubic) alloy of silicon and germanium that has a direct (rather than indirect) bandgap emits light efficiently across a range of wavelengths, enabling electronic and optoelectronic functionalities to be combined on a single chip.


  
Mott and generalized Wigner crystal states in WSe2/WS2 moire superlattices 期刊论文
NATURE, 2020, 579 (7799) : 359-+
作者:  Yuan, Jie;  Chang, Si-Yuan;  Yin, Shi-Gang;  Liu, Zhi-Yang;  Cheng, Xiu;  Liu, Xi-Juan;  Jiang, Qiang;  Gao, Ge;  Lin, De-Ying;  Kang, Xin-Lei;  Ye, Shi-Wei;  Chen, Zheng;  Yin, Jiang-An;  Hao, Pei;  Jiang, Lubin;  Cai, Shi-Qing
收藏  |  浏览/下载:50/0  |  提交时间:2020/07/03

Strongly correlated insulating Mott and generalized Wigner phases are detected in WSe2/WS2 moire superlattices, and their electrical properties and excited spin states are studied using an optical technique.


Moire superlattices can be used to engineer strongly correlated electronic states in two-dimensional van der Waals heterostructures, as recently demonstrated in the correlated insulating and superconducting states observed in magic-angle twisted-bilayer graphene and ABC trilayer graphene/boron nitride moire superlattices(1-4). Transition metal dichalcogenide moire heterostructures provide another model system for the study of correlated quantum phenomena(5) because of their strong light-matter interactions and large spin-orbit coupling. However, experimental observation of correlated insulating states in this system is challenging with traditional transport techniques. Here we report the optical detection of strongly correlated phases in semiconducting WSe2/WS2 moire superlattices. We use a sensitive optical detection technique and reveal a Mott insulator state at one hole per superlattice site and surprising insulating phases at 1/3 and 2/3 filling of the superlattice, which we assign to generalized Wigner crystallization on the underlying lattice(6-11). Furthermore, the spin-valley optical selection rules(12-14) of transition metal dichalcogenide heterostructures allow us to optically create and investigate low-energy excited spin states in the Mott insulator. We measure a very long spin relaxation lifetime of many microseconds in the Mott insulating state, orders of magnitude longer than that of charge excitations. Our studies highlight the value of using moire superlattices beyond graphene to explore correlated physics.


  
Skewed distributions of lifetime reproductive success: beyond mean and variance 期刊论文
ECOLOGY LETTERS, 2020, 23 (4) : 748-756
作者:  Tuljapurkar, Shripad;  Zuo, Wenyun;  Coulson, Tim;  Horvitz, Carol;  Gaillard, Jean-Michel
收藏  |  浏览/下载:7/0  |  提交时间:2020/07/02
Age plus stage  evolution  life history  lifetime reproductive success  
Coherent laser spectroscopy of highly charged ions using quantum logic 期刊论文
NATURE, 2020, 578 (7793) : 60-+
作者:  Oh, Myoung Hwan;  Cho, Min Gee;  Chung, Dong Young;  Park, Inchul;  Kwon, Youngwook Paul;  Ophus, Colin;  Kim, Dokyoon;  Kim, Min Gyu;  Jeong, Beomgyun;  Gu, X. Wendy;  Jo, Jinwoung;  Yoo, Ji Mun;  Hong, Jaeyoung;  McMains, Sara;  Kang, Kisuk;  Sung, Yung-Eun;  Alivisatos, A. Paul;  Hyeon, Taeghwan
收藏  |  浏览/下载:52/0  |  提交时间:2020/07/03

Precision spectroscopy of atomic systems(1) is an invaluable tool for the study of fundamental interactions and symmetries(2). Recently, highly charged ions have been proposed to enable sensitive tests of physics beyond the standard model(2-5) and the realization of high-accuracy atomic clocks(3,5), owing to their high sensitivity to fundamental physics and insensitivity to external perturbations, which result from the high binding energies of their outer electrons. However, the implementation of these ideas has been hindered by the low spectroscopic accuracies (of the order of parts per million) achieved so far(6-8). Here we cool trapped, highly charged argon ions to the lowest temperature reported so far, and study them using coherent laser spectroscopy, achieving an increase in precision of eight orders of magnitude. We use quantum logic spectroscopy(9,10) to probe the forbidden optical transition in Ar-40(13+) at a wavelength of 441 nanometres and measure its excited-state lifetime and g-factor. Our work unlocks the potential of highly charged ions as ubiquitous atomic systems for use in quantum information processing, as frequency standards and in highly sensitive tests of fundamental physics, such as searches for dark-matter candidates(11) or violations of fundamental symmetries(2).


The precision of laser spectroscopy of highly charged ions is improved by eight orders of magnitude by cooling trapped, highly charged ions and using quantum logic spectroscopy, thereby enabling tests of fundamental physics.


  
Inter-decadal variability of the location of maximum intensity of category 4-5 typhoons and its implication on landfall intensity in East Asia 期刊论文
INTERNATIONAL JOURNAL OF CLIMATOLOGY, 2019, 39 (4) : 1839-1852
作者:  Liu, Kin Sik;  Chan, Johnny C. L.
收藏  |  浏览/下载:7/0  |  提交时间:2019/11/26
climate variability  lifetime-maximum intensity  tropical cyclone landfall  
Changes in Global Tropospheric OH Expected as a Result of Climate Change Over the Last Several Decades 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2018, 123 (18) : 10774-10795
作者:  Nicely, Julie M.;  Canty, Timothy P.;  Manyin, Michael;  Oman, Luke D.;  Salawitch, Ross J.;  Steenrod, Stephen D.;  Strahan, Susan E.;  Strode, Sarah A.
收藏  |  浏览/下载:14/0  |  提交时间:2019/04/09
hydroxyl radical  methane lifetime  oxidizing capacity  tropospheric chemistry  climate change  
NO(x) Lifetime and NO(y) Partitioning During WINTER 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2018, 123 (17) : 9813-9827
作者:  Kenagy, Hannah S.;  Sparks, Tamara L.;  Ebben, Carlena J.;  Wooldrige, Paul J.;  Lopez-Hilfiker, Felipe D.;  Lee, Ben H.;  Thornton, Joel A.;  McDuffie, Erin E.;  Fibiger, Dorothy L.;  Brown, Steven S.;  Montzka, Denise D.;  Weinheimer, Andrew J.;  Schroder, Jason C.;  Campuzano-Jost, Pedro;  Day, Douglas A.;  Jimenez, Jose L.;  Dibb, Jack E.;  Campos, Teresa;  Shah, Viral;  Jaegle, Lyatt;  Cohen, Ronald C.
收藏  |  浏览/下载:16/0  |  提交时间:2019/04/09
NOx  nitric acid  WINTER  NOx lifetime  winter  heterogeneous hydrolysis