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国际研究发现臭氧污染影响植物生长与碳吸收能力 快报文章
气候变化快报,2024年第19期
作者:  裴惠娟
Microsoft Word(16Kb)  |  收藏  |  浏览/下载:471/0  |  提交时间:2024/10/05
Tropical Forests  Ground-Level Ozone  Productivity  Carbon  
利用综合建模框架以评估灌溉在区域尺度上的影响 快报文章
资源环境快报,2022年第19期
作者:  吴秀平
Microsoft Word(16Kb)  |  收藏  |  浏览/下载:727/1  |  提交时间:2022/10/14
integrated modeling framework  surface and ground water resources  assess  
Direct evidence of poison-driven widespread population decline in a wild vertebrate 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2020, 117 (28) : 16418-16423
作者:  Mateo-Tomas, Patricia;  Olea, Pedro P.;  Minguez, Eva;  Mateo, Rafael;  Vinuela, Javier
收藏  |  浏览/下载:59/0  |  提交时间:2020/07/06
wildlife poisoning  population dynamics  sentinel species  on-ground monitoring  diclofenac  
Effects of Groundwater Pumping on Ground Surface Temperature: A Regional Modeling Study in the North China Plain 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2020, 125 (9)
作者:  Yang, Chen;  Li, Hong-Yi;  Fang, Yilin;  Cui, Chixiao;  Wang, Tianye;  Zheng, Chunmiao;  Leung, L. Ruby;  Maxwell, Reed M.;  Zhang, You-Kuan;  Yang, Xiaofan
收藏  |  浏览/下载:28/0  |  提交时间:2020/07/02
the North China Plain  groundwater pumping  ground surface temperature  integrated hydrologic modeling  ParFlow  CLM  
Profiles of MBL Cloud and Drizzle Microphysical Properties Retrieved From Ground-Based Observations and Validated by Aircraft In Situ Measurements Over the Azores 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2020, 125 (9)
作者:  Wu, Peng;  Dong, Xiquan;  Xi, Baike;  Tian, Jingjing;  Ward, Dale M.
收藏  |  浏览/下载:22/0  |  提交时间:2020/07/02
aircraft measurements  cloud and precipitation  ground-based observations  microphysics retrieval  
Aerosol Effects on Lightning Characteristics: A Comparison of Polluted and Clean Regimes 期刊论文
GEOPHYSICAL RESEARCH LETTERS, 2020, 47 (9)
作者:  Liu, Y.;  Guha, A.;  Said, R.;  Williams, E.;  Lapierre, J.;  Stock, M.;  Heckman, S.
收藏  |  浏览/下载:20/0  |  提交时间:2020/07/02
lightning  aerosol effects  intracloud lightning  cloud-to-ground lightning  thermodynamic effects  
In Situ Estimates of Freezing/Melting Point Depression in Agricultural Soils Using Permittivity and Temperature Measurements 期刊论文
WATER RESOURCES RESEARCH, 2020, 56 (5)
作者:  Lara, R. Pardo;  Berg, A. A.;  Warland, J.;  Tetlock, Erica
收藏  |  浏览/下载:29/0  |  提交时间:2020/07/02
soil moisture  freeze thaw  freezing point depression  soil freezing curve  seasonally frozen ground  cryosphere  
Confinement of atomically defined metal halide sheets in a metal-organic framework 期刊论文
NATURE, 2020, 577 (7788) : 64-+
作者:  Gonzalez, Miguel I.;  Turkiewicz, Ari B.;  Darago, Lucy E.;  Oktawiec, Julia;  Bustillo, Karen;  Grandjean, Fernande;  Long, Gary J.;  Long, Jeffrey R.
收藏  |  浏览/下载:25/0  |  提交时间:2020/07/03

The size-dependent and shape-dependent characteristics that distinguish nanoscale materials from bulk solids arise from constraining the dimensionality of an inorganic structure(1-3). As a consequence, many studies have focused on rationally shaping these materials to influence and enhance their optical, electronic, magnetic and catalytic properties(4-6). Although a select number of stable clusters can typically be synthesized within the nanoscale regime for a specific composition, isolating clusters of a predetermined size and shape remains a challenge, especially for those derived from two-dimensional materials. Here we realize a multidentate coordination environment in a metal-organic framework to stabilize discrete inorganic clusters within a porous crystalline support. We show confined growth of atomically defined nickel(ii) bromide, nickel(ii) chloride, cobalt(ii) chloride and iron(ii) chloride sheets through the peripheral coordination of six chelating bipyridine linkers. Notably, confinement within the framework defines the structure and composition of these sheets and facilitates their precise characterization by crystallography. Each metal(ii) halide sheet represents a fragment excised from a single layer of the bulk solid structure, and structures obtained at different precursor loadings enable observation of successive stages of sheet assembly. Finally, the isolated sheets exhibit magnetic behaviours distinct from those of the bulk metal halides, including the isolation of ferromagnetically coupled large-spin ground states through the elimination of long-range, interlayer magnetic ordering. Overall, these results demonstrate that the pore environment of a metal-organic framework can be designed to afford precise control over the size, structure and spatial arrangement of inorganic clusters.


  
Entanglement-based secure quantum cryptography over 1,120 kilometres 期刊论文
NATURE, 2020
作者:  Paldi, Flora;  Alver, Bonnie;  Robertson, Daniel;  Schalbetter, Stephanie A.;  Kerr, Alastair;  Kelly, David A.;  Baxter, Jonathan;  Neale, Matthew J.;  Marston, Adele L.
收藏  |  浏览/下载:78/0  |  提交时间:2020/07/03

An efficient entanglement-based quantum key distribution is sent from the Micius satellite to two ground observatories 1,120 kilometres apart to establish secure quantum cryptography for the exchange ofquantum keys.


Quantum key distribution (QKD)(1-3)is a theoretically secure way of sharing secret keys between remote users. It has been demonstrated in a laboratory over a coiled optical fibre up to 404 kilometres long(4-7). In the field, point-to-point QKD has been achieved from a satellite to a ground station up to 1,200 kilometres away(8-10). However, real-world QKD-based cryptography targets physically separated users on the Earth, for which the maximum distance has been about 100 kilometres(11,12). The use of trusted relays can extend these distances from across a typical metropolitan area(13-16)to intercity(17)and even intercontinental distances(18). However, relays pose security risks, which can be avoided by using entanglement-based QKD, which has inherent source-independent security(19,20). Long-distance entanglement distribution can be realized using quantum repeaters(21), but the related technology is still immature for practical implementations(22). The obvious alternative for extending the range of quantum communication without compromising its security is satellite-based QKD, but so far satellite-based entanglement distribution has not been efficient(23)enough to support QKD. Here we demonstrate entanglement-based QKD between two ground stations separated by 1,120 kilometres at a finite secret-key rate of 0.12 bits per second, without the need for trusted relays. Entangled photon pairs were distributed via two bidirectional downlinks from the Micius satellite to two ground observatories in Delingha and Nanshan in China. The development of a high-efficiency telescope and follow-up optics crucially improved the link efficiency. The generated keys are secure for realistic devices, because our ground receivers were carefully designed to guarantee fair sampling and immunity to all known side channels(24,25). Our method not only increases the secure distance on the ground tenfold but also increases the practical security of QKD to an unprecedented level.


  
Detection of metastable electronic states by Penning trap mass spectrometry 期刊论文
NATURE, 2020, 581 (7806) : 42-+
作者:  Rauch, Jennifer N.;  Luna, Gabriel;  Guzman, Elmer;  Audouard, Morgane;  Challis, Collin;  Sibih, Youssef E.;  Leshuk, Carolina;  Hernandez, Israel;  Wegmann, Susanne;  Hyman, Bradley T.;  Gradinaru, Viviana;  Kampmann, Martin;  Kosik, Kenneth S.
收藏  |  浏览/下载:27/0  |  提交时间:2020/07/03

State-of-the-art optical clocks(1) achieve precisions of 10(-18) or better using ensembles of atoms in optical lattices(2,3) or individual ions in radio-frequency traps(4,5). Promising candidates for use in atomic clocks are highly charged ions(6) (HCIs) and nuclear transitions(7), which are largely insensitive to external perturbations and reach wavelengths beyond the optical range(8) that are accessible to frequency combs(9). However, insufficiently accurate atomic structure calculations hinder the identification of suitable transitions in HCIs. Here we report the observation of a long-lived metastable electronic state in an HCI by measuring the mass difference between the ground and excited states in rhenium, providing a non-destructive, direct determination of an electronic excitation energy. The result is in agreement with advanced calculations. We use the high-precision Penning trap mass spectrometer PENTATRAP to measure the cyclotron frequency ratio of the ground state to the metastable state of the ion with a precision of 10(-11)-an improvement by a factor of ten compared with previous measurements(10,11). With a lifetime of about 130 days, the potential soft-X-ray frequency reference at 4.96 x 10(16) hertz (corresponding to a transition energy of 202 electronvolts) has a linewidth of only 5 x 10(-8) hertz and one of the highest electronic quality factors (10(24)) measured experimentally so far. The low uncertainty of our method will enable searches for further soft-X-ray clock transitions(8,12) in HCIs, which are required for precision studies of fundamental physics(6).


Penning trap mass spectrometry is used to measure the electronic transition energy from a long-lived metastable state to the ground state in highly charged rhenium ions with a precision of 10(-11).