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IIASA开发全球气候风险热点交互网站 快报文章
气候变化快报,2020年第21期
作者:  刘燕飞
Microsoft Word(13Kb)  |  收藏  |  浏览/下载:428/0  |  提交时间:2020/11/05
interactive website  climate risk  Water, Energy and Land  
Patterns and trends of Northern Hemisphere snow mass from 1980 to 2018 期刊论文
NATURE, 2020, 581 (7808) : 294-+
作者:  Ibrahim, Nizar;  Maganuco, Simone;  Dal Sasso, Cristiano;  Fabbri, Matteo;  Auditore, Marco;  Bindellini, Gabriele;  Martill, David M.;  Zouhri, Samir;  Mattarelli, Diego A.;  Unwin, David M.;  Wiemann, Jasmina;  Bonadonna, Davide;  Amane, Ayoub;  Jakubczak, Juliana;  Joger, Ulrich;  Lauder, George V.;  Pierce, Stephanie E.
收藏  |  浏览/下载:18/0  |  提交时间:2020/05/25

Warming surface temperatures have driven a substantial reduction in the extent and duration of Northern Hemisphere snow cover(1-3). These changes in snow cover affect Earth'  s climate system via the surface energy budget, and influence freshwater resources across a large proportion of the Northern Hemisphere(4-6). In contrast to snow extent, reliable quantitative knowledge on seasonal snow mass and its trend is lacking(7-9). Here we use the new GlobSnow 3.0 dataset to show that the 1980-2018 annual maximum snow mass in the Northern Hemisphere was, on average, 3,062 +/- 35 billion tonnes (gigatonnes). Our quantification is for March (the month that most closely corresponds to peak snow mass), covers non-alpine regions above 40 degrees N and, crucially, includes a bias correction based on in-field snow observations. We compare our GlobSnow 3.0 estimates with three independent estimates of snow mass, each with and without the bias correction. Across the four datasets, the bias correction decreased the range from 2,433-3,380 gigatonnes (mean 2,867) to 2,846-3,062 gigatonnes (mean 2,938)-a reduction in uncertainty from 33% to 7.4%. On the basis of our bias-corrected GlobSnow 3.0 estimates, we find different continental trends over the 39-year satellite record. For example, snow mass decreased by 46 gigatonnes per decade across North America but had a negligible trend across Eurasia  both continents exhibit high regional variability. Our results enable a better estimation of the role of seasonal snow mass in Earth'  s energy, water and carbon budgets.


Applying a bias correction to a state-of-the-art dataset covering non-alpine regions of the Northern Hemisphere and to three other datasets yields a more constrained quantification of snow mass in March from 1980 to 2018.


  
In situ NMR metrology reveals reaction mechanisms in redox flow batteries 期刊论文
NATURE, 2020, 579 (7798) : 224-+
作者:  Ma, Jianfei;  You, Xin;  Sun, Shan;  Wang, Xiaoxiao;  Qin, Song;  Sui, Sen-Fang
收藏  |  浏览/下载:12/0  |  提交时间:2020/07/03

Large-scale energy storage is becoming increasingly critical to balancing renewable energy production and consumption(1). Organic redox flow batteries, made from inexpensive and sustainable redox-active materials, are promising storage technologies that are cheaper and less environmentally hazardous than vanadium-based batteries, but they have shorter lifetimes and lower energy density(2,3). Thus, fundamental insight at the molecular level is required to improve performance(4,5). Here we report two in situ nuclear magnetic resonance (NMR) methods of studying redox flow batteries, which are applied to two redox-active electrolytes: 2,6-dihydroxyanthraquinone (DHAQ) and 4,4 '  -((9,10-anthraquinone-2,6-diyl)dioxy) dibutyrate (DBEAQ). In the first method, we monitor the changes in the H-1 NMR shift of the liquid electrolyte as it flows out of the electrochemical cell. In the second method, we observe the changes that occur simultaneously in the positive and negative electrodes in the full electrochemical cell. Using the bulk magnetization changes (observed via the H-1 NMR shift of the water resonance) and the line broadening of the H-1 shifts of the quinone resonances as a function of the state of charge, we measure the potential differences of the two single-electron couples, identify and quantify the rate of electron transfer between the reduced and oxidized species, and determine the extent of electron delocalization of the unpaired spins over the radical anions. These NMR techniques enable electrolyte decomposition and battery self-discharge to be explored in real time, and show that DHAQ is decomposed electrochemically via a reaction that can be minimized by limiting the voltage used on charging. We foresee applications of these NMR methods in understanding a wide range of redox processes in flow and other electrochemical systems.


  
A droplet-based electricity generator with high instantaneous power density 期刊论文
NATURE, 2020, 578 (7795) : 392-+
作者:  Dabney, Will;  Kurth-Nelson, Zeb;  Uchida, Naoshige;  Starkweather, Clara Kwon;  Hassabis, Demis;  Munos, Remi;  Botvinick, Matthew
收藏  |  浏览/下载:174/0  |  提交时间:2020/07/03

Extensive efforts have been made to harvest energy from water in the form of raindrops(1-6), river and ocean waves(7,8), tides(9) and others(10-17). However, achieving a high density of electrical power generation is challenging. Traditional hydraulic power generation mainly uses electromagnetic generators that are heavy, bulky, and become inefficient with low water supply. An alternative, the water-droplet/solid-based triboelectric nanogenerator, has so far generated peak power densities of less than one watt per square metre, owing to the limitations imposed by interfacial effects-as seen in characterizations of the charge generation and transfer that occur at solid-liquid(1-4) or liquid-liquid(5,18) interfaces. Here we develop a device to harvest energy from impinging water droplets by using an architecture that comprises a polytetrafluoroethylene film on an indium tin oxide substrate plus an aluminium electrode. We show that spreading of an impinged water droplet on the device bridges the originally disconnected components into a closed-loop electrical system, transforming the conventional interfacial effect into a bulk effect, and so enhancing the instantaneous power density by several orders of magnitude over equivalent devices that are limited by interfacial effects.


A device involving a polytetrafluoroethylene film, an indium tin oxide substrate and an aluminium electrode allows improved electricity generation from water droplets, which bridge the previously disconnected circuit components.


  
An orbital water-ice cycle on comet 67P from colour changes 期刊论文
NATURE, 2020, 578 (7793) : 49-+
作者:  Oh, Myoung Hwan;  Cho, Min Gee;  Chung, Dong Young;  Park, Inchul;  Kwon, Youngwook Paul;  Ophus, Colin;  Kim, Dokyoon;  Kim, Min Gyu;  Jeong, Beomgyun;  Gu, X. Wendy;  Jo, Jinwoung;  Yoo, Ji Mun;  Hong, Jaeyoung;  McMains, Sara;  Kang, Kisuk;  Sung, Yung-Eun;  Alivisatos, A. Paul;  Hyeon, Taeghwan
收藏  |  浏览/下载:52/0  |  提交时间:2020/07/03

Solar heating of a cometary surface provides the energy necessary to sustain gaseous activity, through which dust is removed(1,2). In this dynamical environment, both the coma(3,4) and the nucleus(5,6) evolve during the orbit, changing their physical and compositional properties. The environment around an active nucleus is populated by dust grains with complex and variegated shapes(7), lifted and diffused by gases freed from the sublimation of surface ices(8,9). The visible colour of dust particles is highly variable: carbonaceous organic material-rich grains(10) appear red while magnesium silicate-rich(11,12) and water-ice-rich(13,14) grains appear blue, with some dependence on grain size distribution, viewing geometry, activity level and comet family type. We know that local colour changes are associated with grain size variations, such as in the bluer jets made of submicrometre grains on comet Hale-Bopp(15) or in the fragmented grains in the coma(16) of C/1999 S4 (LINEAR). Apart from grain size, composition also influences the coma'  s colour response, because transparent volatiles can introduce a substantial blueing in scattered light, as observed in the dust particles ejected after the collision of the Deep Impact probe with comet 9P/Tempel 1(17). Here we report observations of two opposite seasonal colour cycles in the coma and on the surface of comet 67P/Churyumov-Gerasimenko through its perihelion passage(18). Spectral analysis indicates an enrichment of submicrometre grains made of organic material and amorphous carbon in the coma, causing reddening during the passage. At the same time, the progressive removal of dust from the nucleus causes the exposure of more pristine and bluish icy layers on the surface. Far from the Sun, we find that the abundance of water ice on the nucleus is reduced owing to redeposition of dust and dehydration of the surface layer while the coma becomes less red.


  
Assimilating GRACE Into a Land Surface Model in the Presence of an Irrigation-Induced Groundwater Trend 期刊论文
WATER RESOURCES RESEARCH, 2019, 55 (12) : 11274-11294
作者:  Nie, Wanshu;  Zaitchik, Benjamin F.;  Rodell, Matthew;  Kumar, Sujay V.;  Arsenault, Kristi R.;  Li, Bailing;  Getirana, Augusto
收藏  |  浏览/下载:16/0  |  提交时间:2020/02/16
GRACE TWS  data assimilation  irrigation  groundwater withdrawal  water and energy fluxes  High Plains Aquifer  
Water security implications of coal-fired power plants financed through China's Belt and Road Initiative 期刊论文
ENERGY POLICY, 2019, 132: 1101-1109
作者:  Alkon, Meir;  He, Xiaogang;  Paris, Aubrey R.;  Liao, Wenying;  Hodson, Thomas;  Wanders, Niko;  Wang, Yaoping
收藏  |  浏览/下载:18/0  |  提交时间:2019/11/27
Sustainability  Belt and Road Initiative  Water-energy nexus  Water resources  Water security  Coal  CPEC  Energy  
Observed Atmospheric and Surface Variability on Heterogeneous Terrain at the Hectometer Scale and Related Advective Transports 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2019, 124 (16) : 9407-9422
作者:  Simo, Gemma;  Cuxart, Joan;  Jimenez, Maria A.;  Martinez-Villagrasa, Daniel;  Picos, Rodrigo;  Lopez-Grifol, Alvaro;  Marti, Belen
收藏  |  浏览/下载:8/0  |  提交时间:2019/11/27
atmospheric and upper-soil variability  surface energy and water budgets  local thermal advection  station representativeness  humidity advection and evapotranspiration  hectometer scale  
Decoupling impact and public utility conservation investment 期刊论文
ENERGY POLICY, 2019, 130: 311-319
作者:  Michelfelder, Richard A.;  39;Ascendis, Dylan
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/27
Decoupling  Public utility cost of common equity  Energy and water efficiency  
Evaluating regulatory strategies for mitigating hydrological risk in Brazil through diversification of its electricity mix 期刊论文
ENERGY POLICY, 2019, 128: 393-401
作者:  Paim, Maria-Augusta;  Dalmarco, Arthur R.;  Yang, Chung-Han;  Salas, Pablo;  Lindner, Soren;  Mercure, Jean-Francois;  Osorio de Andrade Guerra, Jose Baltazar Salgueirinho;  Derani, Cristiane;  da Silva, Tatiana Bruce;  Vinuales, Jorge E.
收藏  |  浏览/下载:22/0  |  提交时间:2019/11/26
Hydropower  Hydrological risk  Electricity mix  Water-Energy-Food Nexus  Brazilian law and regulation  Integrated Assessment Modelling (lAM)