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Estimating US fossil fuel CO2 emissions from measurements of C-14 in atmospheric CO2 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2020, 117 (24) : 13300-13307
作者:  Basu, Sourish;  Lehman, Scott J.;  Miller, John B.;  Andrews, Arlyn E.;  Sweeney, Colm;  Gurney, Kevin R.;  Xu, Xiaomei;  Southon, John;  Tans, Pieter P.
收藏  |  浏览/下载:18/0  |  提交时间:2020/06/09
fossil fuel CO2  radiocarbon  atmospheric inverse modeling  
Early atmospheric contamination on the top of the Himalayas since the onset of the European Industrial Revolution 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2020, 117 (8) : 3967-3973
作者:  Gabrielli, Paolo;  Wegner, Anna;  Sierra-Hernandez, M. Roxana;  Beaudon, Emilie;  Davis, Mary;  Barker, Joel D.;  Thompson, Lonnie G.
收藏  |  浏览/下载:8/0  |  提交时间:2020/05/13
ice cores  trace metals  paleoenvironment  monsoon  North Atlantic Oscillation  
Premature mortality related to United States cross-state air pollution 期刊论文
NATURE, 2020, 578 (7794) : 261-+
作者:  Helmink, Beth A.;  Reddy, Sangeetha M.;  Gao, Jianjun;  Zhang, Shaojun;  Basar, Rafet;  Thakur, Rohit;  Yizhak, Keren;  Sade-Feldman, Moshe;  Blando, Jorge;  Han, Guangchun;  Gopalakrishnan, Vancheswaran;  Xi, Yuanxin;  Zhao, Hao;  Amaria, Rodabe N.;  Tawbi, Hussein A.;  Cogdill, Alex P.;  Liu, Wenbin;  LeBleu, Valerie S.;  Kugeratski, Fernanda G.;  Patel, Sapna;  Davies, Michael A.;  Hwu, Patrick;  Lee, Jeffrey E.;  Gershenwald, Jeffrey E.;  Lucci, Anthony;  Arora, Reetakshi;  Woodman, Scott;  Keung, Emily Z.;  Gaudreau, Pierre-Olivier;  Reuben, Alexandre;  Spencer, Christine N.;  Burton, Elizabeth M.;  Haydu, Lauren E.;  Lazar, Alexander J.;  Zapassodi, Roberta;  Hudgens, Courtney W.;  Ledesma, Deborah A.;  Ong, SuFey;  Bailey, Michael;  Warren, Sarah;  Rao, Disha;  Krijgsman, Oscar;  Rozeman, Elisa A.;  Peeper, Daniel;  Blank, Christian U.;  Schumacher, Ton N.;  Butterfield, Lisa H.;  Zelazowska, Monika A.;  McBride, Kevin M.;  Kalluri, Raghu;  Allison, James;  Petitprez, Florent;  Fridman, Wolf Herman;  Sautes-Fridman, Catherine;  Hacohen, Nir;  Rezvani, Katayoun;  Sharma, Padmanee;  Tetzlaff, Michael T.;  Wang, Linghua;  Wargo, Jennifer A.
收藏  |  浏览/下载:39/0  |  提交时间:2020/05/13

Outdoor air pollution adversely affects human health and is estimated to be responsible for five to ten per cent of the total annual premature mortality in the contiguous United States(1-3). Combustion emissions from a variety of sources, such as power generation or road traffic, make a large contribution to harmful air pollutants such as ozone and fine particulate matter (PM2.5)(4). Efforts to mitigate air pollution have focused mainly on the relationship between local emission sources and local air quality(2). Air quality can also be affected by distant emission sources, however, including emissions from neighbouring federal states(5,6). This cross-state exchange of pollution poses additional regulatory challenges. Here we quantify the exchange of air pollution among the contiguous United States, and assess its impact on premature mortality that is linked to increased human exposure to PM2.5 and ozone from seven emission sectors for 2005 to 2018. On average, we find that 41 to 53 per cent of air-quality-related premature mortality resulting from a state'  s emissions occurs outside that state. We also find variations in the cross-state contributions of different emission sectors and chemical species to premature mortality, and changes in these variations over time. Emissions from electric power generation have the greatest cross-state impacts as a fraction of their total impacts, whereas commercial/residential emissions have the smallest. However, reductions in emissions from electric power generation since 2005 have meant that, by 2018, cross-state premature mortality associated with the commercial/residential sector was twice that associated with power generation. In terms of the chemical species emitted, nitrogen oxides and sulfur dioxide emissions caused the most cross-state premature deaths in 2005, but by 2018 primary PM2.5 emissions led to cross-state premature deaths equal to three times those associated with sulfur dioxide emissions. These reported shifts in emission sectors and emission species that contribute to premature mortality may help to guide improvements to air quality in the contiguous United States.


  
Isotopic constraint on the twentieth-century increase in tropospheric ozone 期刊论文
NATURE, 2019, 570 (7760) : 224-+
作者:  Yeung, Laurence Y.;  Murray, Lee. T.;  Martinerie, Patricia;  Witrant, Emmanuel;  Hu, Huanting;  Banerjee, Asmita;  Orsi, Anais;  Chappellaz, Jerome
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/27
Quantitative constraints on autoxidation and dimer formation from direct probing of monoterpene-derived peroxy radical chemistry 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2018, 115 (48) : 12142-12147
作者:  Zhao, Yue;  Thornton, Joel A.;  Pye, Havala O. T.
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/27
monoterpenes  peroxy radicals  autoxidation  dimers  particle formation  
Five-S-isotope evidence of two distinct mass-independent sulfur isotope effects and implications for the modern and Archean atmospheres 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2018, 115 (34) : 8541-8546
作者:  Lin, Mang;  Zhang, Xiaolin;  Li, Menghan;  Xu, Yilun;  Zhang, Zhisheng;  Tao, Jun;  Su, Binbin;  Liu, Lanzhong;  Shen, Yanan;  Thiemens, Mark H.
收藏  |  浏览/下载:10/0  |  提交时间:2019/11/27
cosmogenic sulfur-35  stable sulfur isotope anomalies  sulfate aerosols  combustion  recombination reactions  
Global-scale evidence for the refractory nature of riverine black carbon 期刊论文
NATURE GEOSCIENCE, 2018, 11 (8) : 584-+
作者:  Coppola, Alysha I.;  Wiedemeier, Daniel B.;  Galy, Valier;  Haghipour, Negar;  Hanke, Ulrich M.;  Nascimento, Gabriela S.;  Usman, Muhammed;  Blattmann, Thomas M.;  Reisser, Moritz;  Freymond, Chantal V.;  Zhao, Meixun;  Voss, Britta;  Wacker, Lukas;  Schefuss, Enno;  Peucker-Ehrenbrink, Bernhard;  Abiven, Samuel;  Schmidt, Michael W. I.;  Eglinton, Timothy I.
收藏  |  浏览/下载:15/0  |  提交时间:2019/04/09
Assessment of methane emissions from the US oil and gas supply chain 期刊论文
SCIENCE, 2018, 361 (6398) : 186-188
作者:  Alvarez, Ramon A.;  Zavala-Araiza, Daniel;  Lyon, David R.;  Allen, David T.;  Barkley, Zachary R.;  Brandt, Adam R.;  Davis, Kenneth J.;  Herndon, Scott C.;  Jacob, Daniel J.;  Karion, Anna;  Kort, Eric A.;  Lamb, Brian K.;  Lauvaux, Thomas;  Maasakkers, Joannes D.;  Marchese, Anthony J.;  Omara, Mark;  Pacala, Stephen W.;  Peischl, Jeff;  Robinson, Allen L.;  Shepson, Paul B.;  Sweeney, Colm;  Townsend-Small, Amy;  Wofsy, Steven C.;  Hamburg, Steven P.
收藏  |  浏览/下载:11/0  |  提交时间:2019/11/27
Atmospheric sulfur isotopic anomalies recorded at Mt. Everest across the Anthropocene 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2018, 115 (27) : 6964-6969
作者:  Lin, Mang;  Kang, Shichang;  Shaheen, Robina;  Li, Chaoliu;  Hsu, Shih-Chieh;  Thiemens, Mark H.
收藏  |  浏览/下载:9/0  |  提交时间:2019/11/27
Himalayas  mass-independent fractionation  aerosol  glacier  Archean  
Beyond fossil fuel-driven nitrogen transformations 期刊论文
SCIENCE, 2018, 360 (6391)
作者:  Chen, Jingguang G.;  Crooks, Richard M.;  Seefeldt, Lance C.;  Bren, Kara L.;  Bullock, R. Morris;  Darensbourg, Marcetta Y.;  Holland, Patrick L.;  Hoffman, Brian;  Janik, Michael J.;  Jones, Anne K.;  Kanatzidis, Mercouri G.;  King, Paul;  Lancaster, Kyle M.;  Lymar, Sergei V.;  Pfromm, Peter;  Schneider, William F.;  Schrock, Richard R.
收藏  |  浏览/下载:45/0  |  提交时间:2019/11/27