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Preindustrial (CH4)-C-14 indicates greater anthropogenic fossil CH4 emissions 期刊论文
NATURE, 2020, 578 (7795) : 409-+
作者:  Keener, Megan;  Hunt, Camden;  Carroll, Timothy G.;  Kampel, Vladimir;  Dobrovetsky, Roman;  Hayton, Trevor W.;  Menard, Gabriel
收藏  |  浏览/下载:25/0  |  提交时间:2020/05/13

Atmospheric methane (CH4) is a potent greenhouse gas, and its mole fraction has more than doubled since the preindustrial era(1). Fossil fuel extraction and use are among the largest anthropogenic sources of CH4 emissions, but the precise magnitude of these contributions is a subject of debate(2,3). Carbon-14 in CH4 ((CH4)-C-14) can be used to distinguish between fossil (C-14-free) CH4 emissions and contemporaneous biogenic sources  however, poorly constrained direct (CH4)-C-14 emissions from nuclear reactors have complicated this approach since the middle of the 20th century(4,5). Moreover, the partitioning of total fossil CH4 emissions (presently 172 to 195 teragrams CH4 per year)(2,3) between anthropogenic and natural geological sources (such as seeps and mud volcanoes) is under debate  emission inventories suggest that the latter account for about 40 to 60 teragrams CH4 per year(6,7). Geological emissions were less than 15.4 teragrams CH4 per year at the end of the Pleistocene, about 11,600 years ago(8), but that period is an imperfect analogue for present-day emissions owing to the large terrestrial ice sheet cover, lower sea level and extensive permafrost. Here we use preindustrial-era ice core (CH4)-C-14 measurements to show that natural geological CH4 emissions to the atmosphere were about 1.6 teragrams CH4 per year, with a maximum of 5.4 teragrams CH4 per year (95 per cent confidence limit)-an order of magnitude lower than the currently used estimates. This result indicates that anthropogenic fossil CH4 emissions are underestimated by about 38 to 58 teragrams CH4 per year, or about 25 to 40 per cent of recent estimates. Our record highlights the human impact on the atmosphere and climate, provides a firm target for inventories of the global CH4 budget, and will help to inform strategies for targeted emission reductions(9,10).


Isotopic evidence from ice cores indicates that preindustrial-era geological methane emissions were lower than previously thought, suggesting that present-day emissions of methane from fossil fuels are underestimated.


  
Challenges for the recovery of the ozone layer 期刊论文
NATURE GEOSCIENCE, 2019, 12 (8) : 592-596
作者:  Fang, Xuekun;  Pyle, John A.;  Chipperfield, Martyn P.;  Daniel, John S.;  Park, Sunyoung;  Prinn, Ronald G.
收藏  |  浏览/下载:9/0  |  提交时间:2019/11/27
Widespread global peatland establishment and persistence over the last 130,000 y 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2019, 116 (11) : 4822-4827
作者:  Treat, Claire C.;  Kleinen, Thomas;  Broothaerts, Nils;  Dalton, April S.;  Dommain, Rene;  Douglas, Thomas A.;  Drexler, Judith Z.;  Finkelstein, Sarah A.;  Grosse, Guido;  Hope, Geoffrey;  Hutchings, Jack;  Jones, Miriam C.;  Kuhry, Peter;  Lacourse, Terri;  Lahteenoja, Outi;  Loisel, Julie;  Notebaert, Bastiaan;  Payne, Richard J.;  Peteet, Dorothy M.;  Sannel, A. Britta K.;  Stelling, Jonathan M.;  Strauss, Jens;  Swindles, Graeme T.;  Talbot, Julie;  Tarnocai, Charles;  Verstraeten, Gert;  Williams, Christopher J.;  Xia, Zhengyu;  Yu, Zicheng;  Valiranta, Minna;  Hattestrand, Martina;  Alexanderson, Helena;  Brovkin, Victor
收藏  |  浏览/下载:18/0  |  提交时间:2019/11/27
peatlands  carbon  methane  carbon burial  Quaternary  
Abiotic methane synthesis and serpentinization in olivine-hosted fluid inclusions 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2019, 116 (36) : 17666-17672
作者:  Klein, Frieder;  Grozeva, Niya G.;  Seewald, Jeffrey S.
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/27
abiotic methane  fluid inclusions  serpentinization  methane seeps  carbon cycling  
Rivers across the Siberian Arctic unearth the patterns of carbon release from thawing permafrost 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2019, 116 (21) : 10280-10285
作者:  Wild, Birgit;  Andersson, August;  Broder, Lisa;  Vonk, Jorien;  Hugelius, Gustaf;  McClelland, James W.;  Song, Wenjun;  Raymond, Peter A.;  Gustafsson, Orjan
收藏  |  浏览/下载:7/0  |  提交时间:2019/11/27
carbon cycle  climate change  radiocarbon  peat  leaching  
Widespread nitrous oxide undersaturation in farm waterbodies creates an unexpected greenhouse gas sink 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2019, 116 (20) : 9814-9819
作者:  Webb, Jackie R.;  Hayes, Nicole M.;  Simpson, Gavin L.;  Leavitt, Peter R.;  Baulch, Helen M.;  Finlay, Kerri
收藏  |  浏览/下载:5/0  |  提交时间:2019/11/27
nitrous oxide  agriculture  farm reservoirs  impoundments  greenhouse gases  
Pyrite formation from FeS and H2S is mediated through microbial redox activity 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2019, 116 (14) : 6897-6902
作者:  Thiel, Joana;  Byrne, James M.;  Kappler, Andreas;  Schink, Bernhard;  Pester, Michael
收藏  |  浏览/下载:7/0  |  提交时间:2019/11/27
sulfur cycle  biogenic mineral transformation  syntrophy  deep biosphere  origin of life  
Termite mounds mitigate half of termite methane emissions 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2018, 115 (52) : 13306-13311
作者:  Nauer, Philipp A.;  Hutley, Lindsay B.;  Arndt, Stefan K.
收藏  |  浏览/下载:9/0  |  提交时间:2019/11/27
termite mounds  methane oxidation  methanotrophs  termite biomass  methane emissions  
Path-dependent reductions in CO2 emission budgets caused by permafrost carbon release 期刊论文
NATURE GEOSCIENCE, 2018, 11 (11) : 830-+
作者:  Gasser, T.;  Kechiar, M.;  Ciais, P.;  Burke, E. J.;  Kleinen, T.;  Zhu, D.;  Huang, Y.;  Ekici, A.;  Obersteiner, M.
收藏  |  浏览/下载:6/0  |  提交时间:2019/04/09
Methane in groundwater before, during, and after hydraulic fracturing of the Marcellus Shale 期刊论文
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2018, 115 (27) : 6970-6975
作者:  Barth-Naftilan, E.;  Sohng, J.;  Saiers, J. E.
收藏  |  浏览/下载:0/0  |  提交时间:2019/11/27
methane  groundwater  hydraulic fracturing  shale gas  water quality