GSTDTAP  > 地球科学
DOI10.1016/j.atmosres.2017.02.008
Source apportionment of PM2.5 size distribution and composition data from multiple stationary sites using a mobile platform
Liao, Ho-Tang1; Chou, Charles C. -K.2; Huang, Sheng-Hsiu1; Lu, Chia-Jung3; Chen, Chih-Chieh1; Hopke, Philip K.4; Wu, Chang-Fu1,5,6
2017-07-01
发表期刊ATMOSPHERIC RESEARCH
ISSN0169-8095
EISSN1873-2895
出版年2017
卷号190
文章类型Article
语种英语
国家Taiwan; USA
英文摘要

Several source apportionment studies considering multiple sites showed spatial variability of source contributions. However, setting up multiple fixed sites to collect comprehensive chemical speciation data is resource demanding. In this study, field campaigns were conducted at multiple receptor sites in the Mailiao and Taishi townships in Yunlin County using a mobile platform to demonstrate the feasibility of receptor modeling with particle size distribution and PM2.5 speciation data. Sources of air pollutants to all of the monitoring sites were identified and quantified using a modified positive matrix factorization (PMF) model. Modeling results indicated that a mixed source dominated by secondary aerosol was the largest contributor to PM2.5 at most sites. Adding VOC measurements with high time resolution helped to improve the source separation. Different patterns of source contributions among sites and seasons were observed showing both spatial heterogeneity and seasonal variation. (c) 2017 Published by Elsevier B.V.


英文关键词Source apportionment Mobile platform Spatial variation Positive matrix factorization (PMF) Multiple time resolution
领域地球科学
收录类别SCI-E
WOS记录号WOS:000399631900003
WOS关键词POSITIVE MATRIX FACTORIZATION ; AIR-POLLUTANT CONCENTRATIONS ; TRACE GAS MEASUREMENTS ; PARTICULATE MATTER ; SPATIAL VARIABILITY ; RECEPTOR MODELS ; SOURCE IDENTIFICATION ; SEASONAL-VARIATION ; CARBON ANALYSIS ; URBAN AREA
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/38108
专题地球科学
作者单位1.Natl Taiwan Univ, Inst Occupat Med & Ind Hyg, 17 Xu Zhou Rd, Taipei 100, Taiwan;
2.Acad Sinica, Res Ctr Environm Changes, Taipei, Taiwan;
3.Natl Taiwan Normal Univ, Dept Chem, Taipei, Taiwan;
4.Clarkson Univ, Dept Chem & Biomol Engn, Ctr Air Resources Engn & Sci, Potsdam, NY USA;
5.Natl Taiwan Univ, Dept Publ Hlth, Taipei, Taiwan;
6.Natl Taiwan Univ, Inst Environm Hlth, Taipei, Taiwan
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GB/T 7714
Liao, Ho-Tang,Chou, Charles C. -K.,Huang, Sheng-Hsiu,et al. Source apportionment of PM2.5 size distribution and composition data from multiple stationary sites using a mobile platform[J]. ATMOSPHERIC RESEARCH,2017,190.
APA Liao, Ho-Tang.,Chou, Charles C. -K..,Huang, Sheng-Hsiu.,Lu, Chia-Jung.,Chen, Chih-Chieh.,...&Wu, Chang-Fu.(2017).Source apportionment of PM2.5 size distribution and composition data from multiple stationary sites using a mobile platform.ATMOSPHERIC RESEARCH,190.
MLA Liao, Ho-Tang,et al."Source apportionment of PM2.5 size distribution and composition data from multiple stationary sites using a mobile platform".ATMOSPHERIC RESEARCH 190(2017).
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