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DOI10.1016/j.atmosres.2016.12.008
Model analysis of soil dust impacts on the boundary layer meteorology and air quality over East Asia in April 2015
Chen, Lei1,2,3; Zhang, Meigen1,2,4,5; Zhu, Jia1,2,3; Skorokhod, Andrei5
2017-05-01
发表期刊ATMOSPHERIC RESEARCH
ISSN0169-8095
EISSN1873-2895
出版年2017
卷号187
文章类型Article
语种英语
国家Peoples R China; Russia
英文摘要

An online coupled meteorology-chemistry-aerosol model (WRF-Chem) is used to quantify the impact of soil dust on radiative forcing, boundary layer meteorology and air quality over East Asia. The simulation is conducted from 14 to 17 April 2015, when an intense dust storm originated in the Gobi Desert and moved through North China. An integrated comparison analysis using surface observations, satellite, and lidar measurements demonstrates the excellent performance of the WRF-Chem model for meteorological parameters, pollutant concentrations, aerosol optical characteristics, and the spatiotemporal evolution of the dust storm. The maximum aerosol optical depth induced by dust aerosols is simulated to exceed 3.0 over the dust source areas and 1.5 over the downwind regions. Dust has a cooling effect (-1.19 W m(-2)) at the surface, a warming effect (+0.90 W m(-2)) in the atmosphere and a relatively small forcing (-0.29 W m(-2)) at the top of the atmosphere averaged over East Asia from 14 to 17 April 2015. Due to the impact of dust aerosols, the near-surface air temperature is decreased by 0.01 degrees C and 0.06 degrees C in the daytime and increased by 0.13 degrees C and 0.14 degrees C at night averaged over the dust sources and the North China Plain (NCP), respectively. The changes in relative humidity are in the range of 0.38% to +0.04% for dust sources and 0.40% to +027% for NCP. The maximum decrease in wind speed of similar to 0.1 m s(-1) is found over NCP. The planetary boundary layer height during the daytime exhibits maximum decreases of 16.34 m and 41.70 m over dust sources and NCP, respectively. The pollutant concentrations are significantly influenced by dust-related heterogeneous chemical reactions, with a maximum decrease of 1.66 ppbV for SO2, 7.15 ppbV for NOy, 35.04 mu g m(-3) for NO3-, and a maximum increase of 9.47 mu g m(-3) for 504 over the downwind areas. (C) 2016 Elsevier B.V. All rights reserved.


英文关键词Dust Boundary layer meteorology Air quality Heterogeneous reaction WRF-Chem
领域地球科学
收录类别SCI-E
WOS记录号WOS:000393635300004
WOS关键词MINERAL DUST ; NORTH CHINA ; HETEROGENEOUS CHEMISTRY ; TROPOSPHERIC CHEMISTRY ; SULFUR-DIOXIDE ; HONO SOURCES ; ACE-ASIA ; AEROSOL ; EMISSION ; STORM
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/38050
专题地球科学
作者单位1.IAP, LAPC, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China;
2.Chinese Acad Sci, Beijing 100029, Peoples R China;
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China;
4.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Urban Atmospher Environm, Xiamen, Peoples R China;
5.Russian Acad Sci, AM Obukhov Inst Atmospher Phys, Lab Atmospher Gas Species, Moscow 119017, Russia
推荐引用方式
GB/T 7714
Chen, Lei,Zhang, Meigen,Zhu, Jia,et al. Model analysis of soil dust impacts on the boundary layer meteorology and air quality over East Asia in April 2015[J]. ATMOSPHERIC RESEARCH,2017,187.
APA Chen, Lei,Zhang, Meigen,Zhu, Jia,&Skorokhod, Andrei.(2017).Model analysis of soil dust impacts on the boundary layer meteorology and air quality over East Asia in April 2015.ATMOSPHERIC RESEARCH,187.
MLA Chen, Lei,et al."Model analysis of soil dust impacts on the boundary layer meteorology and air quality over East Asia in April 2015".ATMOSPHERIC RESEARCH 187(2017).
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