Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1016/j.atmosres.2018.08.011 |
Carbonaceous components and major ions in PM10 from the Amazonian Basin | |
Custodio, Danilo1,2,3; Alves, Celia2; Jomolca, Yendry1; Vasconcellos, Perola de Castro1 | |
2019 | |
发表期刊 | ATMOSPHERIC RESEARCH
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ISSN | 0169-8095 |
EISSN | 1873-2895 |
出版年 | 2019 |
卷号 | 215页码:75-84 |
文章类型 | Article |
语种 | 英语 |
国家 | Brazil; Portugal; Germany |
英文摘要 | Air pollution mainly resulting from deforestation and agricultural activities has become one of the major concerns in the Amazonian Basin. A detailed analysis of the PM15 chemical composition is critical for devising pollution control measures and improving climate models. In this study, daily 24-h filter samples were collected and analyzed in different sites of the Amazon Basin between 2008 and 2016 (over 200 samples). The six sampling sites were classified into two groups, one in South Amazonia, a region with strong influence of land occupation, and another in a remote forest region to the North. The high mean concentrations of PM10 and the occurrences of extreme events at the Southern site denote air pollution episodes. High correlations between the temporal trends of PM10 and primary species linked to soil re -suspension and biomass burning highlight the contribution of these sources of air pollution in the region. Significant differences between PM10 in the South and North regions were observed, for which levels of 72.6 +/- 66.5 mu g m(-3) and 8.9 4.2 mu g m(-3), respectively. The average concentrations of organic carbon (OC) and elemental carbon (EC) in the aerosol were 5,81 +/- 4.18 lig m(-3), 2.43 +/- 1.65 pg m-(3) and 5.17 +/- 5.54 ng m(-3), 0.51 +/- 0.41 pig m(-3), respectively, for the Southern and Northern Amazonia sampling sites. The aerosol was largely composed of inorganic species in Southern Amazonia, whose carbonaceous matter accounted for 16% of the gravimetrically measured PM10. However, in the forest region, the contribution of carbonaceous species, mainly OC, accounted for > 90% and remained more constant throughout the seasons. Na+ was the dominant water soluble ion in samples from the Southern region, followed by SO4-2, NO3-, Ca2+ and K+. High levels of carbonate (CC) were also observed for these samples. For the Northern region, SO4-2 was the dominant soluble ion, followed by K+ and NH4+. Some of these species exhibited a clear seasonal trend during the study period. This study provides a better understanding of the current state of air pollution in diversified Amazon basin sites. |
英文关键词 | Amazon air pollution Amazonia aerosol Aerosol composition Air quality Atmospheric chemistry |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000447575100006 |
WOS关键词 | SUSPENDED PARTICULATE MATTER ; ATMOSPHERIC AEROSOLS ; CHEMICAL-COMPOSITION ; SOURCE APPORTIONMENT ; BIOMASS ; URBAN ; PARTICLES ; EMISSIONS ; PM2.5 ; DUST |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/37944 |
专题 | 地球科学 |
作者单位 | 1.Univ Sao Paulo, Inst Chem, BR-05508000 Sao Paulo, Brazil; 2.Univ Aveiro, Dept Environm, Ctr Environm & Marine Studies, P-3810193 Aveiro, Portugal; 3.HZG, Inst Coastal Res, Geesthacht, Germany |
推荐引用方式 GB/T 7714 | Custodio, Danilo,Alves, Celia,Jomolca, Yendry,et al. Carbonaceous components and major ions in PM10 from the Amazonian Basin[J]. ATMOSPHERIC RESEARCH,2019,215:75-84. |
APA | Custodio, Danilo,Alves, Celia,Jomolca, Yendry,&Vasconcellos, Perola de Castro.(2019).Carbonaceous components and major ions in PM10 from the Amazonian Basin.ATMOSPHERIC RESEARCH,215,75-84. |
MLA | Custodio, Danilo,et al."Carbonaceous components and major ions in PM10 from the Amazonian Basin".ATMOSPHERIC RESEARCH 215(2019):75-84. |
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