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DOI | 10.1029/2021GL095623 |
Impact of Formation Pathways on Secondary Inorganic Aerosol during Haze Pollution in Beijing: Quantitative Evidence from High-Resolution Observation and Modeling | |
Jie Gao; Yiming Li; Jiayun Li; Guoliang Shi; Zirui Liu; Bo Han; Xiao Tian; Yuesi Wang; Yinchang Feng; Armistead G. Russell | |
2021-11-19 | |
发表期刊 | Geophysical Research Letters |
出版年 | 2021 |
英文摘要 | Secondary inorganic aerosol (especially SNA: sulfate, nitrate, ammonium) formed from different pathways, account for significant proportions of ambient particulate matter during haze events. For the first time, we quantitatively explored contributions from different SNA formation pathways by an online monitoring AMS instrument and 3-dimension factor analysis PMF3 model, which called “SNA formation pathway apportionment”. Three formation process were identified: NH4NO3 heterogeneous phase reactions (NH4NO3-heter), (NH4)2SO4 gas phase reactions ((NH4)2SO4-gas), and mixed NH4NO3 & (NH4)2SO4 aqueous phase processes (S&N-aque). Their overall contributions to SNA were 25.7%, 22.1%, and 52.2%, respectively. Moreover, (NH4)2SO4-gas contributed mainly in clean (52.1%); S&N-aque got highest contribution in haze episode (69.6%); while sulfate gas phase formations were also found in haze stage (10.3%). The quantitative findings from this work provide hard evidence that aqueous phase processes (including sulfate aqueous phase reactions and nitrate gas-particle partition) were major drivers for SNA increasing. |
领域 | 气候变化 |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/342049 |
专题 | 气候变化 |
推荐引用方式 GB/T 7714 | Jie Gao,Yiming Li,Jiayun Li,et al. Impact of Formation Pathways on Secondary Inorganic Aerosol during Haze Pollution in Beijing: Quantitative Evidence from High-Resolution Observation and Modeling[J]. Geophysical Research Letters,2021. |
APA | Jie Gao.,Yiming Li.,Jiayun Li.,Guoliang Shi.,Zirui Liu.,...&Armistead G. Russell.(2021).Impact of Formation Pathways on Secondary Inorganic Aerosol during Haze Pollution in Beijing: Quantitative Evidence from High-Resolution Observation and Modeling.Geophysical Research Letters. |
MLA | Jie Gao,et al."Impact of Formation Pathways on Secondary Inorganic Aerosol during Haze Pollution in Beijing: Quantitative Evidence from High-Resolution Observation and Modeling".Geophysical Research Letters (2021). |
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