GSTDTAP  > 气候变化
DOI10.1002/2016JD026157
US CH4 emissions from oil and gas production: Have recent large increases been detected?
Bruhwiler, L. M.1; Basu, S.2; Bergamaschi, P.3; Bousquet, P.4; Dlugokencky, E.1; Houweling, S.5,6; Ishizawa, M.7; Kim, H. -S.7; Locatelli, R.4; Maksyutov, S.7; Montzka, S.1; Pandey, S.5,6; Patra, P. K.8; Petron, G.2; Saunois, M.4; Sweeney, C.2; Schwietzke, S.2; Tans, P.1; Weatherhead, E. C.2
2017-04-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2017
卷号122期号:7
文章类型Article
语种英语
国家USA; Italy; France; Netherlands; Japan
英文摘要

Recent studies have proposed significant increases in CH4 emissions possibly from oil and gas (O&G) production, especially for the U.S. where O&G production has reached historically high levels over the past decade. In this study, we show that an ensemble of time-dependent atmospheric inversions constrained by calibrated atmospheric observations of surface CH4 mole fraction, with some including space-based retrievals of column average CH4 mole fractions, suggests that North American CH4 emissions have been flat over years spanning 2000 through 2012. Estimates of emission trends using zonal gradients of column average CH4 calculated relative to an upstream background are not easy to make due to atmospheric variability, relative insensitivity of column average CH4 to surface emissions at regional scales, and fast zonal synoptic transport. In addition, any trends in continental enhancements of column average CH4 are sensitive to how the upstream background is chosen, and model simulations imply that short-term (4years or less) trends in column average CH4 horizontal gradients of up to 1.5ppb/yr can occur just from interannual transport variability acting on a strong latitudinal CH4 gradient. Finally, trends in spatial gradients calculated from space-based column average CH4 can be significantly biased (>2-3ppb/yr) due to the nonuniform and seasonally varying temporal coverage of satellite retrievals.


Plain Language Summary In this paper we address recent claims of significant increases in methane emissions from U.S. oil and gas production. We find that such claims are inconsistent with observations by examining atmospheric inversions and observations from the NOAA aircraft monitoring program. Furthermore, we show how atmospheric variability, sampling biases, and choice of upwind background can lead to spurious trends in atmospheric column average methane when using both in situ and space-based retrievals.


英文关键词methane emissions oil and gas production
领域气候变化
收录类别SCI-E
WOS记录号WOS:000400172000023
WOS关键词AMERICAN METHANE EMISSIONS ; HIGH-SPATIAL-RESOLUTION ; ATMOSPHERIC METHANE ; FOSSIL-FUEL ; MODEL TM5 ; SATELLITE ; BUDGET ; SCIAMACHY ; INVERSION ; ETHANE
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
被引频次:45[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/34018
专题气候变化
作者单位1.NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA;
2.Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA;
3.European Commiss, Joint Res Ctr, Ispra, Italy;
4.IPSL, CNRS, CEA, UVSQ,Lab Sci Climat & Environm, Gif Sur Yvette, France;
5.SRON Netherlands Inst Space Res, Utrecht, Netherlands;
6.Inst Marine & Atmospher Res Utrecht, Utrecht, Netherlands;
7.Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan;
8.Japan Agcy Marine Earth Sci & Technol, Yokohama, Kanagawa, Japan
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GB/T 7714
Bruhwiler, L. M.,Basu, S.,Bergamaschi, P.,et al. US CH4 emissions from oil and gas production: Have recent large increases been detected?[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2017,122(7).
APA Bruhwiler, L. M..,Basu, S..,Bergamaschi, P..,Bousquet, P..,Dlugokencky, E..,...&Weatherhead, E. C..(2017).US CH4 emissions from oil and gas production: Have recent large increases been detected?.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,122(7).
MLA Bruhwiler, L. M.,et al."US CH4 emissions from oil and gas production: Have recent large increases been detected?".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 122.7(2017).
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