GSTDTAP  > 气候变化
DOI10.1029/2018JD029690
Methane Emissions from the Marcellus Shale in Southwestern Pennsylvania and Northern West Virginia Based on Airborne Measurements
Ren, Xinrong1,2,3; Hall, Dolly L.1; Vinciguerra, Timothy4; Benish, Sarah E.1; Stratton, Philip R.1; Ahn, Doyeon5; Hansford, Jonathan R.6; Cohen, Mark D.2; Sahu, Sayantan5; He, Hao1; Grimes, Courtney5; Fuentes, Jose D.7; Shepson, Paul B.8,9,10; Salawitch, Ross J.1,5,11; Ehrman, Sheryl H.4,12; Dickerson, Russell R.1,11
2019-02-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2019
卷号124期号:3页码:1862-1878
文章类型Article
语种英语
国家USA
英文摘要

Natural gas production in the United States has increased rapidly over the past decade, along with concerns about methane (CH4) fugitive emissions and its climate impacts. Quantification of CH4 emissions from oil and natural gas (O&NG) operations is important for establishing scientifically sound policies for mitigating greenhouse gases. We use the aircraft mass balance approach for three flight experiments in August and September 2015 to estimate CH4 emissions from O&NG operations over the southwestern Marcellus Shale. We estimate a mean CH4 emission rate as 21.2 kg/s with 28% coming from O&NG operations. The mean CH4 emission rate from O&NG operations was estimated to be 1.1% of total NG production. The individual best-estimate emission rates from the three flight experiments ranged from 0.78 to 1.5%, with overall limits of 0% and 3.5%. These emission rates are at the low end of other top-down studies, but consistent with the few observational studies in the Marcellus Shale region as well as the U.S. Environmental Protection Agency CH4 inventory. A substantial source of CH4 (similar to 70% of observed CH4 emissions) was found to contain little ethane, possibly due to coalbed CH4 emitted either directly from coal mines or from wells drilled through coalbed layers in O&NG operations. Recent regulations requiring capture of gas from the completion-venting step of hydraulic fracturing appear to have reduced the atmospheric release of CH4. Our study suggests that for a 20-year time scale, energy derived from the combustion of natural gas extracted from this region likely exerts a net climate benefit compared to coal.


Plain Language Summary In this study methane (CH4) emission rates were estimated for the southwest Marcellus Shale based on airborne observations. A mean emission rate of similar to 21 kg CH4/s was observed from a 4,200-km(2) study area. A significant portion (similar to similar to 70%) of the emitted CH4 was found to originate likely from coalbeds. Our mean estimated emission rate of 1.1% of total natural gas production indicates a climate benefit of natural gas combustion compared to coal, but the full range includes values above the 2.4% break-even point for the CH4 global warming potential over a 20-year time horizon.


英文关键词methane emission Marcellus oil and natural gas leak rate
领域气候变化
收录类别SCI-E
WOS记录号WOS:000459377000038
WOS关键词NATURAL-GAS PRODUCTION ; VOLATILE ORGANIC-COMPOUNDS ; PRODUCTION SITES ; UNITED-STATES ; ATMOSPHERIC METHANE ; PROCESS EQUIPMENT ; PIPELINE LEAKS ; AIR-POLLUTANTS ; OIL ; OPERATIONS
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/33748
专题气候变化
作者单位1.Univ Maryland, Dept Atmospher & Ocean Sci, College Pk, MD 20742 USA;
2.NOAA, Air Resources Lab, College Pk, MD 20740 USA;
3.Univ Maryland, Cooperat Inst Climate & Satellites, College Pk, MD 20742 USA;
4.Univ Maryland, Dept Chem & Biomol Engn, College Pk, MD 20742 USA;
5.Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA;
6.Univ Maryland, Dept Comp Sci, College Pk, MD 20742 USA;
7.Penn State Univ, Dept Meteorol & Atmospher Sci, University Pk, PA 16802 USA;
8.Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA;
9.Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA;
10.SUNY Stony Brook, Sch Marine & Atmospher Sci, Stony Brook, NY 11794 USA;
11.Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA;
12.San Jose State Univ, Charles W Davidson Coll Engn, San Jose, CA 95192 USA
推荐引用方式
GB/T 7714
Ren, Xinrong,Hall, Dolly L.,Vinciguerra, Timothy,et al. Methane Emissions from the Marcellus Shale in Southwestern Pennsylvania and Northern West Virginia Based on Airborne Measurements[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2019,124(3):1862-1878.
APA Ren, Xinrong.,Hall, Dolly L..,Vinciguerra, Timothy.,Benish, Sarah E..,Stratton, Philip R..,...&Dickerson, Russell R..(2019).Methane Emissions from the Marcellus Shale in Southwestern Pennsylvania and Northern West Virginia Based on Airborne Measurements.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,124(3),1862-1878.
MLA Ren, Xinrong,et al."Methane Emissions from the Marcellus Shale in Southwestern Pennsylvania and Northern West Virginia Based on Airborne Measurements".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 124.3(2019):1862-1878.
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