Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1029/2018JD028527 |
Molecular Characterization and Seasonal Variation in Primary and Secondary Organic Aerosols in Beijing, China | |
Li, Linjie1,2,3; Ren, Lujie2; Ren, Hong1,2,3; Yue, Siyao1,3; Xie, Qiaorong1,3; Zhao, Wanyu1,3; Kang, Mingjie1; Li, Jie1; Wang, Zifa1,3; Sun, Yele1,3; Fu, Pingqing2,3 | |
2018-11-16 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2018 |
卷号 | 123期号:21页码:12394-12412 |
文章类型 | Article |
语种 | 英语 |
国家 | Peoples R China |
英文摘要 | Biomass burning (BB) aerosols, primary biological aerosol particles, and secondary organic aerosols, are critical components of particulate matter in the atmosphere. In this study, saccharides, lignin/resin acids, biogenic secondary organic aerosols tracers, aromatic acids, and hydroxyacids/polyacids were measured in total suspended particles collected from April 2012 to March 2013 at an urban site in Beijing using gas chromatography/mass spectrometry. The concentration of levoglucosan was elevated during 18-20 June. The high ratio of levoglucosan to mannosan and low ratio of galactosan to mannosan in June demonstrated the influence of wheat straw combustion in the North China Plain via long-rang transport. Sucrose, glucose, and fructose were more abundant in April, the spring bloom season. The maximum trehalose content (298 ng/m(3)) occurred during a dust storm (27-29 April) with the highest stable carbon isotope ratio (delta C-13, -21.2 parts per thousand) of total carbon. Fungal spore tracers (arabitol and mannitol) peaked in summer. The largest concentrations of the oxidization products of isoprene and alpha/beta-pinene also occurred in summer. However, the beta-caryophyllene tracer was much more abundant on long-lasting haze days in winter and was positively related to levoglucosan. The contributions of biogenic primary sources (plant debris, fungal spores, and BB) to organic carbon were estimated to be in range of 2.64-35.2% (11.8%), with BB being the predominant source. Biogenic secondary sources (isoprene, alpha-pinene, and beta-caryophyllene) and anthropogenic secondary source (naphthalene) accounted for 0.23-10.9% (3.36%) of organic carbon with large contributions in summer and winter, respectively. |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000452001400035 |
WOS关键词 | WESTERN NORTH PACIFIC ; ATMOSPHERIC PARTICULATE MATTER ; BIOMASS BURNING CONTRIBUTION ; CARBON ISOTOPIC COMPOSITION ; FINE-PARTICLE EMISSIONS ; REMOTE MARINE AEROSOLS ; CHEMICAL-CHARACTERIZATION ; DICARBOXYLIC-ACIDS ; FUNGAL SPORES ; ASIAN DUST |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/32635 |
专题 | 气候变化 |
作者单位 | 1.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China; 2.Tianjin Univ, Inst Surface Earth Syst Sci, Tianjin, Peoples R China; 3.Univ Chinese Acad Sci, Coll Earth & Planetary Sci, Beijing, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Linjie,Ren, Lujie,Ren, Hong,et al. Molecular Characterization and Seasonal Variation in Primary and Secondary Organic Aerosols in Beijing, China[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(21):12394-12412. |
APA | Li, Linjie.,Ren, Lujie.,Ren, Hong.,Yue, Siyao.,Xie, Qiaorong.,...&Fu, Pingqing.(2018).Molecular Characterization and Seasonal Variation in Primary and Secondary Organic Aerosols in Beijing, China.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(21),12394-12412. |
MLA | Li, Linjie,et al."Molecular Characterization and Seasonal Variation in Primary and Secondary Organic Aerosols in Beijing, China".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.21(2018):12394-12412. |
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