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DOI10.1029/2017JD028112
Using an Inverse Model to Reconcile Differences in Simulated and Observed Global Ethane Concentrations and Trends Between 2008 and 2014
Monks, S. A.1,2; Wilson, C.3,4; Emmons, L. K.5; Hannigan, J. W.5; Helmig, D.6; Blake, N. J.7; Blake, D. R.7
2018-10-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2018
卷号123期号:19页码:11262-11282
文章类型Article
语种英语
国家USA; England
英文摘要

We use a global model, TOMCAT, and an inverse model, INVICAT, to estimate emissions of ethane (C2H6) between 2008 and 2014 by assimilating surface flask observations. We find that baseline global emissions in 2008 need to increase by a factor of 2.04-2.11 in order for the model to capture C2H6 observations, indicating large biases in current emission inventories. Most of this increase occurs over North America and Eurasia, with temperate North American emissions accounting for 23-26% of the total global emission increase and temperate Eurasian emissions accounting for 35-37%. Further to this, recent peer-reviewed analysis of long-term observational records shows an increase in C2H6 in the Northern Hemisphere since similar to 2009. Our results indicate that annual global emissions of C2H6 have increased at a rate of 0.27 +/- 0.54-0.33 +/- 0.44 Tg/yr(2) between 2008 and 2014. A statistically significant positive trend of 0.20 +/- 0.11-0.24 +/- 0.13 Tg/yr(2) (p <= 0.01) is found in temperate North America, resulting in emissions that are 31-32% larger in 2014 than in 2008. Our results corroborate previous studies' conclusions that a rapid increase in oil and natural gas production in United States over this time period is likely a large driver of the change in emissions.


领域气候变化
收录类别SCI-E
WOS记录号WOS:000448374800028
WOS关键词VOLATILE ORGANIC-COMPOUNDS ; CHEMICAL-TRANSPORT MODEL ; NATURAL-GAS PRODUCTION ; METHANE EMISSIONS ; ATMOSPHERIC METHANE ; AIR-QUALITY ; NONMETHANE HYDROCARBONS ; SATELLITE-OBSERVATIONS ; FIELD CAMPAIGN ; CLIMATE-CHANGE
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/32521
专题气候变化
作者单位1.Univ Colorado, CIRES, Boulder, CO 80309 USA;
2.NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USA;
3.Univ Leeds, Natl Ctr Earth Observat, Leeds, W Yorkshire, England;
4.Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England;
5.Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA;
6.Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA;
7.Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA
推荐引用方式
GB/T 7714
Monks, S. A.,Wilson, C.,Emmons, L. K.,et al. Using an Inverse Model to Reconcile Differences in Simulated and Observed Global Ethane Concentrations and Trends Between 2008 and 2014[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(19):11262-11282.
APA Monks, S. A..,Wilson, C..,Emmons, L. K..,Hannigan, J. W..,Helmig, D..,...&Blake, D. R..(2018).Using an Inverse Model to Reconcile Differences in Simulated and Observed Global Ethane Concentrations and Trends Between 2008 and 2014.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(19),11262-11282.
MLA Monks, S. A.,et al."Using an Inverse Model to Reconcile Differences in Simulated and Observed Global Ethane Concentrations and Trends Between 2008 and 2014".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.19(2018):11262-11282.
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