Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1029/2018JD028836 |
Large Increases in Primary Trimethylaminium and Secondary Dimethylaminium in Atmospheric Particles Associated With Cyclonic Eddies in the Northwest Pacific Ocean | |
Hu, Qingjing1; Qu, Keming1; Gao, Huiwang2,3; Cui, Zhengguo1; Gao, Yang2,3; Yao, Xiaohong2,3 | |
2018-11-16 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2018 |
卷号 | 123期号:21页码:12133-12146 |
文章类型 | Article |
语种 | 英语 |
国家 | Peoples R China |
英文摘要 | Dimethylaminium (DMA(+)) and trimethylaminium (TMA(+)) ions in size-segregated atmospheric particles are measured across the marginal seas of China and the northwest Pacific Ocean (NWPO) in March-May 2014. The concentrations of DMA(+) and TMA(+) in particles with diameters of 0.056-10 mu m (PM0.056-10) collected from the eutrophic seas are 0.22 +/- 0.38 nmol/m(3) and 0.11 +/- 0.23 nmol/m(3), respectively. Surprisingly, an average TMA(+) concentration that is 1 order of magnitude higher and a slightly higher average DMA(+) concentration are observed across the oligotrophic NWPO. However, the concentrations of chlorophyll-a in the NWPO are approximately 5 times lower than those in the marginal seas. The maximum concentrations of TMA(+) (4.39 nmol/m(3)) and DMA(+) (0.92 nmol/m(3)) in PM0.056-10 are observed close to the largest cyclonic eddy in the NWPO under an average wind speed of 14 m/s. The concentrations of TMA(+) increase with decreasing particle size in the sample, whereas those of DMA(+) exhibit a condensation mode at 0.2 mu m and a droplet mode at 1-2 mu m. The bimodal size distribution of DMA(+) is conventionally interpreted in terms of secondary reactions in the atmosphere. The unique size distribution of TMA(+) suggests that it very likely originates from sea-spray aerosols. Based on their size distributions in other samples collected over the NWPO, these conclusions may generally apply for TMA(+) and DMA(+). Moreover, we propose a novel conceptual model to explain how the largely increased primary TMA(+) and secondary DMA(+) are linked to emissions of sea-spray aerosols and gaseous precursors from various cyclonic eddies. |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000452001400021 |
WOS关键词 | SIZE DISTRIBUTION ; METHANESULFONIC-ACID ; MASS-SPECTROMETRY ; GLYCINE BETAINE ; AMBIENT AEROSOL ; SULFURIC-ACID ; N-OXIDE ; MARINE ; AMINES ; NITROGEN |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/32278 |
专题 | 气候变化 |
作者单位 | 1.Chinese Acad Fishery Sci, Minist Agr & Rural Affairs, Yellow Sea Fisheries Res Inst, Key Lab Sustainable Utilizat Marine Fisheries Res, Qingdao, Peoples R China; 2.Ocean Univ China, Key Lab Marine Environm Sci & Ecol, Qingdao, Peoples R China; 3.Pilot Natl Lab Marine Sci & Technol Qingdao, Qingdao, Peoples R China |
推荐引用方式 GB/T 7714 | Hu, Qingjing,Qu, Keming,Gao, Huiwang,et al. Large Increases in Primary Trimethylaminium and Secondary Dimethylaminium in Atmospheric Particles Associated With Cyclonic Eddies in the Northwest Pacific Ocean[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(21):12133-12146. |
APA | Hu, Qingjing,Qu, Keming,Gao, Huiwang,Cui, Zhengguo,Gao, Yang,&Yao, Xiaohong.(2018).Large Increases in Primary Trimethylaminium and Secondary Dimethylaminium in Atmospheric Particles Associated With Cyclonic Eddies in the Northwest Pacific Ocean.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(21),12133-12146. |
MLA | Hu, Qingjing,et al."Large Increases in Primary Trimethylaminium and Secondary Dimethylaminium in Atmospheric Particles Associated With Cyclonic Eddies in the Northwest Pacific Ocean".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.21(2018):12133-12146. |
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