Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1002/2016JD025663 |
Remote sensing evidence of decadal changes in major tropospheric ozone precursors over East Asia | |
Souri, Amir Hossein1; Choi, Yunsoo1; Jeon, Wonbae1; Woo, Jung-Hun2; Zhang, Qiang3; Kurokawa, Jun-ichi4 | |
2017-02-27 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2017 |
卷号 | 122期号:4 |
文章类型 | Article |
语种 | 英语 |
国家 | USA; South Korea; Peoples R China; Japan |
英文摘要 | Recent regulatory policies in East Asia reduce ozone precursors, but these changes are spatially and temporally nonuniform. This study investigates variations in the long-term trends of tropospheric NO2, HCHO, and HCHO/NO2 ratios to diagnose ozone sensitivity to changes in NOx and volatile organic compound using the Ozone Monitoring Instrument (OMI). Using an adaptive-degree polynomial filter, we identify extremums of time series of NO2 to determine when and how NO2 change. Due to the regulations in China, trends which were predominantly upward turned downward. The years undergoing these changes primarily happened in 2011 and 2012. OMI column densities, however, suggest that NOx sources in South Korea, the Pearl River Delta (PRD), Taiwan, and Japan have not consistently decreased. Specifically, as Chinese exports of NO2 started subsiding, increasing trends in NO2 columns over several Korean cities, including Seoul, become evident. To quantify the changes in NOx emissions from summertime 2010 to 2014, we conduct a 3D-Var inverse modeling using a regional model with MIX-Asia inventory and estimate NOx emissions (in 2010 and 2014) for the PRD (1.6 and 1.5 Gg/d), the Yangtze River Delta (3.9 and 3.0 Gg/d), north China (15.6 and 14.3 Gg/d), South Korea (1.6 and 1.5 Gg/d), and Japan (2.7 and 2.6 Gg/d). OMI HCHO shows upward trends in East Asia resulting from anthropogenic effects; however, the magnitudes are negative in the PRD, Japan, North Korea, and Taiwan. OMI HCHO/NO2 ratios reveal that while South Korea, Japan, and the south of China have undergone toward more NOx-sensitive regime, areas around the Bohai Sea have become more NOx saturated. |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000396121200026 |
WOS关键词 | PEARL RIVER DELTA ; SURFACE OZONE ; EMISSION INVENTORY ; ISOPRENE EMISSIONS ; NITROGEN-DIOXIDE ; OMI OBSERVATIONS ; NOX EMISSIONS ; SATELLITE ; SENSITIVITY ; CHINA |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/32268 |
专题 | 气候变化 |
作者单位 | 1.Univ Houston, Dept Earth & Atmospher Sci, Houston, TX 77004 USA; 2.Konkuk Univ, Dept Adv Technol Fus, Seoul, South Korea; 3.Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing, Peoples R China; 4.Asia Ctr Air Pollut Res, Niigata, Japan |
推荐引用方式 GB/T 7714 | Souri, Amir Hossein,Choi, Yunsoo,Jeon, Wonbae,et al. Remote sensing evidence of decadal changes in major tropospheric ozone precursors over East Asia[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2017,122(4). |
APA | Souri, Amir Hossein,Choi, Yunsoo,Jeon, Wonbae,Woo, Jung-Hun,Zhang, Qiang,&Kurokawa, Jun-ichi.(2017).Remote sensing evidence of decadal changes in major tropospheric ozone precursors over East Asia.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,122(4). |
MLA | Souri, Amir Hossein,et al."Remote sensing evidence of decadal changes in major tropospheric ozone precursors over East Asia".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 122.4(2017). |
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