GSTDTAP  > 地球科学
DOI10.5194/acp-17-7175-2017
Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study
Caponi, Lorenzo1,2,3,4; Formenti, Paola1,2; Massabo, Dario3,4; Di Biagio, Claudia1,2; Cazaunau, Mathieu1,2; Pangui, Edouard1,2; Chevaillier, Servanne1,2; Landrot, Gautier5; Andreae, Meinrat O.6,13; Kandler, Konrad7; Piketh, Stuart8; Saeed, Thuraya9; Seibert, Dave10; Williams, Earle11; Balkanski, Yves12; Prati, Paolo3,4; Doussin, Jean-Francois1,2
2017-06-16
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2017
卷号17期号:11
文章类型Article
语种英语
国家France; Italy; Germany; South Africa; Kuwait; USA; Saudi Arabia
英文摘要

This paper presents new laboratory measurements of the mass absorption efficiency (MAE) between 375 and 850 nm for 12 individual samples of mineral dust from different source areas worldwide and in two size classes: PM10 : 6 (mass fraction of particles of aerodynamic diameter lower than 10.6 mu m) and PM2 : 5 (mass fraction of particles of aerodynamic diameter lower than 2.5 mu m). The experiments were performed in the CESAM simulation chamber using mineral dust generated from natural parent soils and included optical and gravimetric analyses.


The results show that the MAE values are lower for the PM10.6 mass fraction (range 37-135 x 10(3) m(2) g(-1) at 375 nm) than for the PM2.5 (range 95-711 x 10(3) m(2) g(-1) at 375 nm) and decrease with increasing wavelength as lambda(-AAE), where the Angstrom absorption exponent (AAE) averages between 3.3 and 3.5, regardless of size. The size independence of AAE suggests that, for a given size distribution, the absorption properties and elemental iron rather than the iron oxide fraction, which could ease the application and the validation of climate models that now start to include the representation of the dust composition, as well as for remote sensing of dust absorption in the UV-vis spectral region.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000403779200002
WOS关键词COMPLEX REFRACTIVE-INDEXES ; IN-SITU MEASUREMENTS ; OPTICAL-PROPERTIES ; SAHARAN DUST ; LIGHT-ABSORPTION ; BROWN CARBON ; CHEMICAL-COMPOSITION ; BLACK CARBON ; RADIATIVE PROPERTIES ; IRON-OXIDES
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/30935
专题地球科学
作者单位1.Univ Paris Est Creteil, UMR CNRS 7583, LISA, Creteil, France;
2.Univ Paris Diderot, Inst Pierre Simon Laplace, Creteil, France;
3.Univ Genoa, Dept Phys, Genoa, Italy;
4.Univ Genoa, INFN, Genoa, Italy;
5.Synchrotron SOLEIL, Lorme Des Merisiers St A, France;
6.Max Planck Inst Chem, Biogeochem Dept, POB 3060, D-55020 Mainz, Germany;
7.Tech Univ Darmstadt, Inst Angew Geowissensch, Schnittspahnstr 9, D-64287 Darmstadt, Germany;
8.Univ Witwatersrand, Climatol Res Grp, Johannesburg, South Africa;
9.Publ Author Appl Educ & Training, Coll Basic Educ, Sci Dept, Al Ardiya, Kuwait;
10.Sallyport Global, Phoenix, AZ USA;
11.MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA;
12.Univ Versailles St Quentin, CEA, CNRS UMR8212, LSCE, Gif Sur Yvette, France;
13.King Saud Univ, Geol & Geophys Dept, Riyadh, Saudi Arabia
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GB/T 7714
Caponi, Lorenzo,Formenti, Paola,Massabo, Dario,et al. Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(11).
APA Caponi, Lorenzo.,Formenti, Paola.,Massabo, Dario.,Di Biagio, Claudia.,Cazaunau, Mathieu.,...&Doussin, Jean-Francois.(2017).Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(11).
MLA Caponi, Lorenzo,et al."Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.11(2017).
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