Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-19-3747-2019 |
Effects of two different biogenic emission models on modelled ozone and aerosol concentrations in Europe | |
Jiang, Jianhui1; 39;Dowd, Colin2 | |
2019-03-22 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2019 |
卷号 | 19期号:6页码:3747-3768 |
文章类型 | Article |
语种 | 英语 |
国家 | Switzerland; France; Ireland; Spain; USA |
英文摘要 | Biogenic volatile organic compound (BVOC) emissions are one of the essential inputs for chemical transport models (CTMs), but their estimates are associated with large uncertainties, leading to significant influence on air quality modelling. This study aims to investigate the effects of using different BVOC emission models on the performance of a CTM in simulating secondary pollutants, i.e. ozone, organic, and inorganic aerosols. European air quality was simulated for the year 2011 by the regional air quality model Comprehensive Air Quality Model with Extensions (CAMx) version 6.3, using BVOC emissions calculated by two emission models: the Paul Scherrer Institute (PSI) model and the Model of Emissions of Gases and Aerosol from Nature (MEGAN) version 2.1. Comparison of isoprene and monoterpene emissions from both models showed large differences in their general amounts, as well as their spatial distribution in both summer and winter. MEGAN produced more isoprene emissions by a factor of 3 while the PSI model generated 3 times the monoterpene emissions in summer, while there was negligible difference (similar to 4 %) in sesquiterpene emissions associated with the two models. Despite the large differences in isoprene emissions (i.e. 3-fold), the resulting impact in predicted summertime ozone proved to be minor (<10 %; MEGAN O-3 was higher than PSI O-3 by similar to 7 ppb). Comparisons with measurements from the Euro concentrations but worsen performance at high ozone levels (>60 ppb). A much larger effect of the different BVOC emissions was found for the secondary organic aerosol (SOA) concentrations. The higher monoterpene emissions (a factor of similar to 3) by the PSI model led to higher SOA by similar to 110% on average in summer, compared to MEGAN, and lead to better agreement between modelled and measured organic aerosol (OA): the mean bias between modelled and measured OA at nine measurement stations using Aerodyne aerosol chemical speciation monitors (ACSMs) or Aerodyne aerosol mass spectrometers (AMSs) was reduced by 21%-83% at rural or remote stations. Effects on inorganic aerosols (particulate nitrate, sulfate, and ammonia) were relatively small (<15 %). |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000462073500004 |
WOS关键词 | VOLATILE ORGANIC-COMPOUNDS ; AIR-QUALITY ; SOURCE APPORTIONMENT ; VOC EMISSIONS ; ISOPRENOID EMISSIONS ; PRECURSOR EMISSIONS ; PARTICULATE MATTER ; COMPOUND EMISSIONS ; SUBMICRON AEROSOLS ; BOREAL FOREST |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/30741 |
专题 | 地球科学 |
作者单位 | 1.Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland; 2.Univ Paris Est Creteil, LISA, UMR CNRS 7583, Creteil, France; 3.Univ Paris Diderot, Inst Pierre Simon Laplace, Creteil, France; 4.Natl Univ Ireland Galway, Sch Phys, Ryan Inst Ctr Climate & Air Pollut Studies, Univ Rd, Galway H91 CF50, Ireland; 5.Natl Univ Ireland Galway, Marine Renewable Energy Ireland, Univ Rd, Galway H91 CF50, Ireland; 6.CSIC, Inst Environm Assessment & Water Res IDAEA, ES-08034 Barcelona, Spain; 7.Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA |
推荐引用方式 GB/T 7714 | Jiang, Jianhui,39;Dowd, Colin. Effects of two different biogenic emission models on modelled ozone and aerosol concentrations in Europe[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(6):3747-3768. |
APA | Jiang, Jianhui,&39;Dowd, Colin.(2019).Effects of two different biogenic emission models on modelled ozone and aerosol concentrations in Europe.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(6),3747-3768. |
MLA | Jiang, Jianhui,et al."Effects of two different biogenic emission models on modelled ozone and aerosol concentrations in Europe".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.6(2019):3747-3768. |
条目包含的文件 | 条目无相关文件。 |
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