资源环境科技发展态势分析平台

We apply the Global Modeling Initiative (GMI) chemistry and transport model driven by NASA's MERRA assimilated meteorological data to simulate the seasonal variations in two radionuclide aerosol tracers (terrigenous Pb-210 and cosmogenic Be-7) at the WMO-GAW station of Mt. Cimone (44 degrees 12'N, 10 degrees 42'E; 2165 m a.s.l.; Italy), which is representative of free-tropospheric conditions most of the year, during 2005 with an aim to understand the roles of transport and precipitation scavenging processes in controlling their seasonality. The total precipitation field in the MERRA data set is evaluated with the Global Precipitation Climatology Project (GPCP) observations, and generally good agreement is found. The model reproduces reasonably the observed seasonal pattern of Pb-210 concentrations, characterized by a wintertime minimum due to lower Rn-222 emissions and weaker uplift from the boundary layer and summertime maxima resulting from strong convection over the continent. The observed seasonal behavior of Be-7 concentrations shows a winter minimum, a summer maximum, and a secondary spring maximum. The model captures the observed Be-7 pattern in winter-spring, which is linked to the larger stratospheric influence during spring. However, the model tends to underestimate the observed Be-7 concentrations in summer, partially due to the sensitivity to spatial sampling in the model. Model sensitivity experiments indicate a dominant role of precipitation scavenging (vs. dry deposition and convection) in controlling the seasonality of Pb-210 and Be-7 concentrations at Mt. Cimone.