Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-18-15145-2018 |
Quantifying uncertainties from mobile-laboratory-derived emissions of well pads using inverse Gaussian methods | |
Caulton, Dana R.1; Li, Qi2; Bou-Zeid, Elie1; Fitts, Jeffrey P.1; Golston, Levi M.1; Pan, Da1; Lu, Jessica1; Lane, Haley M.1; Buchholz, Bernhard3; Guo, Xuehui1; McSpiritt, James1; Wendt, Lars4; Zondlo, Mark A.1 | |
2018-10-22 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
![]() |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2018 |
卷号 | 18期号:20页码:15145-15168 |
文章类型 | Article |
语种 | 英语 |
国家 | USA; Germany |
英文摘要 | Mobile laboratory measurements provide information on the distribution of CH4 emissions from point sources such as oil and gas wells, but uncertainties are poorly constrained or justified. Sources of uncertainty and bias in ground-based Gaussian-derived emissions estimates from a mobile platform were analyzed in a combined field and modeling study. In a field campaign where 1009 natural gas sites in Pennsylvania were sampled, a hierarchical measurement strategy was implemented with increasing complexity. Of these sites, similar to 93% were sampled with an average of 2 transects in < 5 min (standard sampling), similar to 5% were sampled with an average of 10 transects in < 15 min (replicate sampling) and similar to 2% were sampled with an average of 20 transects in 15-60 min. For sites sampled with 20 transects, a tower was simultaneously deployed to measure high-frequency meteorological data (intensive sampling). Five of the intensive sampling sites were modeled using large eddy simulation (LES) to reproduce CH4 concentrations in a turbulent environment. The LES output and LES-derived emission estimates were used to compare with the results of a standard Gaussian approach. The LES and Gaussian-derived emission rates agreed within a factor of 2 in all except one case; the average difference was 25 %. A controlled release was also used to investigate sources of bias in either technique. The Gaussian method agreed with the release rate more closely than the LES, underlining the importance of inputs as sources of uncertainty for the LES. The LES was also used as a virtual experiment to determine an optimum number of repeat transects and spacing needed to produce representative statistics. Approximately 10 repeat transects spaced at least 1 min apart are required to produce statistics similar to the observed variability over the entire LES simulation period of 30 min. Sources of uncertainty from source location, wind speed, background concentration and atmospheric stability were also analyzed. The largest contribution to the total uncertainty was from atmospheric variability; this is caused by insufficient averaging of turbulent variables in the atmosphere (also known as random errors). Atmospheric variability was quantified by repeat measurements at individual sites under relatively constant conditions. Accurate quantification of atmospheric variability provides a reasonable estimate of the lower bound for emission uncertainty. The uncertainty bounds calculated for this work for sites with > 50 ppb enhancements were 0.05-6.5q (where q is the emission rate) for single-transect sites and 0.5-2.7q for sites with 10+ transects. More transects allow a mean emission rate to be calculated with better precision. It is recommended that future mobile monitoring schemes quantify atmospheric variability, and attempt to minimize it, under representative conditions to accurately estimate emission uncertainty. These recommendations are general to mobile-laboratory-derived emissions from other sources that can be treated as point sources. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000447837100002 |
WOS关键词 | LARGE-EDDY SIMULATION ; NATURAL-GAS PRODUCTION ; ATMOSPHERIC SURFACE-LAYER ; FUGITIVE METHANE EMISSIONS ; MONIN-OBUKHOV SIMILARITY ; NUMBER BOUNDARY-LAYER ; BARNETT SHALE REGION ; UNITED-STATES ; PRODUCTION SITES ; ANTHROPOGENIC EMISSIONS |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/30526 |
专题 | 地球科学 |
作者单位 | 1.Princeton Univ, Dept Civil & Environm Engn, 59 Olden St, Princeton, NJ 08540 USA; 2.Columbia Univ, Dept Earth & Environm Engn, 500 W 120th St, New York, NY 10027 USA; 3.Tech Univ Darmstadt, RMS, D-64287 Darmstadt, Germany; 4.Hunterdon Cent Reg High Sch, Flemington, NJ 08822 USA |
推荐引用方式 GB/T 7714 | Caulton, Dana R.,Li, Qi,Bou-Zeid, Elie,et al. Quantifying uncertainties from mobile-laboratory-derived emissions of well pads using inverse Gaussian methods[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(20):15145-15168. |
APA | Caulton, Dana R..,Li, Qi.,Bou-Zeid, Elie.,Fitts, Jeffrey P..,Golston, Levi M..,...&Zondlo, Mark A..(2018).Quantifying uncertainties from mobile-laboratory-derived emissions of well pads using inverse Gaussian methods.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(20),15145-15168. |
MLA | Caulton, Dana R.,et al."Quantifying uncertainties from mobile-laboratory-derived emissions of well pads using inverse Gaussian methods".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.20(2018):15145-15168. |
条目包含的文件 | 条目无相关文件。 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论