Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-18-7691-2018 |
Particle and VOC emission factor measurements for anthropogenic sources in West Africa | |
Keita, Sekou1; 39;Datchoh, E. Toure2 | |
2018-06-01 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2018 |
卷号 | 18期号:10页码:7691-7708 |
文章类型 | Article |
语种 | 英语 |
国家 | Cote Ivoire; France; England; Benin |
英文摘要 | A number of campaigns have been carried out to establish the emission factors of pollutants from fuel combustion in West Africa, as part of work package 2 ("Air Pollution and Health") of the DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa) FP7 program. Emission sources considered here include wood (hevea and iroko) and charcoal burning, charcoal making, open trash burning, and vehicle emissions, including trucks, cars, buses and two-wheeled vehicles. Emission factors of total particulate matter (TPM), elemental carbon (EC), primary organic carbon (OC) and volatile organic compounds (VOCs) have been established. In addition, emission factor measurements were performed in combustion chambers in order to reproduce field burning conditions for a tropical hardwood (hevea), and obtain particulate emission factors by size (PM0.25, PM1, PM2.5 and PM10). Particle samples were collected on quartz fiber filters and analyzed using gravimetric method for TPM and thermal methods for EC and OC. The emission factors of 58 VOC species were determined using offline sampling on a sorbent tube. Emission factor results for two species of tropical hardwood burning of EC, OC and TPM are 0.98 +/- 0.46 g kg(-1) of fuel burned (g kg(-1)), 11.05 +/- 4.55 and 41.12 +/- 24.62 g kg(-1), respectively. For traffic sources, the highest emission factors among particulate species are found for the two-wheeled vehicles with two-stroke engines (2.74 g kg(-1) fuel for EC, 65.11 g kg(-1) fuel for OC and 496 g kg(-1) fuel for TPM). The largest VOC emissions are observed for two-stroke two-wheeled vehicles, which are up to 3 times higher than emissions from light-duty and heavy-duty vehicles. Isoprene and monoterpenes, which are usually associated with biogenic emissions, are present in almost all anthropogenic sources investigated during this work and could be as significant as aromatic emissions in wood burning (1 g kg(-1) fuel). EC is primarily emitted in the ultrafine fraction, with 77% of the total mass being emitted as particles smaller than 0.25 mu m. The particles and VOC emission factors obtained in this study are generally higher than those in the literature whose values are discussed in this paper. This study underlines the important role of in situ measurements in deriving realistic and representative emission factors. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000433963400006 |
WOS关键词 | VOLATILE ORGANIC-COMPOUNDS ; PARTICULATE MATTER ; BLACK CARBON ; MOTOR-VEHICLES ; FINE-PARTICLE ; AIR-POLLUTION ; TRACE GASES ; BIOFUEL CONSUMPTION ; GASOLINE VEHICLES ; UNITED-STATES |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/30413 |
专题 | 地球科学 |
作者单位 | 1.Univ Felix Houphouet Boigny, Lab Phys Atmosphere, BPV 34, Abidjan, Cote Ivoire; 2.Univ Toulouse, Lab Aerol, CNRS, UPS, Toulouse, France; 3.Univ Clermont Auvergne, CNRS, LaMP, F-63000 Clermont Ferrand, France; 4.Univ Manchester, Ctr Atmospher Sci, Manchester M13 9PL, Lancs, England; 5.Univ Abomey Calavi, Lab Phys Rayonnement, Abomey Calavi, Benin |
推荐引用方式 GB/T 7714 | Keita, Sekou,39;Datchoh, E. Toure. Particle and VOC emission factor measurements for anthropogenic sources in West Africa[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(10):7691-7708. |
APA | Keita, Sekou,&39;Datchoh, E. Toure.(2018).Particle and VOC emission factor measurements for anthropogenic sources in West Africa.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(10),7691-7708. |
MLA | Keita, Sekou,et al."Particle and VOC emission factor measurements for anthropogenic sources in West Africa".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.10(2018):7691-7708. |
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