GSTDTAP  > 地球科学
DOI10.5194/acp-19-1881-2019
Impacts of short-term mitigation measures on PM2.5 and radiative effects: a case study at a regional background site near Beijing, China
Wang, Qiyuan1,2; Liu, Suixin1; Li, Nan3; Dai, Wenting1; Wu, Yunfei4; Tian, Jie5; Zhou, Yaqing1; Wang, Meng1; Sai, Steven1; Ho, Hang; Chen, Yang6; Zhang, Renjian4; Zhao, Shuyu1; Zhu, Chongshu1; Han, Yongming1,2,7; Tie, Xuexi1; Cao, Junji1,2,8
2019-02-12
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2019
卷号19期号:3页码:1881-1899
文章类型Article
语种英语
国家Peoples R China
英文摘要

Measurements at a background site near Beijing showed that pollution controls implemented during the 19th National Congress of the Communist Party of China (NC-CPC) were effective in reducing PM2.5. Mass concentrations of PM2.5 and its major chemical components were 20.6%-43.1% lower during the NCCPC-control period compared with a non-control period, and differences were greater on days with stable meteorological conditions. A receptor model showed that PM2.5 from traffic-related emissions, biomass burning, industrial processes, and mineral dust was 38.5%-77.8% lower during the NCCPC-control versus non-control period, but differences in PM2.5 from coal burning were small, and secondary sources were higher during the NCCPC-control period. During one pollution episode in the non-control period, secondary sources dominated, and the WRF-Chem model showed that the Beijing-Tianjin-Hebei (BTH) region contributed 73.6% of PM2.5 mass. A second pollution episode was linked to biomass burning, and BTH contributed 46.9% of PM2.5 mass. Calculations based on Interagency Monitoring of Protected Visual Environments (IMPROVE) algorithms showed that organic matter was the largest contributor to light extinction during the non-control period whereas NH4NO3 was the main contributor during the NCCPC. The Tropospheric Ultraviolet and Visible radiation model showed that the average direct radiative forcing (DRF) values at the Earth's surface were -14.0 and -19.3 W m(-2) during the NCCPC-control and non-control periods, respectively, and the DRF for the individual PM2.5 components were 22.7%-46.7% lower during the NCCPC. The information and dataset from this study will be useful for developing air pollution control strategies in the BTH region and for understanding associated aerosol radiative effects.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000458362200004
WOS关键词SECONDARY ORGANIC AEROSOL ; FINE PARTICULATE MATTER ; BLACK CARBON AEROSOL ; AIR-QUALITY IMPROVEMENT ; SEVERE WINTER HAZE ; PEARL RIVER DELTA ; SOURCE APPORTIONMENT ; CHEMICAL-COMPOSITION ; EMISSION CONTROLS ; MEXICO-CITY
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/30393
专题地球科学
作者单位1.Chinese Acad Sci, State Key Lab Loess & Quaternary Geol, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China;
2.CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China;
3.Nanjing Univ Informat Sci & Technol, Sch Environm Sci & Engn, Nanjing 210044, Jiangsu, Peoples R China;
4.Chinese Acad Sci, Inst Atmospher Phys, Key Lab Reg Climate Environm Res Temperate East A, Beijing 100029, Peoples R China;
5.Xi An Jiao Tong Univ, Sch Energy & Power Engn, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China;
6.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China;
7.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Shaanxi, Peoples R China;
8.Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Wang, Qiyuan,Liu, Suixin,Li, Nan,et al. Impacts of short-term mitigation measures on PM2.5 and radiative effects: a case study at a regional background site near Beijing, China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(3):1881-1899.
APA Wang, Qiyuan.,Liu, Suixin.,Li, Nan.,Dai, Wenting.,Wu, Yunfei.,...&Cao, Junji.(2019).Impacts of short-term mitigation measures on PM2.5 and radiative effects: a case study at a regional background site near Beijing, China.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(3),1881-1899.
MLA Wang, Qiyuan,et al."Impacts of short-term mitigation measures on PM2.5 and radiative effects: a case study at a regional background site near Beijing, China".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.3(2019):1881-1899.
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