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DOI | 10.1175/JAS-D-16-0074.1 |
A New Ice Nucleation Active Site Parameterization for Desert Dust and Soot | |
Ullrich, Romy; Hoose, Corinna; Moehler, Ottmar; Niemand, Monika; Wagner, Robert; Hoehler, Kristina; Hiranuma, Naruki; Saathoff, Harald; Leisner, Thomas | |
2017-03-01 | |
发表期刊 | JOURNAL OF THE ATMOSPHERIC SCIENCES
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ISSN | 0022-4928 |
EISSN | 1520-0469 |
出版年 | 2017 |
卷号 | 74期号:3 |
文章类型 | Article |
语种 | 英语 |
国家 | Germany |
英文摘要 | Based on results of 11 yr of heterogeneous ice nucleation experiments at the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) chamber in Karlsruhe, Germany, a new empirical parameterization framework for heterogeneous ice nucleation was developed. The framework currently includes desert dust and soot aerosol and quantifies the ice nucleation efficiency in terms of the ice nucleation active surface site (INAS) approach. The immersion freezing INAS densities n(S) of all desert dust experiments follow an exponential fit as a function of temperature, well in agreement with an earlier analysis of AIDA experiments. The deposition nucleation n(S) isolines for desert dust follow u-shaped curves in the ice saturation ratio-temperature (Si-T) diagram at temperatures below about 240 K. The negative slope of these isolines toward lower temperatures may be explained by classical nucleation theory (CNT), whereas the behavior toward higher temperatures may be caused by a pore condensation and freezing mechanism. The deposition nucleation measured for soot at temperatures below about 240K also follows u-shaped isolines with a shift toward higher Si for soot with higher organic carbon content. For immersion freezing of soot aerosol, only upper limits for n(S) were determined and used to rescale an existing parameterization line. The new parameterization framework is compared to a CNT-based parameterization and an empirical framework as used in models. The comparison shows large differences in shape and magnitude of the n(S) isolines especially for deposition nucleation. For the application in models, implementation of this new framework is simple compared to that of other expressions. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000394344800004 |
WOS关键词 | MINERAL DUST ; AEROSOL-PARTICLES ; CLOUD FORMATION ; NUCLEI ; ACTIVATION ; PHASE ; SIMULATION ; EFFICIENCY ; DROPLETS ; ABILITY |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/29792 |
专题 | 地球科学 |
作者单位 | Karlsruhe Inst Technol, Inst Meteorol & Climate Res, Karlsruhe, Germany |
推荐引用方式 GB/T 7714 | Ullrich, Romy,Hoose, Corinna,Moehler, Ottmar,et al. A New Ice Nucleation Active Site Parameterization for Desert Dust and Soot[J]. JOURNAL OF THE ATMOSPHERIC SCIENCES,2017,74(3). |
APA | Ullrich, Romy.,Hoose, Corinna.,Moehler, Ottmar.,Niemand, Monika.,Wagner, Robert.,...&Leisner, Thomas.(2017).A New Ice Nucleation Active Site Parameterization for Desert Dust and Soot.JOURNAL OF THE ATMOSPHERIC SCIENCES,74(3). |
MLA | Ullrich, Romy,et al."A New Ice Nucleation Active Site Parameterization for Desert Dust and Soot".JOURNAL OF THE ATMOSPHERIC SCIENCES 74.3(2017). |
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