GSTDTAP  > 地球科学
DOI10.5194/acp-19-3007-2019
Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016
Si, Meng1; Evoy, Erin1; Yun, Jingwei1; Xi, Yu1; Hanna, Sarah J.1; Chivulescu, Alina2; Rawlings, Kevin2; Veber, Daniel2; Platt, Andrew2; Kunkel, Daniel3; Hoor, Peter3; Sharma, Sangeeta2; Leaitch, W. Richard2; Bertram, Allan K.1
2019-03-08
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2019
卷号19期号:5页码:3007-3024
文章类型Article
语种英语
国家Canada; Germany
英文摘要

Modelling studies suggest that the climate and the hydrological cycle are sensitive to the concentrations of ice-nucleating particles (INPs). However, the concentrations, composition, and sources of INPs in the atmosphere remain uncertain. Here, we report daily concentrations of INPs in the immersion freezing mode and tracers of mineral dust (Al, Fe, Ti, and Mn), sea spray aerosol (Na+ and Cl-), and anthropogenic aerosol (Zn, Pb, NO3-, NH4+, and non-sea-salt SO42-) at Alert, Canada, during a 3-week campaign in March 2016. In total, 16 daily measurements of INPs are reported. The average INP concentrations measured in the immersion freezing mode were 0.005 +/- 0.002, 0.020 +/- 0.004, and 0.186 +/- 0.040 L-1 at -15, -20, and -25 degrees C, respectively. These concentrations are within the range of concentrations measured previously in the Arctic at ground level or sea level. Mineral dust tracers all correlated with INPs at -25 degrees C (correlation coefficient, R, ranged from 0.70 to 0.76), suggesting that mineral dust was a major contributor to the INP population at -25 degrees C. Particle dispersion modelling suggests that the source of the mineral dust may have been long-range transport from the Gobi Desert. Sea spray tracers were anti-correlated with INPs at -25 degrees C (R = -0.56). In addition, INP concentrations at 25 degrees C divided by mass concentrations of aluminum were anti-correlated with sea spray tracers (R = -0.51 and -0.55 for Na-4(+) and Cl-, respectively), suggesting that the components of sea spray aerosol suppressed the ice-nucleating ability of mineral dust in the immersion freezing mode. Correlations between INPs and anthropogenic aerosol tracers were not statistically significant. These results will improve our understanding of INPs in the Arctic during spring.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000460817300001
WOS关键词RELATIVE-HUMIDITY ; DISPERSION MODEL ; FORMING NUCLEI ; AIR-POLLUTION ; FREEZING NUCLEATION ; TECHNICAL NOTE ; AEROSOL ; MARINE ; CLOUD ; SNOW
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/29508
专题地球科学
作者单位1.Univ British Columbia, Dept Chem, Vancouver, BC V6T 1Z1, Canada;
2.Environm & Climate Change Canada, Climate Res Div, Toronto, ON M3H 5T4, Canada;
3.Johannes Gutenberg Univ Mainz, Inst Atmospher Phys, D-55128 Mainz, Germany
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GB/T 7714
Si, Meng,Evoy, Erin,Yun, Jingwei,et al. Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(5):3007-3024.
APA Si, Meng.,Evoy, Erin.,Yun, Jingwei.,Xi, Yu.,Hanna, Sarah J..,...&Bertram, Allan K..(2019).Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(5),3007-3024.
MLA Si, Meng,et al."Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.5(2019):3007-3024.
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