Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-17-981-2017 |
Concentrations and stable carbon isotope compositions of oxalic acid and related SOA in Beijing before, during, and after the 2014 APEC | |
Wang, Jiayuan1,3; Wang, Gehui1,2,3,4; Gao, Jian5,6; Wang, Han5,6; Ren, Yanqin1,3; Li, Jianjun1; Zhou, Bianhong1; Wu, Can1,3; Zhang, Lu1,3; Wang, Shulan5,6; Chai, Fahe5,6 | |
2017-01-23 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2017 |
卷号 | 17期号:2 |
文章类型 | Article |
语种 | 英语 |
国家 | Peoples R China |
英文摘要 | To ensure good air quality for the 2014 AsiaPacific Economic Cooperation (APEC) summit, stringent emission controls were implemented in Beijing and its surrounding regions, leading to a significant reduction in PM2.5 loadings. To investigate the impact of the emission controls on aerosol chemistry, high-volume PM2.5 samples were collected in Beijing from 8 October to 24 November 2014 and determined for secondary inorganic aerosols (SIA, i.e., SO42-, NO3-, and NH4+), dicarboxylic acids, keto-carboxylic acid, and alpha-dicarbonyls, as well as stable carbon isotope composition of oxalic acid (C-2). Our results showed that SIA, C-2, and related secondary organic aerosols in PM2.5 during APEC were 2-4 times lower than those before APEC, which is firstly ascribed to the strict emission control measures and secondly attributed to the relatively colder and drier conditions during the event that are unfavorable for secondary aerosol production. C-2 in the polluted air masses, which mostly occurred before APEC, are abundant and enriched in C-13. On the contrary, C-2 in the clean air masses, which mostly occurred during APEC, is much less abundant but still enriched in C-13. In the mixed type of clean and polluted air masses, which mostly occurred after APEC, C-2 is lower than that before APEC but higher than that during APEC and enriched in lighter C-12. A comparison on chemical composition of fine particles and delta C-13 values of C-2 in two events that are characterized by high loadings of PM2.5 further showed that after APEC SIA and the total detected organic compounds (TDOC) are much less abundant and fine aerosols are enriched with primary organics and relatively fresh, compared with those before APEC. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000394595300002 |
WOS关键词 | ORGANIC AEROSOL FORMATION ; DICARBOXYLIC-ACIDS ; KETOCARBOXYLIC ACIDS ; ATMOSPHERIC AEROSOLS ; CHINA IMPLICATIONS ; ALPHA-DICARBONYLS ; EMISSION CONTROLS ; PARTICLES ; DISTRIBUTIONS ; TROPOSPHERE |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/28353 |
专题 | 地球科学 |
作者单位 | 1.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, State Key Lab Loess & Quaternary Geol, Xian 710061, Peoples R China; 2.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710079, Peoples R China; 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China; 4.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China; 5.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100084, Peoples R China; 6.Collaborat Innovat Ctr Atmospher Environm & Equip, Nanjing 210000, Jiangsu, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Jiayuan,Wang, Gehui,Gao, Jian,et al. Concentrations and stable carbon isotope compositions of oxalic acid and related SOA in Beijing before, during, and after the 2014 APEC[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(2). |
APA | Wang, Jiayuan.,Wang, Gehui.,Gao, Jian.,Wang, Han.,Ren, Yanqin.,...&Chai, Fahe.(2017).Concentrations and stable carbon isotope compositions of oxalic acid and related SOA in Beijing before, during, and after the 2014 APEC.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(2). |
MLA | Wang, Jiayuan,et al."Concentrations and stable carbon isotope compositions of oxalic acid and related SOA in Beijing before, during, and after the 2014 APEC".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.2(2017). |
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