GSTDTAP  > 资源环境科学
DOI10.1038/s41467-020-16510-3
Ambient weathering of magnesium oxide for CO2 removal from air
McQueen, Noah1; Kelemen, Peter2; Dipple, Greg3; Renforth, Phil4; Wilcox, Jennifer1
2020-07-03
发表期刊NATURE COMMUNICATIONS
ISSN2041-1723
出版年2020
卷号11期号:1
文章类型Article
语种英语
国家USA; Canada; Scotland
英文摘要

To avoid dangerous climate change, new technologies must remove billions of tonnes of CO2 from the atmosphere every year by mid-century. Here we detail a land-based enhanced weathering cycle utilizing magnesite (MgCO3) feedstock to repeatedly capture CO2 from the atmosphere. In this process, MgCO3 is calcined, producing caustic magnesia (MgO) and high-purity CO2. This MgO is spread over land to carbonate for a year by reacting with atmospheric CO2. The carbonate minerals are then recollected and re-calcined. The reproduced MgO is spread over land to carbonate again. We show this process could cost approximately $46-159 tCO(2)(-1) net removed from the atmosphere, considering grid and solar electricity without post-processing costs. This technology may achieve lower costs than projections for more extensively engineered Direct Air Capture methods. It has the scalable potential to remove at least 2-3 GtCO(2) year(-1), and may make a meaningful contribution to mitigating climate change. To remove CO2 from the atmosphere every year by mid-century will need new technologies. Here the authors proposed the use of magnesia (MgO) in ambient looping processes to remove CO2 from the air and they found that the proposed approach will cost $46-195 tCO(2)(-1) net removed from the atmosphere considering both grid and solar electricity resources without including post-processing costs.


领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000546621600015
WOS关键词MINERAL CARBONATION ; CAPTURE ; MGO ; DISSOLUTION ; SERPENTINE ; PERIDOTITE ; DIOXIDE ; DEHYDROXYLATION ; SEQUESTRATION ; PRECIPITATION
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/281820
专题资源环境科学
作者单位1.Worcester Polytech Inst, Dept Chem Engn, Clean Energy Convers Lab, 100 Inst Rd, Worcester, MA 01609 USA;
2.Columbia Univ, Dept Earth & Environm Sci, Lamont Doherty Earth Observ, 91 Rte 9W, Palisades, NY 10964 USA;
3.Univ British Columbia, Bradshaw Res Initiat Minerals & Min, Dept Earth Ocean & Atmospher Sci, 2020-2207 Main Mall, Vancouver, BC V6T 1Z4, Canada;
4.Heriot Watt Univ, Sch Engn & Phys Sci, Res Ctr Carbon Solut, Edinburgh EH14 4AS, Midlothian, Scotland
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GB/T 7714
McQueen, Noah,Kelemen, Peter,Dipple, Greg,et al. Ambient weathering of magnesium oxide for CO2 removal from air[J]. NATURE COMMUNICATIONS,2020,11(1).
APA McQueen, Noah,Kelemen, Peter,Dipple, Greg,Renforth, Phil,&Wilcox, Jennifer.(2020).Ambient weathering of magnesium oxide for CO2 removal from air.NATURE COMMUNICATIONS,11(1).
MLA McQueen, Noah,et al."Ambient weathering of magnesium oxide for CO2 removal from air".NATURE COMMUNICATIONS 11.1(2020).
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