GSTDTAP  > 资源环境科学
DOI10.1029/2018WR024436
Identifying Hydrogeochemical Conditions for Fault Self-Sealing in Geological CO2 Storage
Patil, Vivek V.1; McPherson, Brian J.1,2
2020-03-01
发表期刊WATER RESOURCES RESEARCH
ISSN0043-1397
EISSN1944-7973
出版年2020
卷号56期号:3
文章类型Article
语种英语
国家USA
英文摘要

Injection of anthropogenic CO2 into a subsurface reservoir will significantly impact the geochemistry, porosity, and permeability of the reservoir. If a fault or fracture penetrates the reservoir, CO2-enriched brine may migrate into that fault, eventually sealing it via precipitation or opening it up via dissolution. The goal of this study was to identify and quantify such conditions of fault self-sealing or self-enhancing. We found the Damkohler number (Da) provides a meaningful framework for characterizing the propensity of (fault) systems to seal or open up. We tailored a spatiotemporally varying Da framework and applied it to simplified fault models with eight conditions derived from four geologic compositions and two reservoir conditions. The four geologic compositions were chosen such that three of them were representative of distinct geologic end-members (sandstone, mudstone, and dolomitic limestone) and one was a mixed composition based on an average of three end-member compositions. The two sets of P-T conditions chosen included one for CO2 in a gaseous phase ("shallow conditions") and the other for supercritical phase CO2 ("deep conditions"). Simulation results suggest that fault sealing via carbonate precipitation was a possibility for shallow conditions within limestone and mixed composition settings. The concentration of cations in the water was found to be an important control on the carbonate precipitation. A key conclusion suggested by the results of this study is that carbonate precipitation in the near-surface (top 50-100 m) depths of a fault is the most likely mechanism of "self-sealing" for most geological settings.


领域资源环境
收录类别SCI-E
WOS记录号WOS:000538000800004
WOS关键词NATURAL CO2 ; FLUID-FLOW ; COUPLED MODEL ; REACTIVE FLOW ; TRANSPORT ; LEAKAGE ; DISPOSAL ; PERMEABILITY ; SIMULATION ; RESERVOIR
WOS类目Environmental Sciences ; Limnology ; Water Resources
WOS研究方向Environmental Sciences & Ecology ; Marine & Freshwater Biology ; Water Resources
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/280589
专题资源环境科学
作者单位1.Univ Utah, Energy & Geosci Inst, Salt Lake City, UT 84112 USA;
2.Univ Utah, Dept Civil & Environm Engn, Salt Lake City, UT 84112 USA
推荐引用方式
GB/T 7714
Patil, Vivek V.,McPherson, Brian J.. Identifying Hydrogeochemical Conditions for Fault Self-Sealing in Geological CO2 Storage[J]. WATER RESOURCES RESEARCH,2020,56(3).
APA Patil, Vivek V.,&McPherson, Brian J..(2020).Identifying Hydrogeochemical Conditions for Fault Self-Sealing in Geological CO2 Storage.WATER RESOURCES RESEARCH,56(3).
MLA Patil, Vivek V.,et al."Identifying Hydrogeochemical Conditions for Fault Self-Sealing in Geological CO2 Storage".WATER RESOURCES RESEARCH 56.3(2020).
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