GSTDTAP  > 气候变化
DOI10.1029/2019GL085706
Effects of Chemical Feedbacks on Decadal Methane Emissions Estimates
Nguyen, Newton H.1; Turner, Alexander J.2,3,4; Yin, Yi1; Prather, Michael J.5; Frankenberg, Christian1,4
2020-02-16
发表期刊GEOPHYSICAL RESEARCH LETTERS
ISSN0094-8276
EISSN1944-8007
出版年2020
卷号47期号:3
文章类型Article
语种英语
国家USA
英文摘要

The coupled chemistry of methane, carbon monoxide (CO), and hydroxyl radical (OH) can modulate methane's 9-year lifetime. This is often ignored in methane flux inversions, and the impacts of neglecting interactive chemistry have not been quantified. Using a coupled-chemistry box model, we show that neglecting the effect of methane source perturbation on [OH] can lead to a 25% bias in estimating abrupt changes in methane sources after only 10 years. Further, large CO emissions, such as from biomass burning, can increase methane concentrations by extending the methane lifetime through impacts on [OH]. Finally, we quantify the biases of including (or excluding) coupled chemistry in the context of recent methane and CO trends. Decreasing CO concentrations, beginning in the 2000's, have notable impacts on methane flux inversions. Given these nonnegligible errors, decadal methane emissions inversions should incorporate chemical feedbacks for more robust methane trend analyses and source attributions.


领域气候变化
收录类别SCI-E
WOS记录号WOS:000529107400040
WOS关键词INTERANNUAL VARIABILITY ; ATMOSPHERIC CHEMISTRY ; OH VARIABILITY ; FOSSIL-FUEL ; HYDROXYL ; CLIMATE ; GROWTH ; BUDGET ; MODEL ; CH4
WOS类目Geosciences, Multidisciplinary
WOS研究方向Geology
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/279573
专题气候变化
作者单位1.CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA;
2.Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA;
3.Univ Calif Berkeley, Coll Chem, Berkeley, CA 94720 USA;
4.CALTECH, NASA Jet Prop Lab, Pasadena, CA 91125 USA;
5.Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA USA
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GB/T 7714
Nguyen, Newton H.,Turner, Alexander J.,Yin, Yi,et al. Effects of Chemical Feedbacks on Decadal Methane Emissions Estimates[J]. GEOPHYSICAL RESEARCH LETTERS,2020,47(3).
APA Nguyen, Newton H.,Turner, Alexander J.,Yin, Yi,Prather, Michael J.,&Frankenberg, Christian.(2020).Effects of Chemical Feedbacks on Decadal Methane Emissions Estimates.GEOPHYSICAL RESEARCH LETTERS,47(3).
MLA Nguyen, Newton H.,et al."Effects of Chemical Feedbacks on Decadal Methane Emissions Estimates".GEOPHYSICAL RESEARCH LETTERS 47.3(2020).
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