GSTDTAP  > 气候变化
DOI10.1029/2018GL079873
Evidence for Changes in Arctic Cloud Phase Due to Long-Range Pollution Transport
Coopman, Q.1,2,3; Riedi, J.1; Finch, D. P.4; Garrett, T. J.2
2018-10-16
发表期刊GEOPHYSICAL RESEARCH LETTERS
ISSN0094-8276
EISSN1944-8007
出版年2018
卷号45期号:19页码:10709-10718
文章类型Article
语种英语
国家France; USA; Germany; Scotland
英文摘要

Reduced precipitation rates allow pollution within air parcels from midlatitudes to reach the Arctic without being scavenged. We use satellite and tracer transport model data sets to evaluate the degree of supercooling required for 50% of a chosen ensemble of low-level clouds to be in the ice phase for a given meteorological regime. Our results suggest that smaller cloud droplet effective radii are related to higher required amounts of supercooling but that, overall, pollution plumes from fossil fuel combustion lower the degree of supercooling that is required for freezing by approximately 4 degrees C. The relationship between anthropogenic plumes and the freezing transition temperature from liquid to ice remains to be explained.


Plain Language Summary Anthropogenic pollution plumes from midlatitudes can be transported long distances to the Arctic. In this study, we analyze the impact of these plumes on how easily liquid clouds over the Arctic Ocean freeze by using a novel combination of satellite measurements and a pollution transport model. We find that liquid clouds in polluted air switch phase to become ice clouds at temperatures that are 4 degrees C higher they would otherwise in pristine air. Because ice clouds in the Arctic precipitate more easily than liquid clouds, the potential is that distant industrial pollution sources are acting to reduce arctic cloud life time.


领域气候变化
收录类别SCI-E
WOS记录号WOS:000448656800076
WOS关键词MICROPHYSICAL PROPERTIES ; AIR-POLLUTION ; ICE PARTICLES ; AEROSOL ; VARIABILITY ; MODEL ; EMISSIONS ; POLDER ; SMOKE ; IDENTIFICATION
WOS类目Geosciences, Multidisciplinary
WOS研究方向Geology
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/27927
专题气候变化
作者单位1.Univ Lille, CNRS, UMR 8518, LOA, Lille, France;
2.Univ Utah, Dept Atmospher Sci, Salt Lake City, UT 84112 USA;
3.Karlsruhe Inst Technol, Inst Meteorol & Climate Res, Karlsruhe, Germany;
4.Univ Edinburgh, Sch Geosci, Edinburgh, Midlothian, Scotland
推荐引用方式
GB/T 7714
Coopman, Q.,Riedi, J.,Finch, D. P.,et al. Evidence for Changes in Arctic Cloud Phase Due to Long-Range Pollution Transport[J]. GEOPHYSICAL RESEARCH LETTERS,2018,45(19):10709-10718.
APA Coopman, Q.,Riedi, J.,Finch, D. P.,&Garrett, T. J..(2018).Evidence for Changes in Arctic Cloud Phase Due to Long-Range Pollution Transport.GEOPHYSICAL RESEARCH LETTERS,45(19),10709-10718.
MLA Coopman, Q.,et al."Evidence for Changes in Arctic Cloud Phase Due to Long-Range Pollution Transport".GEOPHYSICAL RESEARCH LETTERS 45.19(2018):10709-10718.
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