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DOI10.5194/acp-20-771-2020
Natural sea-salt emissions moderate the climate forcing of anthropogenic nitrate
Chen, Ying1,2,3,9; Cheng, Yafang2; Ma, Nan1,2,3,4; Wei, Chao3; Ran, Liang5; Wolke, Ralf6; Groess, Johannes1; Wang, Qiaoqiao4; Pozzer, Andrea7; van der Gon, Hugo A. C. Denier8; Spindler, Gerald10; Lelieveld, Jos7,11; Tegen, Ina6; Su, Hang3; Wiedensohler, Alfred1
2020-01-22
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2020
卷号20期号:2页码:771-786
文章类型Article
语种英语
国家Germany; Peoples R China; Netherlands; England; Cyprus
英文摘要

Natural sea-salt aerosols, when interacting with anthropogenic emissions, can enhance the formation of particulate nitrate. This enhancement has been suggested to increase the direct radiative forcing of nitrate, called the "mass-enhancement effect". Through a size-resolved dynamic mass transfer modeling approach, we show that interactions with sea salt shift the nitrate from sub- to super-micron-sized particles ("redistribution effect"), and hence this lowers its efficiency for light extinction and reduces its lifetime. The redistribution effect overwhelms the mass-enhancement effect and significantly moderates nitrate cooling; e.g., the nitrate-associated aerosol optical depth can be reduced by 10 %-20 % over European polluted regions during a typical sea-salt event, in contrast to an increase by similar to 10 % when only accounting for the mass-enhancement effect. Global model simulations indicate significant redistribution over coastal and offshore regions worldwide. Our study suggests a strong buffering by natural sea-salt aerosols that reduces the climate forcing of anthropogenic nitrate, which had been expected to dominate the aerosol cooling by the end of the century. Comprehensive considerations of this redistribution effect foster better understandings of climate change and nitrogen deposition.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000508615500004
WOS关键词GENERAL-CIRCULATION ; NORTHWESTERN EUROPE ; HYGROSCOPIC GROWTH ; GLOBAL SIMULATIONS ; AIR-POLLUTION ; MINERAL DUST ; CHEM MODEL ; AEROSOL ; CHEMISTRY ; SIZE
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/278583
专题地球科学
作者单位1.Leibniz Inst Tropospher Res, Dept Expt Aerosol & Cloud Microphys, Leipzig, Germany;
2.Max Planck Inst Chem, Minerva Res Grp, Mainz, Germany;
3.Max Planck Inst Chem, Multiphase Chem Dept, Mainz, Germany;
4.Jinan Univ, Ctr Pollut & Climate Change Res APCC, Inst Environm & Climate Res, Guangzhou, Peoples R China;
5.Chinese Acad Sci, Inst Atmospher Phys, Key Lab Middle Atmosphere & Global Environm Obser, Beijing, Peoples R China;
6.Leibniz Inst Tropospher Res, Modelling Atmospher Proc, Leipzig, Germany;
7.Max Planck Inst Chem, Atmospher Chem Dept, Mainz, Germany;
8.TNO, Dept Climate Air & Sustainabil, Princetonlaan 6, Utrecht, Netherlands;
9.Univ Lancaster, Lancaster Environm Ctr, Lancaster, England;
10.Leibniz Inst Tropospher Res, Atmospher Chem Dept, Leipzig, Germany;
11.Cyprus Inst, Nicosia, Cyprus
推荐引用方式
GB/T 7714
Chen, Ying,Cheng, Yafang,Ma, Nan,et al. Natural sea-salt emissions moderate the climate forcing of anthropogenic nitrate[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2020,20(2):771-786.
APA Chen, Ying.,Cheng, Yafang.,Ma, Nan.,Wei, Chao.,Ran, Liang.,...&Wiedensohler, Alfred.(2020).Natural sea-salt emissions moderate the climate forcing of anthropogenic nitrate.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(2),771-786.
MLA Chen, Ying,et al."Natural sea-salt emissions moderate the climate forcing of anthropogenic nitrate".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.2(2020):771-786.
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