Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1002/2017GL074215 |
Gas-aerosol partitioning of ammonia in biomass burning plumes: Implications for the interpretation of spaceborne observations of ammonia and the radiative forcing of ammonium nitrate | |
Paulot, F.1,2; Paynter, D.2; Ginoux, P.2; Naik, V.2; Whitburn, S.3; Van Damme, M.3; Clarisse, L.3; Coheur, P. -F.3; Horowitz, L. W.2 | |
2017-08-16 | |
发表期刊 | GEOPHYSICAL RESEARCH LETTERS |
ISSN | 0094-8276 |
EISSN | 1944-8007 |
出版年 | 2017 |
卷号 | 44期号:15 |
文章类型 | Article |
语种 | 英语 |
国家 | USA; Belgium |
英文摘要 | Satellite-derived enhancement ratios of NH3 relative to CO column burden (ERNH3/CO) in fires over Alaska, the Amazon, and South Equatorial Africa are 35, 45, and 70% lower than the corresponding ratio of their emissions factors (EFNH3/CO) from biomass burning derived from in situ observations. Simulations performed using the Geophysical Fluid Dynamics Laboratory AM3 global chemistry-climate model show that these regional differences may not entirely stem from an overestimate of NH3 emissions but rather from changes in the gas-aerosol partitioning of NH3 to NH4+. Differences between ERNH3/CO and EFNH3/CO are largest in regions where EFNOx/NH3 is high, consistent with the production of NH4NO3. Biomass burning is estimated to contribute 11-23% of the global burden and direct radiative effect (DRE) of NH4NO3 (-15 to -28 mW m(-2)), despite accounting for less than 6% of the global source of NH3. Production of NH4NO3 is largely concentrated over the Amazon and South Equatorial Africa, where its DRE can reach -1.9Wm(-2) during the biomass burning season. |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000408379000059 |
WOS关键词 | ATMOSPHERIC AMMONIA ; REACTIVE NITROGEN ; TRACE GASES ; CHEMICAL CHARACTERISTICS ; GLOBAL DISTRIBUTIONS ; PARTICULATE MATTER ; CARBON-MONOXIDE ; EMISSIONS ; FIRE ; MODEL |
WOS类目 | Geosciences, Multidisciplinary |
WOS研究方向 | Geology |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/26587 |
专题 | 气候变化 |
作者单位 | 1.Princeton Univ, Program Atmospher & Ocean Sci, Princeton, NJ 08544 USA; 2.Natl Ocean & Atmospher Adm, Geophys Fluid Dynam Lab, Princeton, NJ 20230 USA; 3.Univ Libre Bruxelles, Atmospher Spect, Serv Chim Quant & Photophys, Brussels, Belgium |
推荐引用方式 GB/T 7714 | Paulot, F.,Paynter, D.,Ginoux, P.,et al. Gas-aerosol partitioning of ammonia in biomass burning plumes: Implications for the interpretation of spaceborne observations of ammonia and the radiative forcing of ammonium nitrate[J]. GEOPHYSICAL RESEARCH LETTERS,2017,44(15). |
APA | Paulot, F..,Paynter, D..,Ginoux, P..,Naik, V..,Whitburn, S..,...&Horowitz, L. W..(2017).Gas-aerosol partitioning of ammonia in biomass burning plumes: Implications for the interpretation of spaceborne observations of ammonia and the radiative forcing of ammonium nitrate.GEOPHYSICAL RESEARCH LETTERS,44(15). |
MLA | Paulot, F.,et al."Gas-aerosol partitioning of ammonia in biomass burning plumes: Implications for the interpretation of spaceborne observations of ammonia and the radiative forcing of ammonium nitrate".GEOPHYSICAL RESEARCH LETTERS 44.15(2017). |
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