Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1002/2017GL073359 |
Evidence for marine biogenic influence on summertime Arctic aerosol | |
Willis, Megan D.1; Koellner, Franziska2; Burkart, Julia1; Bozem, Heiko3; Thomas, Jennie L.4; Schneider, Johannes2; Aliabadi, Amir A.5; Hoor, Peter M.3; Schulz, Hannes6; Herber, Andreas B.6; Leaitch, W. Richard7; Abbatt, Jonathan P. D.1 | |
2017-06-28 | |
发表期刊 | GEOPHYSICAL RESEARCH LETTERS |
ISSN | 0094-8276 |
EISSN | 1944-8007 |
出版年 | 2017 |
卷号 | 44期号:12 |
文章类型 | Article |
语种 | 英语 |
国家 | Canada; Germany; France |
英文摘要 | We present vertically resolved observations of aerosol composition during pristine summertime Arctic background conditions. The methansulfonic acid (MSA)-to-sulfate ratio peaked near the surface (mean 0.10), indicating a contribution from ocean-derived biogenic sulfur. Similarly, the organic aerosol (OA)-to-sulfate ratio increased toward the surface (mean 2.0). Both MSA-to-sulfate and OA-to-sulfate ratios were significantly correlated with FLEXPART-WRF-predicted air mass residence time over open water, indicating marine-influenced OA. External mixing of sea salt aerosol from a larger number fraction of organic, sulfate, and amine-containing particles, together with low wind speeds (median 4.7ms(-1)), suggests a role for secondary organic aerosol formation. Cloud condensation nuclei concentrations were nearly constant (approximate to 120cm(-3)) when the OA fraction was <60% and increased to 350cm(-3) when the organic fraction was larger and residence times over open water were longer. Our observations illustrate the importance of marine-influenced OA under Arctic background conditions, which are likely to change as the Arctic transitions to larger areas of open water. |
英文关键词 | Arctic aerosol marine organic aerosol methanesulfonic acid aerosol mass spectrometry Arctic summer secondary organic aerosol |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000405854200067 |
WOS关键词 | CLOUD CONDENSATION NUCLEI ; SEA-SPRAY AEROSOL ; CHEMICAL CHARACTERISTICS ; ATMOSPHERIC PARTICLES ; ORGANIC-COMPOUNDS ; ZEPPELIN STATION ; AIR-POLLUTION ; SIZE ; OCEAN ; DISTRIBUTIONS |
WOS类目 | Geosciences, Multidisciplinary |
WOS研究方向 | Geology |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/26276 |
专题 | 气候变化 |
作者单位 | 1.Univ Toronto, Dept Chem, Toronto, ON, Canada; 2.Max Planck Inst Chem, Mainz, Germany; 3.Johannes Gutenberg Univ Mainz, Inst Atmospher Phys, Mainz, Germany; 4.UPMC, CNRS, LATMOS IPSL, UVSQ, Paris, France; 5.Univ Guelph, Sch Engn, Guelph, ON, Canada; 6.Helmholtz Ctr Polar & Marine Res Bremerhaven, Alfred Wegener Inst, Bremerhaven, Germany; 7.Environm & Climate Change Canada, Toronto, ON, Canada |
推荐引用方式 GB/T 7714 | Willis, Megan D.,Koellner, Franziska,Burkart, Julia,et al. Evidence for marine biogenic influence on summertime Arctic aerosol[J]. GEOPHYSICAL RESEARCH LETTERS,2017,44(12). |
APA | Willis, Megan D..,Koellner, Franziska.,Burkart, Julia.,Bozem, Heiko.,Thomas, Jennie L..,...&Abbatt, Jonathan P. D..(2017).Evidence for marine biogenic influence on summertime Arctic aerosol.GEOPHYSICAL RESEARCH LETTERS,44(12). |
MLA | Willis, Megan D.,et al."Evidence for marine biogenic influence on summertime Arctic aerosol".GEOPHYSICAL RESEARCH LETTERS 44.12(2017). |
条目包含的文件 | 条目无相关文件。 |
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