GSTDTAP  > 地球科学
DOI10.5194/acp-17-1511-2017
The impact of resolution on meteorological, chemical and aerosol properties in regional simulations with WRF-Chem
Crippa, Paola1; Sullivan, Ryan C.2; Thota, Abhinav3; Pryor, Sara C.2,3
2017-01-31
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2017
卷号17期号:2
文章类型Article
语种英语
国家England; USA
英文摘要

Limited area (regional) models applied at high resolution over specific regions of interest are generally expected to more accurately capture the spatiotemporal variability of key meteorological and climate parameters. However, improved performance is not inevitable, and there remains a need to optimize use of numerical resources and to quantify the impact on simulation fidelity that derives from increased resolution. The application of regional models for climate forcing assessment is currently limited by the lack of studies quantifying the sensitivity to horizontal spatial resolution and the physical-dynamical-chemical schemes driving the simulations. Here we investigate model skill in simulating meteorological, chemical and aerosol properties as a function of spatial resolution, by applying the Weather Research and Forecasting model with coupled Chemistry (WRF-Chem) over eastern North America at different resolutions. Using Brier skill scores and other statistical metrics it is shown that enhanced resolution (from 60 to 12 km) improves model performance for all of the meteorological parameters and gas-phase concentrations considered, in addition to both mean and extreme aerosol optical depth (AOD) in three wavelengths in the visible relative to satellite observations, principally via increase of potential skill. Some of the enhanced model performance for AOD appears to be attributable to improved simulation of meteorological conditions and the concentration of key aerosol precursor gases (e.g., SO2 and NH3). Among other reasons, a dry bias in the specific humidity in the boundary layer and a substantial underestimation of total monthly precipitation in the 60 km simulations are identified as causes for the better performance of WRF-Chem simulations at 12 km.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000394610700006
WOS关键词SOUTHEASTERN UNITED-STATES ; RELATIVE-HUMIDITY ; OPTICAL DEPTH ; PHYSICAL PARAMETERIZATIONS ; SUBGRID VARIABILITY ; GEOS-CHEM ; MODEL ; SENSITIVITY ; EMISSIONS ; CHEMISTRY
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/26228
专题地球科学
作者单位1.Newcastle Univ, Sch Civil Engn & Geosci, COMET, Cassie Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England;
2.Cornell Univ, Dept Earth & Atmospher Sci, Bradfield Hall,306 Tower Rd, Ithaca, NY 14853 USA;
3.Indiana Univ, Pervas Technol Inst, Bloomington, IN 47405 USA
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Crippa, Paola,Sullivan, Ryan C.,Thota, Abhinav,et al. The impact of resolution on meteorological, chemical and aerosol properties in regional simulations with WRF-Chem[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(2).
APA Crippa, Paola,Sullivan, Ryan C.,Thota, Abhinav,&Pryor, Sara C..(2017).The impact of resolution on meteorological, chemical and aerosol properties in regional simulations with WRF-Chem.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(2).
MLA Crippa, Paola,et al."The impact of resolution on meteorological, chemical and aerosol properties in regional simulations with WRF-Chem".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.2(2017).
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