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DOI10.5194/acp-18-14445-2018
Air quality in the middle and lower reaches of the Yangtze River channel: a cruise campaign
Li, Zhong1; Li, Chunlin1,2; Ye, Xingnan1; Fu, Hongbo1; Wang, Lin1; Yang, Xin1; Wang, Xinke3; Zhao, Zhuohui4; Kan, Haidong4; Mellouki, Abdelwahid5; Chen, Jianmin1,4
2018-10-10
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:19页码:14445-14464
文章类型Article
语种英语
国家Peoples R China; Israel; France
英文摘要

The Yangtze River is the longest river in China; nearly one-third of the national population lives along the river. Air quality over the Yangtze River is important as it may have significant influences on the aquatic ecosystem, the health of everyone living along the Yangtze River, and regional climate change. Chemical compositions of ambient aerosol were determined during a comprehensive cruise campaign carried out along the mid lower reaches of the Yangtze River (MLYR) in winter of 2015. The total average concentration of PM2.5 was 119.29 +/- 33.67 ittg m(-3), and the dominant ionic composition in PM2.5 was SO42- with an average concentration of 15.21 +/- 6.69 mu g m(-3), followed by NO3- (13.76 +/- 4.99 mu g m(-3)), NH4 (9.38 +/- 4.35 mu g m(-3)), and Ca2+ (2.23 +/- 1.24 mu g m(-3)) in this cruise. Based on the filter samples, the concentration and chemical composition of PM2.5 were remarkably varied or fluctuated from coastal areas to inland over the MLYR region. Crustal elements (Ca, Mg, Al, and K) from floating dust showed peak concentrations in the Yangtze River Delta (YRD) region, while secondary inorganic species (SO42-, NO3-, and NH4+) and some of the most enriched elements (Pb, As, Se, and Cd) presented high levels in central China (Wuhan region). The significant correlation between Se and SO42- suggested that coal combustion may play an important role in secondary inorganic aerosol formation. The relatively high enrichment factors (EFs) of Ca (EFs > 100) suggested the crustal elements may derive from anthropogenic sources. Furthermore, the concentration of levoglucosan in PM2.5 and the CO column level from satellite observation were greatly enhanced in the rural areas (Anhui and Jiangxi), indicating that biomass burning may make a remarkable contribution to rural areas. The concentrations of typical tracer for heavy oil (V and Ni) significantly increased in the Shanghai port, which was mainly ascribed to ship emissions, based on the air mass source analysis and the relatively high ratio of V / Ni as well. The results shown herein portray a good picture of air pollution along the Yangtze River.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000446919300001
WOS关键词NORTH CHINA PLAIN ; CHEMICAL CHARACTERISTICS ; ATMOSPHERIC AEROSOLS ; SOURCE APPORTIONMENT ; SHIP EMISSIONS ; EAST CHINA ; PARTICULATE MATTER ; SOUTHERN CHINA ; FINE PARTICLES ; ORGANIC AEROSOLS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/26182
专题地球科学
作者单位1.Fudan Univ, Inst Atmospher Sci, Shanghai Key Lab Atmospher Particle Pollut & Prev, Fudan Tyndall Ctr,Dept Environm Sci & Engn, Shanghai 200433, Peoples R China;
2.Weizmann Inst Sci, Dept Earth & Planetary Sci, IL-7610001 Rehovot, Israel;
3.Univ Lyon, Univ Claude Bernard Lyon 1, CNRS, IRCELYON, F-69626 Villeurbanne, France;
4.Fudan Univ, Sch Publ Hlth, Shanghai 200032, Peoples R China;
5.CNRS, Inst Combust Aerotherm React & Environm, F-45071 Orleans 2, France
推荐引用方式
GB/T 7714
Li, Zhong,Li, Chunlin,Ye, Xingnan,et al. Air quality in the middle and lower reaches of the Yangtze River channel: a cruise campaign[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(19):14445-14464.
APA Li, Zhong.,Li, Chunlin.,Ye, Xingnan.,Fu, Hongbo.,Wang, Lin.,...&Chen, Jianmin.(2018).Air quality in the middle and lower reaches of the Yangtze River channel: a cruise campaign.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(19),14445-14464.
MLA Li, Zhong,et al."Air quality in the middle and lower reaches of the Yangtze River channel: a cruise campaign".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.19(2018):14445-14464.
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