Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1016/j.atmosres.2020.105020 |
Nocturnal PM2.5 explosive growth dominates severe haze in the rural North China Plain | |
Yaqi Wei, Hui Chen, Hao Sun, Fei Zhang, ... Jianmin Chen | |
2020-05-04 | |
发表期刊 | Atmospheric Research |
出版年 | 2020 |
英文摘要 | The North China Plain (NCP) is the most heavily polluted region in China and the explosive growth (EG) events of PM2.5 frequently occur in winter in this region. A campaign from 17 Nov. 2018 to 1 Mar 2019 was conducted at a rural site in NCP. EG events of PM2.5 were defined as the dynamic increase in PM2.5 concentration by 100 μg/m3 within half day. The intensity of EG events were then graded by the time cost, i.e. 3, 6 and 9 h. EG events with a total number of 120 were identified during the study. Mean growth rates and corresponding standard deviations of PM2.5 of 3 h-, 6 h- and 9 h-EG events were 43.4 ± 6.9, 19.3 ± 1.8 and 12.5 ± 0.5 μg/m3/h, respectively. All of them except one 3 h-EG event occurred with windspeed lower than 2 m/s. Based on the evolution of hourly chemical composition of PM2.5, the EG events were investigated on their formation mechanism. The average mass fraction ratios of SNA (sulphate, SO42−; nitrate, NO3−; ammonium, NH4+) in PM2.5 were 26.3%/18.7%, 32.6%/18.0% and 33.6%/26.9% in 3 h-, 6 h- and 9 h-EG events in the daytime/nighttime, respectively. About two thirds of EG events occurred in the nighttime with a significant increase in the concentrations of organic matter (OM) and chloride (Cl−), which is attributable to nocturnal primary emissions such as coal combustion. In addition, CO-scaled growth rate was calculated as chemical growth rate, the results indicate that OM was the dominant components in EG events. |
领域 | 地球科学 |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/248777 |
专题 | 地球科学 |
推荐引用方式 GB/T 7714 | Yaqi Wei, Hui Chen, Hao Sun, Fei Zhang, ... Jianmin Chen. Nocturnal PM2.5 explosive growth dominates severe haze in the rural North China Plain[J]. Atmospheric Research,2020. |
APA | Yaqi Wei, Hui Chen, Hao Sun, Fei Zhang, ... Jianmin Chen.(2020).Nocturnal PM2.5 explosive growth dominates severe haze in the rural North China Plain.Atmospheric Research. |
MLA | Yaqi Wei, Hui Chen, Hao Sun, Fei Zhang, ... Jianmin Chen."Nocturnal PM2.5 explosive growth dominates severe haze in the rural North China Plain".Atmospheric Research (2020). |
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