GSTDTAP  > 地球科学
DOI10.5194/acp-17-12197-2017
Aerosols at the poles: an AeroCom Phase II multi-model evaluation
Sand, Maria1,2,3; Samset, Bjorn H.1; Balkanski, Yves4; Bauer, Susanne2,3; Bellouin, Nicolas5; Berntsen, Terje K.1,6; Bian, Huisheng7; Chin, Mian8; Diehl, Thomas9; Easter, Richard10; Ghan, Steven J.10; Iversen, Trond11; Kirkevag, Alf11; Lamarque, Jean-Francois12; Lin, Guangxing10; Liu, Xiaohong13; Luo, Gan14; Myhre, Gunnar1; van Noije, Twan15; Penner, Joyce E.16; Schulz, Michael11; Seland, Oyvind11; Skeie, Ragnhild B.1; Stier, Philip17; Takemura, Toshihiko18; Tsigaridis, Kostas2,3; Yu, Fangqun14; Zhang, Kai10,19; Zhang, Hua20
2017-10-13
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2017
卷号17期号:19
文章类型Article
语种英语
国家Norway; USA; France; England; Italy; Netherlands; Japan; Germany; Peoples R China
英文摘要

Atmospheric aerosols from anthropogenic and natural sources reach the polar regions through long-range transport and affect the local radiation balance. Such transport is, however, poorly constrained in present-day global climate models, and few multi-model evaluations of polar anthropogenic aerosol radiative forcing exist. Here we compare the aerosol optical depth (AOD) at 550 nm from simulations with 16 global aerosol models from the AeroCom Phase II model intercomparison project with available observations at both poles. We show that the annual mean multi-model median is representative of the observations in Arctic, but that the intermodel spread is large. We also document the geographical distribution and seasonal cycle of the AOD for the individual aerosol species: black carbon (BC) from fossil fuel and biomass burning, sulfate, organic aerosols (OAs), dust, and sea-salt. For a subset of models that represent nitrate and secondary organic aerosols (SOAs), we document the role of these aerosols at high latitudes.


The seasonal dependence of natural and anthropogenic aerosols differs with natural aerosols peaking in winter (sea-salt) and spring (dust), whereas AOD from anthropogenic aerosols peaks in late spring and summer. The models produce a median annual mean AOD of 0.07 in the Arctic (defined here as north of 60 degrees N). The models also predict a noteworthy aerosol transport to the Antarctic (south of 70 degrees S) with a resulting AOD varying between 0.01 and 0.02. The models have estimated the shortwave anthropogenic radiative forcing contributions to the direct aerosol effect (DAE) associated with BC and OA from fossil fuel and biofuel (FF), sulfate, SOAs, nitrate, and biomass burning from BC and OA emissions combined. The Arctic modelled annual mean DAE is slightly negative ( -0.12Wm(-2)), dominated by a positive BC FF DAE in spring and a negative sulfate DAE in summer. The Antarctic DAE is governed by BC FF. We perform sensitivity experiments with one of the AeroCom models (GISS modelE) to investigate how regional emissions of BC and sulfate and the lifetime of BC influence the Arctic and Antarctic AOD. A doubling of emissions in eastern Asia results in a 33% increase in Arctic AOD of BC. A doubling of the BC lifetime results in a 39% increase in Arctic AOD of BC. However, these radical changes still fall within the AeroCom model range.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000412937900001
WOS关键词COMMUNITY ATMOSPHERE MODEL ; BLACK CARBON ; CLIMATE RESPONSE ; OPTICAL DEPTH ; SEA-ICE ; TROPOSPHERIC AEROSOLS ; VERTICAL-DISTRIBUTION ; GLOBAL CLIMATE ; AIR-POLLUTION ; ARCTIC-OCEAN
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/23854
专题地球科学
作者单位1.CICERO, Oslo, Norway;
2.NASA, Goddard Inst Space Studies, New York, NY 10025 USA;
3.NASA, Columbia Earth Inst, New York, NY 10025 USA;
4.CEA CNRS UVSQ, Lab Sci Climat & Environm, Gif Sur Yvette, France;
5.Univ Reading, Dept Meteorol, Reading, Berks, England;
6.Univ Oslo, Dept Geosci, Oslo, Norway;
7.Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA;
8.NASA, Goddard Space Flight Ctr, Greenbelt, MD USA;
9.European Commiss, Joint Res Ctr, Directorate Sustainable Resources, Ispra, Italy;
10.Pacific Northwest Natl Lab, Richland, WA USA;
11.Norwegian Meteorol Inst, Oslo, Norway;
12.Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA;
13.Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA;
14.SUNY Albany, Atmospher Sci Res Ctr, Albany, NY 12222 USA;
15.Royal Netherlands Meteorol Inst, De Bilt, Netherlands;
16.Univ Michigan, Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA;
17.Univ Oxford, Dept Phys, Oxford, England;
18.Kyushu Univ, Res Inst Appl Mech, Fukuoka, Japan;
19.Max Planck Inst Meteorol, Hamburg, Germany;
20.China Meteorol Adm, Natl Climate Ctr, Lab Climate Studies, Beijing, Peoples R China
推荐引用方式
GB/T 7714
Sand, Maria,Samset, Bjorn H.,Balkanski, Yves,et al. Aerosols at the poles: an AeroCom Phase II multi-model evaluation[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(19).
APA Sand, Maria.,Samset, Bjorn H..,Balkanski, Yves.,Bauer, Susanne.,Bellouin, Nicolas.,...&Zhang, Hua.(2017).Aerosols at the poles: an AeroCom Phase II multi-model evaluation.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(19).
MLA Sand, Maria,et al."Aerosols at the poles: an AeroCom Phase II multi-model evaluation".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.19(2017).
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