Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-18-2049-2018 |
High-resolution sampling and analysis of ambient particulate matter in the Pearl River Delta region of southern China: source apportionment and health risk implications | |
Zhou, Shengzhen1,2; Davy, Perry K.3; Huang, Minjuan1; Duan, Jingbo4; Wang, Xuemei1,5; Fan, Qi1; Chang, Ming5; Liu, Yiming1; Chen, Weihua1; Xie, Shanju6; Ancelet, Travis3; Trompetter, William J.3 | |
2018-02-13 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2018 |
卷号 | 18期号:3页码:2049-2064 |
文章类型 | Article |
语种 | 英语 |
国家 | Peoples R China; New Zealand |
英文摘要 | Hazardous air pollutants, such as trace elements in particulate matter (PM), are known or highly suspected to cause detrimental effects on human health. To understand the sources and associated risks of PM to human health, hourly time-integrated major trace elements in size-segregated coarse (PM2.5-10) and fine (PM2.5) particulate matter were collected at the industrial city of Foshan in the Pearl River Delta region, China. Receptor modeling of the data set by positive matrix factorization (PMF) was used to identify six sources contributing to PM2.5 and PM10 concentrations at the site. Dominant sources included industrial coal combustion, secondary inorganic aerosol, motor vehicles and construction dust along with two intermittent sources (biomass combustion and marine aerosol). The biomass combustion source was found to be a significant contributor to peak PM2 : 5 episodes along with motor vehicles and industrial coal combustion. Conditional probability function (CPF) analysis was applied to estimate the source locations using the PMF-resolved source contribution coupled with the surface wind direction data. Health exposure risk of hazardous trace elements (Pb, As, Si, Cr, Mn and Ni) and source-specific values were estimated. The total hazard quotient (HQ) of PM2.5 was 2.09, higher than the acceptable limit (HQ = 1). The total carcinogenic risk (CR) was 3.37 x 10(-3) for PM2.5, which was 3 times higher than the least stringent limit (1.0 x 10(-4)). Among the selected trace elements, As and Pb posed the highest non-carcinogenic and carcinogenic risks to human health, respectively. In addition, our results show that the industrial coal combustion source is the dominant non-carcinogenic and carcinogenic risk contributor, highlighting the need for stringent control of this source. This study provides new insight for policy makers to prioritize sources in air quality management and health risk reduction. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000424928100003 |
WOS关键词 | POSITIVE MATRIX FACTORIZATION ; TRACE-ELEMENTS ; AIR-QUALITY ; ATMOSPHERIC AEROSOL ; BLACK CARBON ; ESTIMATING UNCERTAINTY ; CHEMICAL-COMPOSITION ; STREAKER SAMPLERS ; COARSE PARTICLES ; FINE-PARTICLE |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/21714 |
专题 | 地球科学 |
作者单位 | 1.Sun Yat Sen Univ, Sch Atmospher Sci, Guangzhou 510275, Guangdong, Peoples R China; 2.Sun Yat Sen Univ, Guangdong Prov Key Lab Climate Change & Nat Disas, Guangzhou 510275, Guangdong, Peoples R China; 3.Inst Geol & Nucl Sci, Natl Isotope Ctr, 30 Gracefield Rd,POB 31312, Lower Hutt, New Zealand; 4.Chinese Acad Sci, Key Lab Environm Opt & Technol, Anhui Inst Opt & Fine Mech, 350 Shu Shan Hu Rd, Hefei 230031, Anhui, Peoples R China; 5.Jinan Univ, Inst Environm & Climate Res, Guangzhou, Guangdong, Peoples R China; 6.Auckland Council, Auckland, New Zealand |
推荐引用方式 GB/T 7714 | Zhou, Shengzhen,Davy, Perry K.,Huang, Minjuan,et al. High-resolution sampling and analysis of ambient particulate matter in the Pearl River Delta region of southern China: source apportionment and health risk implications[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(3):2049-2064. |
APA | Zhou, Shengzhen.,Davy, Perry K..,Huang, Minjuan.,Duan, Jingbo.,Wang, Xuemei.,...&Trompetter, William J..(2018).High-resolution sampling and analysis of ambient particulate matter in the Pearl River Delta region of southern China: source apportionment and health risk implications.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(3),2049-2064. |
MLA | Zhou, Shengzhen,et al."High-resolution sampling and analysis of ambient particulate matter in the Pearl River Delta region of southern China: source apportionment and health risk implications".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.3(2018):2049-2064. |
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