GSTDTAP  > 地球科学
DOI10.5194/acp-18-11599-2018
Seasonality of aerosol optical properties in the Arctic
Schmeisser, Lauren1,3,9; Backman, John2; Ogren, John A.1,3; Andrews, Elisabeth1; Asmi, Eija2; Starkweather, Sandra1,3; Uttal, Taneil3; Fiebig, Markus4; Sharma, Sangeeta5; Eleftheriadis, Kostas6; Vratolis, Stergios6; Bergin, Michael7; Tunved, Peter8; Jefferson, Anne1
2018-08-16
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:16页码:11599-11622
文章类型Article
语种英语
国家USA; Finland; Norway; Canada; Greece; Sweden
英文摘要

Given the sensitivity of the Arctic climate to short-lived climate forcers, long-term in situ surface measurements of aerosol parameters are useful in gaining insight into the magnitude and variability of these climate forcings. Seasonality of aerosol optical properties - including the aerosol light-scattering coefficient, absorption coefficient, single-scattering albedo, scattering Angstrom exponent, and asymmetry parameter - are presented for six monitoring sites throughout the Arctic: Alert, Canada; Barrow, USA; Pallas, Finland; Summit, Greenland; Tiksi, Russia; and Zeppelin Mountain, Ny-Alesund, Svalbard, Norway. Results show annual variability in all parameters, though the seasonality of each aerosol optical property varies from site to site. There is a large diversity in magnitude and variability of scattering coefficient at all sites, reflecting differences in aerosol source, transport, and removal at different locations throughout the Arctic. Of the Arctic sites, the highest annual mean scattering coefficient is measured at Tiksi (12.47 Mm(-1)), and the lowest annual mean scattering coefficient is measured at Summit (1.74 Mm(-1)). At most sites, aerosol absorption peaks in the winter and spring, and has a minimum throughout the Arctic in the summer, indicative of the Arctic haze phenomenon; however, nuanced variations in seasonalities suggest that this phenomenon is not identically observed in all regions of the Arctic. The highest annual mean absorption coefficient is measured at Pallas (0.48 Mm(-1)), and Summit has the lowest annual mean absorption coefficient (0.12 Mm(-1)). At the Arctic monitoring stations analyzed here, mean annual single-scattering albedo ranges from 0.909 (at Pallas) to 0.960 (at Barrow), the mean annual scattering Angstrom exponent ranges from 1.04 (at Barrow) to 1.80 (at Summit), and the mean asymmetry parameter ranges from 0.57 (at Alert) to 0.75 (at Summit). Systematic variability of aerosol optical properties in the Arctic supports the notion that the sites presented here measure a variety of aerosol populations, which also experience different removal mechanisms. A robust conclusion from the seasonal cycles presented is that the Arctic cannot be treated as one common and uniform environment but rather is a region with ample spatiotemporal variability in aerosols. This notion is important in considering the design or aerosol monitoring networks in the region and is important for informing climate models to better represent short-lived aerosol climate forcers in order to yield more accurate climate predictions for the Arctic.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000441783700003
WOS关键词FILTER-BASED MEASUREMENTS ; VISIBLE-LIGHT ABSORPTION ; LONG-TERM TRENDS ; BLACK CARBON ; SEA-ICE ; ATMOSPHERIC TRANSPORT ; RADIATIVE PROPERTIES ; SIZE DISTRIBUTION ; CLIMATE-CHANGE ; AIR-POLLUTION
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/21637
专题地球科学
作者单位1.Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA;
2.Finnish Meteorol Inst, Atmospher Composit Res, Helsinki, Finland;
3.NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA;
4.Norwegian Inst Air Res, Kjeller, Norway;
5.Environm & Climate Change Canada, Climate Res Div, Sci & Technol Branch, Toronto, ON, Canada;
6.NCSR Demokritos, Environm Radioact Lab, Inst Nucl & Radiol Sci & Technol, Energy & Safety, Athens, Greece;
7.Duke Univ, Dept Civil & Environm Engn, Durham, NC 27706 USA;
8.Stockholm Univ, Dept Environm Sci & Analyt Chem, Stockholm, Sweden;
9.Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA
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GB/T 7714
Schmeisser, Lauren,Backman, John,Ogren, John A.,et al. Seasonality of aerosol optical properties in the Arctic[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(16):11599-11622.
APA Schmeisser, Lauren.,Backman, John.,Ogren, John A..,Andrews, Elisabeth.,Asmi, Eija.,...&Jefferson, Anne.(2018).Seasonality of aerosol optical properties in the Arctic.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(16),11599-11622.
MLA Schmeisser, Lauren,et al."Seasonality of aerosol optical properties in the Arctic".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.16(2018):11599-11622.
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