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DOI10.1073/pnas.1811282116
K isotopes as a tracer for continental weathering and geological K cycling
Li, Shilei1,2; Li, Weiqiang3; Beard, Brian L.4,5; Raymo, Maureen E.2; Wang, Xiaomin3; Chen, Yang1; Chen, Jun1
2019
发表期刊PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
ISSN0027-8424
出版年2019
卷号116期号:18页码:8740-8745
文章类型Article
语种英语
国家Peoples R China; USA
英文摘要

The causal effects among uplift, climate, and continental weathering cannot be fully addressed using presently available geochemical proxies. However, stable potassium (K) isotopes can potentially overcome the limitations of existing isotopic proxies. Here we report on a systematic investigation of K isotopes in dissolved load and sediments from major rivers and their tributaries in China, which have drainage basins with varied climate, lithology, and topography. Our results show that during silicate weathering, heavy K isotopes are preferentially partitioned into aqueous solutions. Moreover, delta K-41 values of riverine dissolved load vary remarkably and correlate negatively with the chemical weathering intensity of the drainage basin. This correlation allows an estimate of the average K isotope composition of global riverine runoff (delta K-41 = -0.22 parts per thousand), as well as modeling of the global K cycle based on mass balance calculations. Modeling incorporating K isotope mass balance better constrains estimated K fluxes for modern global K cycling, and the results show that the delta K-41 value of seawater is sensitive to continental weathering intensity changes. Thus, it is possible to use the delta K-41 record of paleo-seawater to infer continental weathering intensity through Earth's history.


英文关键词continental weathering K isotopes rivers fractionation K cycling
领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000466446500021
WOS关键词CO2 CONSUMPTION ; CHEMICAL-COMPOSITION ; CARBON-DIOXIDE ; POTASSIUM ; RIVER ; GEOCHEMISTRY ; FLUXES ; SEA ; SEAWATER ; RECORD
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/205102
专题地球科学
资源环境科学
气候变化
作者单位1.Nanjing Univ, Sch Earth Sci & Engn, Key Lab Surficial Geochem, Minist Educ, Nanjing 210023, Jiangsu, Peoples R China;
2.Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY 10964 USA;
3.Nanjing Univ, Sch Earth Sci & Engn, State Key Lab Mineral Deposits Res, Nanjing 210093, Jiangsu, Peoples R China;
4.Univ Wisconsin, Dept Geosci, Madison, WI 53706 USA;
5.Univ Wisconsin, NASA, Astrobiol Inst, Madison, WI 53706 USA
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Li, Shilei,Li, Weiqiang,Beard, Brian L.,et al. K isotopes as a tracer for continental weathering and geological K cycling[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2019,116(18):8740-8745.
APA Li, Shilei.,Li, Weiqiang.,Beard, Brian L..,Raymo, Maureen E..,Wang, Xiaomin.,...&Chen, Jun.(2019).K isotopes as a tracer for continental weathering and geological K cycling.PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,116(18),8740-8745.
MLA Li, Shilei,et al."K isotopes as a tracer for continental weathering and geological K cycling".PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 116.18(2019):8740-8745.
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