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DOI | 10.1038/s41467-018-05934-7 |
Copolymer dielectrics with balanced chain-packing density and surface polarity for high-performance flexible organic electronics | |
Ji, Deyang1,2; Li, Tao3; Zou, Ye4; Chu, Ming5; Zhou, Ke4; Liu, Jinyu4; Tian, Guofeng6; Zhang, Zhaoyang3; Zhang, Xu3; Li, Liqiang7; Wu, Dezhen6; Dong, Huanli4; Miao, Qian5; Fuchs, Harald1,2; Hu, Wenping8,9 | |
2018-06-14 | |
发表期刊 | NATURE COMMUNICATIONS
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ISSN | 2041-1723 |
出版年 | 2018 |
卷号 | 9 |
文章类型 | Article |
语种 | 英语 |
国家 | Germany; Peoples R China |
英文摘要 | The ever-increasing demand for flexible electronics calls for the development of low-voltage and high-mobility organic thin-film transistors (OTFTs) that can be integrated into emerging display and labeling technologies. Polymer dielectrics with comprehensive and balanced dielectric properties (i.e., a good balance between their insulating characteristics and compatibility with organic semiconductors) are considered particularly important for this end. Here, we introduce a simple but highly efficient strategy to realize this target by using a new type of copolymer as dielectrics. Benefiting from both high chain packing density guaranteeing dielectric properties and surface polarity optimizing molecular packing of organic semiconductors, this rationally designed copolymer dielectric endows flexible OTFTs with high mobility (5.6 cm(2) V-1 s(-1)), low operating voltage (3 V) and outstanding stability. Further, their applicability in integrated circuits is verified. The excellent device performance shows exciting prospects of this molecular-scale engineered copolymer for the realization of plastic high-performance integrated electronics. |
领域 | 资源环境 |
收录类别 | SCI-E |
WOS记录号 | WOS:000435341000003 |
WOS关键词 | FIELD-EFFECT TRANSISTORS ; THIN-FILM TRANSISTORS ; POLYIMIDE GATE INSULATORS ; HIGH-MOBILITY ; LOW-VOLTAGE ; PHOTOSENSITIVE POLYIMIDE ; SEMICONDUCTOR ; MORPHOLOGY ; ENERGY ; HOLE |
WOS类目 | Multidisciplinary Sciences |
WOS研究方向 | Science & Technology - Other Topics |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/203970 |
专题 | 资源环境科学 |
作者单位 | 1.Westfalische Wilhelms Univ, Phys Inst, Wilhelm Klemm Str 10, D-48149 Munster, Germany; 2.Ctr Nanotechnol, Heisenbergstr 11, D-48149 Munster, Germany; 3.Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai Key Lab Elect Insulat & Thermal Aging, Shanghai 200240, Peoples R China; 4.Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China; 5.Chinese Univ Hong Kong, Dept Chem, Shatin, Hong Kong, Peoples R China; 6.Beijing Univ Chem Technol, Beijing 100029, Peoples R China; 7.Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion SINANO, Adv Nanomat Div, Suzhou 215123, Peoples R China; 8.Tianjin Univ, Dept Chem, Sch Sci, Tianjin Key Lab Mol Optoelect Sci, Tianjin 300072, Peoples R China; 9.Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China |
推荐引用方式 GB/T 7714 | Ji, Deyang,Li, Tao,Zou, Ye,et al. Copolymer dielectrics with balanced chain-packing density and surface polarity for high-performance flexible organic electronics[J]. NATURE COMMUNICATIONS,2018,9. |
APA | Ji, Deyang.,Li, Tao.,Zou, Ye.,Chu, Ming.,Zhou, Ke.,...&Hu, Wenping.(2018).Copolymer dielectrics with balanced chain-packing density and surface polarity for high-performance flexible organic electronics.NATURE COMMUNICATIONS,9. |
MLA | Ji, Deyang,et al."Copolymer dielectrics with balanced chain-packing density and surface polarity for high-performance flexible organic electronics".NATURE COMMUNICATIONS 9(2018). |
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