GSTDTAP  > 地球科学
DOI10.1126/science.aax3489
Sub-single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity
Kozlov, Oleg V.1; Park, Young-Shin1,2; Roh, Jeongkyun1; Fedin, Igor1; Nakotte, Tom1,3; Klimov, Victor I.1
2019-08-16
发表期刊SCIENCE
ISSN0036-8075
EISSN1095-9203
出版年2019
卷号365期号:6454页码:672-+
文章类型Article
语种英语
国家USA
英文摘要

Colloidal semiconductor quantum dots (QDs) are attractive materials for realizing highly flexible, solution-processable optical gain media, but they are difficult to use in lasing because of complications associated with extremely short optical-gain lifetimes limited by nonradiative Auger recombination. By combining compositional grading of the QD's interior for hindering Auger decay with postsynthetic charging for suppressing parasitic ground-state absorption, we can reduce the lasing threshold to values below the single-exciton-per-dot limit. As a favorable departure from traditional multi-exciton-based lasing schemes, our approach should facilitate the development of solution-processable lasing devices and thereby help to extend the reach of lasing technologies into areas not accessible with traditional, epitaxially grown semiconductor materials.


领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000481688700042
WOS关键词OPTICAL GAIN ; EMISSION
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/202088
专题地球科学
资源环境科学
气候变化
作者单位1.Los Alamos Natl Lab, Chem Div, C PCS, Los Alamos, NM 87545 USA;
2.Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87131 USA;
3.New Mexico State Univ, Dept Chem & Mat Engn, Las Cruces, NM 88003 USA
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Kozlov, Oleg V.,Park, Young-Shin,Roh, Jeongkyun,et al. Sub-single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity[J]. SCIENCE,2019,365(6454):672-+.
APA Kozlov, Oleg V.,Park, Young-Shin,Roh, Jeongkyun,Fedin, Igor,Nakotte, Tom,&Klimov, Victor I..(2019).Sub-single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity.SCIENCE,365(6454),672-+.
MLA Kozlov, Oleg V.,et al."Sub-single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity".SCIENCE 365.6454(2019):672-+.
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