GSTDTAP  > 地球科学
DOI10.1126/science.aax1748
Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume
Yu, Pengfei1,2,3; Toon, Owen B.4,5; Bardeen, Charles G.6; Zhu, Yunqian5; Rosenlof, Karen H.2; Portmann, Robert W.2; Thornberry, Troy D.1,2; Gao, Ru-Shan2; Davis, Sean M.2; Wolf, Eric T.5,7; de Gouw, Joost1,8; Peterson, David A.9; Fromm, Michael D.10; Robock, Alan11
2019-08-09
发表期刊SCIENCE
ISSN0036-8075
EISSN1095-9203
出版年2019
卷号365期号:6453页码:587-590
文章类型Article
语种英语
国家USA; Peoples R China
英文摘要

In 2017, western Canadian wildfires injected smoke into the stratosphere that was detectable by satellites for more than 8 months. The smoke plume rose from 12 to 23 kilometers within 2 months owing to solar heating of black carbon, extending the lifetime and latitudinal spread. Comparisons of model simulations to the rate of observed lofting indicate that 2% of the smoke mass was black carbon. The observed smoke lifetime in the stratosphere was 40% shorter than calculated with a standard model that does not consider photochemical loss of organic carbon. Photochemistry is represented by using an empirical ozone-organics reaction probability that matches the observed smoke decay. The observed rapid plume rise, latitudinal spread, and photochemical reactions provide new insights into potential global climate impacts from nuclear war.


领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000483195200039
WOS关键词OZONE ; CONSEQUENCES ; SENSITIVITY ; MODEL
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/202041
专题地球科学
资源环境科学
气候变化
作者单位1.Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA;
2.NOAA, Earth Syst Res Lab, Boulder, CO USA;
3.Jinan Univ, Inst Environm & Climate Res, Guangzhou, Guangdong, Peoples R China;
4.Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA;
5.Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80309 USA;
6.Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA;
7.Virtual Planetary Lab, Seattle, WA 98195 USA;
8.Univ Colorado, Dept Chem, Boulder, CO 80309 USA;
9.Naval Res Lab, Monterey, CA 93943 USA;
10.Naval Res Lab, Washington, DC 20375 USA;
11.Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ USA
推荐引用方式
GB/T 7714
Yu, Pengfei,Toon, Owen B.,Bardeen, Charles G.,et al. Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume[J]. SCIENCE,2019,365(6453):587-590.
APA Yu, Pengfei.,Toon, Owen B..,Bardeen, Charles G..,Zhu, Yunqian.,Rosenlof, Karen H..,...&Robock, Alan.(2019).Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume.SCIENCE,365(6453),587-590.
MLA Yu, Pengfei,et al."Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume".SCIENCE 365.6453(2019):587-590.
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