GSTDTAP  > 地球科学
DOI10.1126/science.aan8721
State-to-state chemistry for three-body recombination in an ultracold rubidium gas
Wolf, Joschka1; 39;Incao, Jose P.2
2017-11-17
发表期刊SCIENCE
ISSN0036-8075
EISSN1095-9203
出版年2017
卷号358期号:6365页码:921-924
文章类型Article
语种英语
国家Germany; USA
英文摘要

Experimental investigation of chemical reactions with full quantum state resolution for all reactants and products has been a long-term challenge. Here we prepare an ultracold few-body quantum state of reactants and demonstrate state-to-state chemistry for the recombination of three spin-polarized ultracold rubidium (Rb) atoms to form a weakly bound Rb-2 molecule. The measured product distribution covers about 90% of the final products, and we are able to discriminate between product states with a level splitting as small as 20 megahertz multiplied by Planck's constant. Furthermore, we formulate propensity rules for the distribution of products, and we develop a theoretical model that predicts many of our experimental observations. The scheme can readily be adapted to other species and opens a door to detailed investigations of inelastic or reactive processes.


领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000415293000046
WOS关键词ATOMS ; SPECTROSCOPY ; COLLISIONS ; MOLECULES ; DYNAMICS ; DECAY ; COLD
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/197348
专题地球科学
资源环境科学
气候变化
作者单位1.Univ Ulm, Inst Quantenmaterie, D-89069 Ulm, Germany;
2.Univ Ulm, Ctr Integrated Quantum Sci & Technol IQST, D-89069 Ulm, Germany;
3.Leibniz Univ Hannover, Inst Quantenopt, D-30167 Hannover, Germany;
4.Univ Maryland, Joint Quantum Inst, College Pk, MD 20742 USA;
5.NIST, College Pk, MD 20742 USA;
6.Amer Phys Soc, Ridge, NY 11961 USA;
7.Univ Colorado, NIST, JILA, Boulder, CO 80309 USA;
8.Univ Colorado, Dept Phys, Boulder, CO 80309 USA
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GB/T 7714
Wolf, Joschka,39;Incao, Jose P.. State-to-state chemistry for three-body recombination in an ultracold rubidium gas[J]. SCIENCE,2017,358(6365):921-924.
APA Wolf, Joschka,&39;Incao, Jose P..(2017).State-to-state chemistry for three-body recombination in an ultracold rubidium gas.SCIENCE,358(6365),921-924.
MLA Wolf, Joschka,et al."State-to-state chemistry for three-body recombination in an ultracold rubidium gas".SCIENCE 358.6365(2017):921-924.
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